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The field-induced multiferroic transition in TbMnO3 has been studied by neutron scattering. Apart strong hysteresis, the magnetic transition associated with the flop of electronic polarization exhibits a memory effect: after a field sweep,…

强关联电子 · 物理学 2009-11-13 D. Senff , P. Link , N. Aliouane , D. N. Argyriou , M. Braden

Single-crystal synchrotron x-ray diffraction measurements in strong magnetic fields have been performed for magnetoelectric compounds GdMnO3 and TbMnO3. It has been found that the P || a ferroelectric phase induced by the application of a…

强关联电子 · 物理学 2007-05-23 T. Arima , T. Goto , Y. Yamasaki , S. Miyasaka , K. Ishii , M. Tsubota , T. Inami , Y. Murakami , Y. Tokura

Using in-field single crystal neutron diffraction we have determined the magnetic structure of TbMnO3 in the high field P||a phase. We unambiguously establish that the ferroelectric polarization arises from a cycloidal Mn spins ordering,…

强关联电子 · 物理学 2010-07-20 N. Aliouane , K. Schmalzl , D. Senff , A. Maljuk , K. Prokes , M. Braden , D. N. Argyriou

The relationship between magnetic order and ferroelectric properties has been investigated for MnWO$_4$ with long-wavelength magnetic structure. Spontaneous electric polarization is observed in an elliptical spiral spin phase. The…

强关联电子 · 物理学 2009-11-11 K. Taniguchi , N. Abe , T. Takenobu , Y. Iwasa , T. Arima

We review the phenomenology of coupled magnetic and electric order parameters for systems in which ferroelectric and incommensurate magnetic order occur simultaneously. We discuss the role that such materials might play in fabricating novel…

材料科学 · 物理学 2007-05-23 A. B. Harris , G. Lawes

Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO3 above TNDy = 6.5 K. We observe the…

强关联电子 · 物理学 2007-05-23 O. Prokhnenko , R. Feyerherm , E. Dudzik , S. Landsgesell , N. Aliouane , L. C. Chapon , D. N. Argyriou

We propose a microscopic theory for magnetic switching of electric polarization (P) in the spin-spiral multiferroics by taking TbMnO3 and DyMnO3 as examples. We reproduce their phase diagrams under a magnetic field H_ex by Monte-Carlo…

强关联电子 · 物理学 2010-10-29 Masahito Mochizuki , Nobuo Furukawa

The (H,T)-phase diagram of the multiferroic perovskite TbMnO$_3$ was studied by high-resolution thermal expansion $\alpha(T)$ and magnetostriction $\Delta L(H)/L$ measurements. Below $T_{N}\simeq 42$ K, TbMnO$_3$ shows antiferromagnetic…

强关联电子 · 物理学 2009-11-13 D. Meier , N. Aliouane , D. N. Argyriou , J. A. Mydosh , T. Lorenz

The magnetic-field-induced 90-degree flop of ferroelectric polarization P in a spin-spiral multiferroic material TbMnO3 is theoretically studied based on a microscopic spin model. We find that the direction of the P-flop or the choice of…

强关联电子 · 物理学 2016-01-20 Masahito Mochizuki

TbMnO3 is an orthorhombic insulator where incommensurate spin order for temperature T_N < 41K is accompanied by ferroelectric order for T < 28K. To understand this, we establish the magnetic structure above and below the ferroelectric…

The electronic and magnetic properties of TbMnO3 leading to its ferroelectric (FE) polarization were investigated on the basis of relativistic density functional theory (DFT) calculations. In agreement with experiment, we show that the…

材料科学 · 物理学 2008-07-18 H. J. Xiang , Su-Huai Wei , M. -H. Whangbo , Juarez L. F. Da Silva

We have used in-field neutron and X-ray single crystal diffraction to measure the incommensurability &#948; of the crystal and magnetic structure of multiferroic TbMnO3 . We show that the flop in the electric polarization at the critical…

强关联电子 · 物理学 2009-11-11 N. Aliouane , D. N. Argyriou , J. Strempfer , I. Zegkinoglou , S. Landsgesell , M. v. Zimmermann

Lattice modulation and magnetic structures in magnetoelectric compounds Tb1-xDyxMnO3 have been studied around the ferroelectric (FE) Curie temperature T_C by x-ray and neutron diffraction. Temperature-independent modulation vectors through…

强关联电子 · 物理学 2009-11-11 T. Arima , A. Tokunaga , T. Goto , H. Kimura , Y. Noda , Y. Tokura

Orthorhombic HoMnO3 is a multiferroic in which Mn antiferromagnetic order induces ferroelectricity. A second transition occurs within the multiferroic phase, in which a strong enhancement of the ferroelectric polarization occurs…

强关联电子 · 物理学 2021-01-04 Y. W. Windsor , M. Ramakrishnan , L. Rettig , A. Alberca , T. Lippert , C. W. Schneider , U. Staub

Synchrotron x-ray diffraction and resonant magnetic scattering experiments on single crystal DyMnO3 have been carried out between 4 and 40 K. Below TN(Dy) = 5K, the Dy magnetic moments order in a commensurate structure with propagation…

强关联电子 · 物理学 2007-05-23 R. Feyerherm , E. Dudzik , N. Aliouane , D. N. Argyriou

All-electrical control of a dynamic magnetoelectric effect is demonstrated in a classical multiferroic manganite DyMnO3, a material containing coupled antiferromagnetic and ferroelectric orders. Due to intrinsic magnetoelectric coupling…

强关联电子 · 物理学 2017-04-06 A. Shuvaev , V. Dziom , Anna Pimenov , M. Schiebl , A. A. Mukhin , A. Komarek , T. Finger , M. Braden , A. Pimenov

Multiferroic TbMnO3 is investigated using x-ray diffraction in high magnetic fields. Measurements on first and second harmonic structural reflections due to modulations induced by the Mn and Tb magnetic order are presented as function of…

This work investigates the magnetically driven ferroelectricity in orthorhombic manganites RMnO3 (R=Gd, Dy or Tb) from the point of view of the symmetry. The method adopted generalizes the one used to characterize the polar properties of…

材料科学 · 物理学 2009-11-13 J. L. Ribeiro

We present the microscopic theory of improper multiferroicity in BiMnO3, which can be summarized as follows: (1) the ferroelectric polarization is driven by the hidden antiferromagnetic order in the otherwise centrosymmetric C2/c structure;…

材料科学 · 物理学 2010-11-01 I. V. Solovyev , Z. V. Pchelkina

We report the magnetic field dependent dc magnetization and the pressure-dependent (pmax ~ 16 kbar) ac susceptibilities Xp(T) on both powder and bulk multiferroic BiMnO3 samples, synthesized in different batches under high pressure. A clear…

强关联电子 · 物理学 2010-03-11 C. C. Chou , S. Taran , J. L. Her , C. P. Sun , C. L. Huang , H. Sakurai , A. A. Belik , E. Takayama-Muromachi , H. D. Yang
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