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We present the CFHTLS-Archive-Research Survey (CARS). It is a virtual multi-colour survey based on public archive images from the CFHT-Legacy-Survey. Our main scientific interests in CARS are optical searches for galaxy clusters from low to…
We study resonance contrast by a two-step pulse observation method to enhance the frequency stability of coherent population trapping (CPT) atomic clocks. The proposed method is a two-step Raman--Ramsey scheme with low intensity during…
We present the first calculation of coherent backscattering with inelastic scattering by saturated atoms. We consider the scattering of a quasi-monochromatic laser pulse by two distant atoms in free space. By restricting ourselves to…
Statistical properties of light produced in spontaneous Raman scattering on an ensemble of molecules indicate the quantum nature of this phenomenon. The scattered light is non-classical and has high non-classical intensity correlations…
We have developed a novel in situ methodology for the direct study of mass transport properties in oxides with spatial and unprecedented time resolution, based on Raman spectroscopy coupled to isothermal isotope exchanges. Changes in the…
We demonstrate how a narrowband pump and a broadband spectrum can be spatially multiplexed by selective coupling them in two distinct modes of a few-mode microstructure fiber. The first mode carries most of the input pump energy, and…
Coherent Raman scattering microscopy is a fast, label-free and chemically specific imaging technique that has a high potential for future in-vivo optical histology. However, its imaging depth into tissues is limited to the sub-millimeter…
We present multi-color imaging by stimulated Raman scattering (SRS) enabled by an ultrafast fiber-based light source with integrated amplitude modulation and frame-to-frame wavelength tuning. With a relative intensity noise level of -153.7…
Fluorescence spectroscopy is an image correlation technique to analyze and characterize the molecular dynamics from a sequence of fluorescence images. Many image correlation techniques have been developed for different applications [1]. But…
We demonstrate for the first time, Raman random lasing in a continuous-wave (CW) excited, completely biocompatible and biodegradable carrot medium. The Stokes Raman mode of carotene renders carrot as a gain medium whereas random scattering…
The interaction between molecules is commonly ignored in surface-enhanced Raman scattering (SERS). Under this assumption, the total SERS signal is described as the sum of the individual contributions of each molecule treated independently.…
Helium atom scattering (HAS) is a well established technique for examining the surface structure and dynamics of materials at atomic sized resolution. The HAS technique Helium spin-echo spectroscopy opens up the possibility of compressing…
Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding…
Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…
Imaging of the structure of single proteins or other biomolecules with atomic resolution would be enormously beneficial to structural biology. X-ray free-electron lasers generate highly intense and ultrashort x-ray pulses, providing a route…
Nuclear magnetic resonance spectroscopy (MRS) allows for the determination of atomic structures and concentrations of different chemicals in a biochemical sample of interest. MRS is used in vivo clinically to aid in the diagnosis of several…
Researchers routinely characterize optical samples by computing the scattering cross-section. However, the experimental determination of this magnitude requires the measurement and integration of the components of the scattered field in all…
The multiple scattering of coherent light is a problem of both fundamental and applied importance. In optics, phase conjugation allows spatial focussing and imaging through a multiply scattering medium; however, temporal control is…
Recent advances in the field of attosecond science hold the promise of tracking electronic processes at the shortest space and time scales. Imaging methods that combine attosecond temporal with nanometer spatial resolution are currently out…
Analytic solutions for steady-state expectation values of atomic quantities and second order correlations are obtained for a fully quantum treatment of two stationary dipole-coupled atoms driven in a standard geometric configuration by a…