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The collisions between linear polar molecules, trapped in a microwave field with circular polarization, are theoretically analyzed. The microwave trap suggested by DeMille \cite{DeMille} seems to be rather advantageous in comparison with…

Atomic Physics · Physics 2015-05-13 Alexander V. Avdeenkov

Measurements of interactions between cold molecules and ultracold atoms can allow for a detailed understanding of fundamental collision processes. These measurements can be done using various experimental geometries including where both…

Atomic Physics · Physics 2020-03-25 N. J. Fitch , L. P. Parazzoli , H. J. Lewandowski

We present a theoretical study of atom - molecule collisions in superimposed electric and magnetic fields and show that dynamics of electronic spin relaxation in molecules at temperatures below 0.5 K can be manipulated by varying the…

Chemical Physics · Physics 2009-11-11 T. V. Tscherbul , R. V. Krems

We study the thermodynamics of the Bose-condensed atomic hydrogen confined in the Ioffe-Pritchard potential. Such a trapping potential, that models the magnetic trap used in recent experiments with hydrogen, is anharmonic and strongly…

Statistical Mechanics · Physics 2016-08-31 B. Pozzi , L. Salasnich , A. Parola , L. Reatto

Elastic and spin-changing inelastic collision cross sections are presented for cold and ultracold magnetically trapped NH. The cross sections are obtained from coupled-channel scattering calculations as a function of energy and magnetic…

For conventional ion traps, the trapping potential is close to independent of the electronic state, providing confinement for ions dependent primarily on their charge-to-mass ratio $Q/m$. In contrast, storing ions within an optical dipole…

We consider the practical feasibility of using the direct, electric dipole-dipole interaction between co-trapped molecular ions for robust quantum logic without the need for static polarizing fields. The use of oscillating dipole moments,…

Atomic Physics · Physics 2018-10-31 Eric R. Hudson , Wesley C. Campbell

For the first time, ordered polar molecules confined in monolayer-deep rectangular pits produced on an alkali halide surface by electron irradiation have been resolved at room temperature by non-contact atomic force microscopy. Molecules…

In optical dipole traps, the excited rotational states of a molecule may experience a very different light shift than the ground state. For particles with two polarizability components (parallel and perpendicular), such as linear $^1\Sigma$…

Atomic Physics · Physics 2018-07-26 Till Rosenband , David D. Grimes , Kang-Kuen Ni

Collisions of polar $^{1}\Sigma$ state molecules at ultralow energies are considered, within a model that accounts for long-range dipole-dipole interactions, plus rotation of the molecules. We predict a substantial suppression of…

Atomic Physics · Physics 2016-09-08 Alexander V. Avdeenkov , Masatoshi Kajita , John L. Bohn

We demonstrate sub-Doppler laser cooling and magneto-optical trapping of the rare earth element Holmium. Atoms are loaded from an atomic beam source and captured in six-beam $\sigma_+ - \sigma_-$ molasses using a strong $J=15/2…

Atomic Physics · Physics 2016-07-26 J. Miao , J. Hostetter , G. Stratis , M. Saffman

We introduce, analyze, and compare two novel methods of Single Photon Cooling that generically cool and compress molecular gases. The first method compresses the molecular gas density by three orders of magnitude and increases collision…

Chemical Physics · Physics 2012-05-07 Yuval Shagam , Edvardas Narevicius

The single-molecule magnet $\mathrm{[Ni(hmp)(MeOH)Cl]_4}$ is studied using both density functional theory (DFT) and the DFT+U method, and the results are compared. By incorporating a Hubbard-U like term for both the nickel and oxygen atoms,…

Strongly Correlated Electrons · Physics 2008-04-30 Chao Cao , Stephen Hill , Hai-Ping Cheng

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…

Quantum Physics · Physics 2009-10-07 M. Zeppenfeld , M. Motsch , P. W. H. Pinkse , G. Rempe

Ultra-cold RbCs molecules in high-lying vibrational levels of the a$^3\Sigma^+$ ground electronic state are confined in an optical trap. Inelastic collision rates of these molecules with both Rb and Cs atoms are determined for individual…

We experimentally investigate $\sigma^+$-$\sigma^-$ polarization gradient cooling~(PGC) of a single $^{87}$Rb atom in a tightly focused dipole trap and show that the cooling limit strongly depends on the polarization of the trapping field.…

Atomic Physics · Physics 2017-09-08 Yue-Sum Chin , Matthias Steiner , Christian Kurtsiefer

Complex molecular structure demands customized solutions to laser cooling by extending its general set of principles and practices. Yttrium monoxide (YO) has unique intramolecular interactions. The Fermi-contact interaction dominates over…

Atomic Physics · Physics 2020-06-18 Shiqian Ding , Yewei Wu , Ian A. Finneran , Justin J. Burau , Jun Ye

We present the simultaneous cooling and trapping of an isotopic mixture in a magneto-optical trap and we describe the transfer of the mixture into a conservative, far-off resonant dipole trap. The mixture is prepared with a new technique…

Atomic Physics · Physics 2007-05-23 N. Poli , R. E. Drullinger , G. Ferrari , J. Leonard , F. Sorrentino , G. M. Tino

Ultracold atoms confined in a dipole trap are submitted to a potential whose depth is proportional to the real part of their dynamic dipole polarizability. The atoms also experience photon scattering whose rate is proportional to the…

Atomic Physics · Physics 2017-04-11 Maxence Lepers , Jean-François Wyart , Olivier Dulieu , --

We investigate the dynamical process of optically trapped X$^{1}$$\Sigma$$^{+}$ (v" = 0) state $^{85}$Rb$^{133}$Cs molecules distributing in J" = 1 and J" = 3 rotational states. The considered molecules, formed from short-range…

Atomic Physics · Physics 2018-03-14 Zhonghao Li , Ting Gong , Zhonghua Ji , Yanting Zhao , Liantuan Xiao , Suotang Jia