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We present a microscopic theory of single-electron tunneling through metallic nanoparticles connected to the electrodes through molecular bridges. It combines the theory of electron transport through molecular junctions with the description…

介观与纳米尺度物理 · 物理学 2009-11-10 Yongqiang Xue , Mark A. Ratner

The effects of different contact geometries, bond dimerization, and gate voltage on quantum transport through a C$_{60}$ molecule are studied by the Landauer-B\"{u}ttiker formula based on the Green's function technique. It is shown that the…

介观与纳米尺度物理 · 物理学 2008-08-12 Alireza Saffarzadeh

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

介观与纳米尺度物理 · 物理学 2013-02-18 R. Härtle , M. Butzin , M. Thoss

Single-molecule biosensing, with a promise of being applied in protein and DNA sequencing, could be achieved using tunneling current approach. Electrode-molecule-electrode tunneling current critically depends on whether molecular levels…

A theory of electrical transport through molecular wires is used to estimate the electronic factor in the intramolecular electron transfer (ET) in porphyrin-nitrobenzene supermolecules, and to analyze its structure. The chosen molecules…

软凝聚态物质 · 物理学 2007-05-23 Natalya Zimbovskaya , Godfrey Gumbs

We present a conceptually simple method for treating electron-phonon scattering and phonon limited mobilities. By combining Green's function based transport calculations and molecular dynamics (MD), we obtain a temperature dependent…

介观与纳米尺度物理 · 物理学 2017-06-28 Troels Markussen , Mattias Palsgaard , Daniele Stradi , Tue Gunst , Mads Brandbyge , Kurt Stokbro

Achieving highly transmitting molecular junctions through resonant transport at low bias is key to the next-generation low-power molecular devices. Although, resonant transport in molecular junctions was observed by connecting a molecule…

For adjusting the charging state of a molecular metal complex in the context of a density functional theory description of coherent electron transport through single molecule junctions, we correct for self interaction effects by fixing the…

介观与纳米尺度物理 · 物理学 2015-06-12 Georg Kastlunger , Robert Stadler

We investigate the effect on molecular transport due to the different structural aspects of metal-molecule interfaces. The example system chosen is the prototypical molecular device formed by sandwiching the phenyl dithiolate molecule (PDT)…

介观与纳米尺度物理 · 物理学 2009-11-10 Yongqiang Xue , Mark Ratner

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

介观与纳米尺度物理 · 物理学 2012-12-18 Muhammad Imran

We describe a first-principles method for calculating electronic structure, vibrational modes and frequencies, electron-phonon couplings, and inelastic electron transport properties of an atomic-scale device bridging two metallic contacts…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Magnus Paulsson , Mads Brandbyge , Antti-Pekka Jauho

We study the electrical modulation of the transport properties of silicene constrictions with different geometrical structures by adopting the tight-binding model and non-equilibrium Green's function method. The band structure and…

介观与纳米尺度物理 · 物理学 2022-06-17 Yawen Guo , Wenqi Jiang , Xinru Wang , Yijing Bai , Fei Wan , Guanqing Wang , Yuan Li

We study lateral tunneling through a quantum box including electron-electron interactions in the presence of a magnetic field which breaks single particle degeneracies. The conductance at zero temperature as a function of the Fermi energy…

凝聚态物理 · 物理学 2009-10-22 J. J. Palacios , L. Martin-Moreno , C. Tejedor

It is understood that molecular conjugation plays an important role in charge transport through single-molecule junctions. Here, we investigate electron transport through an anthraquinone based single-molecule three-terminal device. With…

介观与纳米尺度物理 · 物理学 2016-05-19 M. Koole , J. M. Thijssen , H. Valkenier , J. C. Hummelen , H. S. J. van der Zant

Interference effects strongly affect the transport characteristics of a benzene single-electron transistor (SET) and for this reason we call it interference SET (I-SET). We focus on the effects of degeneracies between many-body states of…

强关联电子 · 物理学 2009-07-01 D. Darau , G. Begemann , A. Donarini , M. Grifoni

We analyze non-equilibrium current transport in molecular electronic devices, using as an example devices formed by two terphenyl dithiol molecules attached to gold electrodes. Using a first-principles based self-consistent matrix Green's…

介观与纳米尺度物理 · 物理学 2009-11-10 Yongqiang Xue , Mark A. Ratner

We demonstrate a new class of molecules for exceptional performance in molecular electronics and spintronics. Phenalenyl-based radicals are stable radicals whose electronic properties can be tuned readily by heteroatom substitution. We…

介观与纳米尺度物理 · 物理学 2021-11-24 Manuel Smeu , Oliver L. A. Monti , Dominic McGrath

Transport in molecular electronic devices is different from that in semiconductor mesoscopic devices in two important aspects: (1) the effect of the electronic structure and (2) the effect of the interface to the external contact. A…

介观与纳米尺度物理 · 物理学 2009-11-07 Yongqiang Xue , Supriyo Datta , Mark A. Ratner

We investigate the conformation-dependent electron transfer in a biphenyl molecule within a simple tight-binding framework. The overall junction current and circular currents in two benzene rings driven by applied bias voltage are…

介观与纳米尺度物理 · 物理学 2013-07-02 Santanu K. Maiti

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , M. Thoss