原子物理
We report on the use of ditellurium ($\mathrm{^{130}Te_2}$) as a frequency reference for laser locking at 391 nm and 498 nm optical wavelengths, which are of interest in titanium (Ti) laser-cooling experiments. In the ultraviolet region…
We demonstrate a technique for spatially resolved temperature measurement utilizing Rydberg Doppler broadening thermometry. This method employs two focused laser beams arranged perpendicularly to excite laser-cooled atoms from the ground…
Chip-scale microwave atomic systems based on thermal atomic beams offer a promising approach to realize low-power and low-drift clocks for timing holdover applications. Miniature beam clocks are expected to suppress many of the shifts that…
By employing singles, doubles, and triples excitations within the relativistic coupled-cluster framework, we perform comprehensive calculations of a wide range of atomic properties for the Th$^{3+}$ ion. These properties are essential for…
In a wide range of quantum technology applications, ranging from atomic clocks to the creation of ultracold or quantum degenerate samples for atom interferometry, optimal laser sources are critical. In particular, two phase-locked laser…
We study the parity-violating electron-electron interaction mediated by the axion-like in the hexatomic molecule of a symmetric top type. The rich rovibrational behavior require electronic computations for multiple molecular configurations…
We demonstrate a delay-programmable two-color femtosecond source based on a chirped-seed noncollinear optical parametric amplifier. Introducing controlled dispersion into the seed enables spectral selection through pump-seed delay, allowing…
We study the isotopic dependence of collisional widths and shifts of the Hg clock transition $^1$S$_0$-$^3$P$_0$ perturbed by the Rb atoms in the temperature range from 1 nK to 1 K. For this purpose, we model the Born-Oppenheimer effective…
We propose a laser isotope separation mechanism in which selectivity arises from nuclear spin rather than isotope shifts, enabling the use of broadband ultrafast lasers. A Ramsey pulse sequence is applied to paramagnetic molecular…
We report on efficient rovibrational state-selective loading of single H$_2^+$ molecular ions into a cryogenic linear Paul trap using (2+1) resonance-enhanced multi-photon ionization (REMPI). The H$_2^+$ ions are created by resonant…
Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying…
We use coupled-channel calculations to explore the nature of near-threshold bound states in a simplified model of Rb+KRb. This is a prototype for systems with very strong coupling at short range and chaotic behavior for the short-range…
We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…
We use a $^{87}\text{Rb}$ atomic vapor, suitable for an optically-pumped magnetometer (OPM) in Earth-field conditions, to study the noise properties of three strategies for generating pulsed optical pumping. We compare a frequency-modulated…
Penning traps, renowned for their unparalleled precision in determining fundamental properties such as mass and magnetic moments, are cornerstone instruments in modern physics. Their applications span from nuclear structure studies to…
We present absolute frequency measurements of 2S_{1/2}-nS_{1/2} two-photon transitions with n = 8, 9, and 10 in a cryogenic beam of atomic hydrogen. Each transition has been measured with a fractional uncertainty of approximately…
Tricationic protactinium monofluoride ($^{229}$PaF$^{3+}$) has been proposed as a candidate for probing physics beyond the Standard Model of particle physics. Since studies with $^{229}$PaF$^{3+}$ require significant experimental advances,…
A key advantage of quantum metrology is the ability to surpass the standard quantum limit~(SQL) for measurement precision through the use of non-classical states. However, there is typically little to no improvement in precision with the…
The generation of vortex matter waves carrying quantized orbital angular momentum is challenging and relies heavily on the material nanofabrication methods due to their extremely small de-Broglie wavelengths. Here, we introduce an…
We report relativistic many-body calculations of the interelectronic-interaction correction to the Land\'{e} $g$-factor of the $2s_{1/2}$, $2p_{1/2}$, $2p_{3/2}$, and $3s_{1/2}$ states in lithium-like ions with nuclear charge $Z = 4-20$.…