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We have developed a single-shot imaging technique that can capture ultrafast events occurring on femtosecond to picosecond time scales. The technique is based on an optical pump-probe method, in which multiple time-delayed femtosecond…

Instrumentation and Detectors · Physics 2018-11-14 Sarang Yeola , Donghoon Kuk , Ki-Yong Kim

Inverse Compton scattering (ICS) is a unique mechanism for producing fast pulses - picosecond and below - of bright X- to gamma-rays. These nominally narrow spectral bandwidth electromagnetic radiation pulses are efficiently produced in the…

This lab note introduces the "Stokes Camera," a simple and novel experimental arrangement for real-time measurement of spatial amplitude and polarisation and thus spatially resolved Stokes parameters. It uses a polarisation sensitive camera…

Optics · Physics 2023-08-31 Mitchell A. Cox , Carmelo Rosales Guzmán

The Photon wave function Formalism provides an alternative description of some quantum optical phenomena in a more intuitive way. We use this formalism to describe the process of correlated Stokes--anti-Stokes Raman scattering. In this…

Quantum Physics · Physics 2020-12-08 A. V. A. Guimarães , M. F. Santos , A. Jorio , C. H. Monken

Spontaneous Raman spectroscopy (SRS) is a conventional in-situ laser diagnostic method that has been widely used for measurements of temperature and major species. However, SRS in sooting flames suffers from strong interference including…

Optics · Physics 2023-02-15 Hu Meng , Yihua Ren , Heinz Pitsch

State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a…

Quantum Physics · Physics 2022-12-28 Alireza Aghababaei , Christoph Biesek , Frank Vewinger , Simon Stellmer

Spontaneous Raman scattering (SpRS) is a weak non-linear effect, particularly relevant to classical-quantum coexistence transmission and sensing applications. In classical transmission, the relevant Raman effect is stimulated Raman…

Femtosecond, broadband stimulated Raman spectroscopy is a popular approach to measuring molecular dynamics with excellent signal-to-noise and spectral resolution. We present a new method for broadband stimulated Raman spectroscopy that…

Optics · Physics 2025-08-19 Nathan G. Drouillard , TJ Hammond

The transport of CO2 across the air-water interface is central to physical oceanography and carbon sequestration. A comprehensive understanding of this process requires high-resolution diagnostics of diffusion, absorption, and reaction…

Fluid Dynamics · Physics 2025-09-23 Dongfang Zhao , Yumin Shi , Shengkai Wang

Through-wall synthetic aperture radar (SAR) imaging is of significant interest for security purposes, in particular when using multi-static SAR systems consisting of multiple distributed radar transmitters and receivers to improve…

Numerical Analysis · Mathematics 2024-10-30 Francis Watson , Daniel Andre , William Robert Breckon Lionheart

Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…

Instrumentation and Detectors · Physics 2020-05-06 Yanwen Sun , Mike Dunne , Paul Fuoss , Taito Osaka , Aymeric Robert , Mark Sutton , Makina Yabashi , Diling Zhu

We show that time-resolved coherent anti-Stokes Raman signals of isolated transitions deviate from the exponential decay whose time constant is nowadays used for measuring Raman linewidths. The deviation is caused by probe pulse-shape…

Optics · Physics 2014-07-25 Michele Marrocco

From the famous 1918 H1N1 influenza to the present COVID-19 pandemic, the need for improved virial detection techniques is all too apparent. The aim of the present paper is to show that identification of individual virus particles in…

Medical Physics · Physics 2020-11-23 V. Deckert , T. Deckert-Gaudig , D. Cialla , J. Popp , R. Zell , A. V. Sokolov , Z. Yi , M. O. Scully

We present a method to characterize the spatial coherence of soft X-ray radiation from a single diffraction pattern. The technique is based on scattering from non-redundant arrays (NRA) of slits and records the degree of spatial coherence…

Accurate characterization using static light scattering (SLS) and dynamic light scattering (DLS) methods mandates the measurement and analysis of singly-scattered light. In turbid samples, the suppression of multiple scattering is therefore…

Soft Condensed Matter · Physics 2012-09-18 Ian Block , Frank Scheffold

We experimentally studied the spatial coherence of random laser emission from dye solutions containing nanoparticles. The spatial coherence, measured in a double-slit experiment, varied significantly with the density of scatterers and the…

Optics · Physics 2017-03-30 Brandon Redding , Michael A. Choma , Hui Cao

We report on the observation of the natural isotopic spread of carbon from single-molecule Surface Enhanced Raman Spectroscopy (SM-SERS). By choosing a dye molecule with a very localized Raman active vibration in a cyano bond (C$\equiv$N…

Soft Condensed Matter · Physics 2008-11-04 P. G. Etchegoin , E. C. Le Ru , M. Meyer

Charge-density waves (CDWs) are ordered quantum states of conduction electrons accompanied by periodic lattice distortions. Raman scattering (RS) spectroscopy is therefore well suited for probing CDW-induced structural modulations. We…

A dual color, frequency and pulse duration agile laser system, capable of delivering laser pulses in arbitrary temporal profiles with ~1 ns to ~1 us pulse duration, chirping rates of ~27 MHz/ns with an achievable chirping range of several…

Optics · Physics 2022-11-09 Junhwi Bak , Robert Randolph , Alexandros Gerakis

Coherent multi-transducer ultrasound (CoMTUS) creates an extended effective aperture through the coherent combination of multiple arrays, which results in images with enhanced resolution, extended field-of-view, and higher sensitivity. The…