Related papers: Cold Molecule Spectroscopy for Constraining the Ev…

We present the results of GBT observations of all four ground-state hydroxyl (OH) transitions toward 15 supernova remnants (SNRs) which show OH(1720 MHz) maser emission. This species of maser is well established as an excellent tracer of an…

Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…

We report a direct measurement of the 0-1 R(0) vibrational transition frequency in ground-state hydrogen deuteride (HD) using infrared-ultraviolet double resonance spectroscopy in a molecular beam. Ground-state molecules are vibrationally…

We use optical frequency comb Fourier transform spectroscopy to record high-resolution, low-pressure, room-temperature spectra of formaldehyde (H$_2$$^{12}$C$^{16}$O) in the range of 1250 to 1390 cm$^{-1}$. Through line-by-line fitting, we…

We demonstrate a new technique for measuring the absolute frequencies of atomic transitions. The technique uses a ring-cavity resonator whose length is calibrated using a reference laser locked to the D_2 line in {87}Rb. The frequency of…

Polar heavy-atom molecules have been well recognized as promising candidates for precision measurements and tests of fundamental physics. A much slower molecular beam to increase the interaction time should lead to a more sensitive…

We use sub-Doppler optical-optical double-resonance (OODR) spectroscopy with a 3.3 ${\mu}$m single-frequency pump and a cavity-enhanced 1.65 ${\mu}$m comb probe to measure 33 ladder-type (3${\nu}$${_3}$ ${\leftarrow}$ ${\nu}$${_3}$) and 8…

Precision spectroscopy on cold molecules can potentially enable novel tests of fundamental laws of physics and alternative determination of some fundamental constants. Realizing this potential requires a thorough understanding of the…

We have measured the 1S - 2S transition frequency in atomic hydrogen via two photon spectroscopy on a 5.8 K atomic beam. We obtain $f_{1S-2S} = 2 466 061 413 187 035 (10)$ Hz for the hyperfine centroid. This is a fractional frequency…

Molecules with deep vibrational potential wells provide optical intervals sensitive to variation in the proton-electron mass ratio ($\mu$). On one hand, polar molecules are of interest since optical state preparation techniques have been…

Direct measurements of the ground-state magnetically insensitive hyperfine transition |F=2,mF=0>->|F=1,mF=0> of $^9Be^+$ ions have been performed using microwave-driven state transfer. The $^9Be^+$ ions are confined and laser-cooled in a…

We experimentally investigate an optical frequency standard based on the 467 nm (642 THz) electric-octupole reference transition 2S1/2(F=0) -> F7/2(F=3) in a single trapped 171Yb+ ion. The extraordinary features of this transition result…

Spectroscopic measurements of the helium atom are performed to high precision using an atomic beam apparatus and electro-optic laser techniques. These measurements, in addition to serving as a test of helium theory, also provide a new…

Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane…

Recently it was pointed out that transition frequencies in certain diatomic molecules have an enhanced sensitivity to variations in the fine-structure constant $\alpha$ and the proton-to-electron mass ratio $m_p/m_e$ due to a near…

We identify two metastable excited states in Sm$ ^{10+} $ highly charged ion as candidates for high accuracy optical clocks. Several atomic properties relevant to optical clock development are calculated using relativistic many-body…

This article reports the first optical frequency measurement of the $1\mathrm{S}-3\mathrm{S}$ transition in hydrogen. The excitation of this transition occurs at a wavelength of 205 nm which is obtained with two frequency doubling stages of…

Over a period of eight months, we have monitored transition frequencies between nearly degenerate, opposite-parity levels in two isotopes of atomic dysprosium (Dy). These transition frequencies are highly sensitive to temporal variation of…

Using a Ramsey-type setup, the lambda-doublet transition in the $J=1,\, \Omega=1$ level of the $a^3\Pi$ state of CO was measured to be 394 064 870(10) Hz. In our molecular beam apparatus, a beam of metastable CO is prepared in a single…

The hydroxyl radical (OH) is found in various environments within the interstellar medium (ISM) of the Milky Way and external galaxies, mostly either in diffuse interstellar clouds or in the warm, dense environments of newly formed low-mass…