原子物理
In this work, we measure the properties of ensembles of rubidium atoms trapped in solid neon that are relevant for use as quantum sensors of magnetic fields: the spin coherence of the trapped atoms and the ability to optically control and…
We report the value of the electric quadrupole moment of $^{209}$Bi extracted from the atomic data. For this, we performed electronic structure calculations for the ground $^4S^o_{3/2}$ and excited $^2P^o_{3/2}$ states of atomic Bi using…
Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We…
We report a generally applicable computational and experimental approach to determine vibronic branching ratios in linear polyatomic molecules to the $10^{-5}$ level, including for nominally symmetry forbidden transitions. These methods are…
We present a full quantal study on the dissociation of a weakly bound molecular ion in the presence of an external time-dependent electric field. We focus on the dissociation dynamics of a molecular ion in a Paul trap relevant for atom-ion…
We report on the observation and coherent excitation of atoms on the narrow inner-shell orbital transition, connecting the erbium ground state $[\mathrm{Xe}] 4f^{12} (^3\text{H}_6)6s^{2}$ to the excited state $[\mathrm{Xe}]…
We report the measurement of one-body loss rates for magnetically trapped metastable europium atoms and the study of their loss mechanism. The loss of atoms observed in a magneto-optical trap is not fully understood because of the…
Lasing in the bad cavity regime has promising applications in precision metrology due to the reduced sensitivity to cavity noise. Here we investigate the spectral properties and phase behavior of pulsed lasing on the $^1$S$_0 - ^3$P$_1$…
In this paper we investigate the feasibility of Zeeman slowing calcium monofluoride (CaF) molecules originating from a cryogenic buffer gas cell. We measure the $A^2\Pi_{1/2} (v=0, J=\frac{1}{2}) - X^2\Sigma_{1/2} (v=0, N=1)$ hyperfine…
We describe the creation and characterisation of a velocity tunable, spin-polarized beam of slow metastable argon atoms. We show that beam velocity can be determined with a precision below 1 \% using matter-wave interferometry. The profile…
We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…
Compact vacuum systems are key enabling components for cold atom technologies, facilitating extremely accurate sensing applications. There has been important progress towards a truly portable compact vacuum system, however size, weight and…
Inspired by the work of Pratt and coworkers on a sum rule for the polarization correlations in electron bremsstrahlung when the outgoing electron is not observed, we derive the corresponding sum rule for the elementary process of…
We observe EIT in a V-system in a thermal rubidium-87 vapour in the hyperfine Paschen-Back regime, realised with a 0.6 T axial magnetic field. In this regime energy levels are no longer degenerate and EIT features from different initial…
We study ultracold long-range collisions of heteronuclear alkali-metal dimers with a reservoir gas of alkali-metal Rydberg atoms in a two-photon laser excitation scheme. In a low density regime where molecules remain outside the Rydberg…
We reconsider the calculation of rovibrational transition frequencies in hydrogen molecular ions. Some previously neglected contributions, such as the deuteron polarizability, are included into consideration in comparison with our previous…
We study the fragmentation of very large dimers into two singly charged ions caused by absorption of a photon. In this process a photo electron emitted from one atom of the dimer has certain chances to hit the other atom knocking out one of…
Energy loss in collisions of charged projectiles with many-electron systems can be dealt with in time-dependent density functional theory by invoking Ehrenfest's theorem for the time evolution of expectation values of observables. We derive…
We report on measurements of the anisotropic dynamical polarizability of Dy near the 626-nm intercombination line, employing modulation spectroscopy in a one-dimensional optical lattice. To eliminate large systematic uncertainties resulting…
We study the spectral signatures and coherence properties of radiofrequency dressed hyperfine Zeeman sub-levels of 87Rb. Experimentally, we engineer combinations of static and RF magnetic fields to modify the response of the atomic spin…