原子物理
The present work reports the parity ($\mathcal{P}$)-odd and time-reversal ($\mathcal{T}$)-odd interaction constants for the ground electronic state, X$^2\Sigma^{+}_{1/2}$, of YbX, X: Cu, Ag and Au molecules. The reported results have been…
The coherent pulse propagation of a Bessel beam resonant to the 8.4 eV nuclear clock transition in $^{229}$Th-doped crystals is investigated theoretically. Due to the magnetic dipole character of the clock transition, Bessel beams which…
We have developed a vacuum-ultraviolet spectropolarimeter to measure the linear polarization of spectral lines around the Lyman-$\alpha$ wavelength. The main components for polarimetry are a rotatable MgF$_2$ waveplate and a SiO$_2$/MgF$_2$…
We report the coherent excitation of the highly forbidden $^2S_{1/2} \rightarrow {^2}F_{7/2}$ clock transition in the odd isotope $^{173}\mathrm{Yb}^+$ with nuclear spin $I = 5/2$, and reveal the hyperfine-state-dependent, nuclear spin…
We report on a cryogenic platform at 4 K incorporating high numerical aperture optics for the generation of large-scale tweezers arrays, and compatible with Rydberg-state manipulation. We achieve trapping lifetimes of around 5000 s,…
This work attempts to present a complete theory of the $\mu$H hyperfine splitting, including all contributions above 1 ppm. Quantum electrodynamic and recoil corrections are calculated directly, while the proton structure correction is…
Strong-field ionization is the cornerstone of attosecond physics, which has been extensively studied under coherent-state driving. Recently, the interface between attosecond physics and quantum optics has emerged as a new frontier. Yet,…
In this paper, we present an all-optical method to produce shell-shaped traps for ultracold atoms in microgravity. Our scheme exploits optical double dressing of the ground state to create a short range strongly repulsive central potential…
Optically pumped magnetometers (OPMs) have emerged as a powerful technique for high-resolution magnetic field imaging. However, achieving sub-millimeter spatial resolution at sub-picotesla sensitivities ($\mathrm{< 1\,pT/\sqrt{Hz}}$)…
New high-precision microwave spectroscopic measurements and analysis of rotational energy level transitions in the ground vibronic state of the open-shell BaF molecule are reported with the purpose of contributing to studies of physics…
The AlF molecule, currently subject to laser cooling and trapping efforts, has the advantage that it can be efficiently produced in a thermochemical reaction between sublimated aluminum trifluoride and aluminum metal. Here we present a…
Gold monocarbide (AuC) has been produced and characterized using laser spectroscopy, representing the first reported observation of AuC. We recorded the optical spectrum of gas-phase AuC between 400 nm and 700 nm, assigning excitations from…
We report time-resolved photoelectron spectroscopy of the $3s3p$ doubly excited states of helium dressed by an intense near-infrared (NIR) laser field. Using synchronized XUV free-electron-laser and 800-nm NIR laser pulses, we observe a…
The performance of atom interferometers is commonly limited by the finite spectral acceptance of atomic beam splitters and mirrors, which restricts efficient coupling to atoms with large Doppler shifts and reduces the usable atomic flux.…
For over a century, termolecular, or third order, chemical reactions have been explained by the Lindemann Hinshelwood mechanism, assuming sequential stabilization via bimolecular encounters. Here, we demonstrate that barrierless…
We present a spectroscopic investigation of $^{169}\mathrm{Tm}^+$ that provides two key foundations for its use as a platform for advanced quantum applications. First, we establish the complete spectroscopic road map for optical cycling…
Optically pumped magnetometers (OPMs) have demonstrated significant potential in weak magnetic field detection due to their high sensitivity. In this study, we developed an Mz-type optically pumped rubidium magnetometer using a…
The Bell-Bloom-type optically pumped atomic magnetometers are well suited for weak geomagnetic field detection. However, conventional single-beam pumping introduces an atomic spin polarization gradient, which limits the measurement accuracy…
We report a study of the diazabicyclo[2.2.2]octane (DABCO) molecule photoionized using VUV synchrotron radiation in combination with an ion--electron coincidence spectrometer. We determine accurately the adiabatic ionization energy to…
We demonstrate that strong-field ionization of atoms in circularly polarized laser fields generates a photoelectron spin texture with toroidal topology in momentum space. Using time-dependent Schr\"odinger equation simulations,…