相关论文: Photon Statistics for Single Molecule Non-Linear S…
In this research, we employ accurate time-dependent density functional calculations for ultrashort laser spectroscopy of nitrogen molecule. Laser pulses with different frequencies, intensities, and durations are applied to the molecule and…
We propose and demonstrate a method for measuring the spectral density matrix of a single photon pulse. The method is based on registering Hong-Ou-Mandel interference between photon to be measured and a pair of attenuated and suitably…
The modulational instability of broadband optical pulses in a four-state atomic system is investigated. In particular, starting from a recently derived generalized nonlinear Schr\"odinger equation, a wave-kinetic equation is derived. A…
In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…
Attosecond spectroscopy comprises several techniques to probe matter through electrons and photons. One frontier of attosecond methods is to reveal complex phenomena arising from quantum-mechanical correlations in the matter system, in the…
We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…
The working principles of linear optical quantum computing are based on photodetection, namely, projective measurements. The use of photodetection can provide efficient nonlinear interactions between photons at the single-photon level,…
We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical…
The boson sampling problem has triggered a lot of interest in the scientific community because of its potential of demonstrating the computational power of quantum interference without the need of non-linear processes. However, the…
We present a new concept of nonlinear dynamics of incoherent superstrong radiation in plasmas. Recently we have disclosed a novel mechanism of the establishment of equilibrium between a photon and a dense photon bunch through the exchange…
Measuring the power spectral density of a stochastic process, such as a stochastic force or magnetic field, is a fundamental task in many sensing applications. Quantum noise is becoming a major limiting factor to such a task in future…
We present an optical study of closely-spaced self-assembled InAs/GaAs quantum dots. The energy spectrum and correlations between photons subsequently emitted from a single pair provide not only clear evidence of coupling between the…
We report the results of coincidence counting experiments at the output of a Michelson interferometer using the zero-phonon-line emission of a single molecule at $1.4 K$. Under continuous wave excitation, we observe the absence of…
High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…
In this paper, we extend the results of an earlier paper in which we had demonstrated the limitations of the notion of non-resonant multiphoton ionization, in the exploration of photon statistics effects in non-linear processes. Through the…
Based on the four wave mixing, a three mode nonlinear system is proposed. The single photon blockade is discussed through analytical analysis and numerical calculation. The analytical analysis shows that the conventional photon blockade and…
We demonstrate two solid-state sources of indistinguishable single photons. High resolution laser spectroscopy and optical microscopy were combined at T = 1.4 K to identify individual molecules in two independent microscopes. The Stark…
Nonlinear optical processes are used in biological microscopy to surpass the diffraction limit on resolution, image deeper into brain tissues, and identify biomolecules without exogenous labels. These techniques typically require high…
When a laser cavity supports the propagation of several ultrashort pulses, these pulses interact and can form compact bound states called soliton molecules. Soliton molecules are fascinating objects of nonlinear science, which present…
We study the nonlinear mean-field dynamics of molecule formation at coherent photo- and magneto-association of an atomic Bose-Einstein condensate for the case when the external field configuration is defined by the quasi-linear level…