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Sub-ppb measurement of a fundamental band rovibrational transition in HD

Atomic Physics 2020-07-14 v1 Chemical Physics

Abstract

We report a direct measurement of the 0-1 R(0) vibrational transition frequency in ground-state hydrogen deuteride (HD) using infrared-ultraviolet double resonance spectroscopy in a molecular beam. Ground-state molecules are vibrationally excited using a frequency comb referenced continuous-wave infrared laser, and the excited molecules are detected via state-selective ionization with a pulsed ultraviolet laser. We determine an absolute transition frequency of 111 448 815 477(13) kHz. The 0.12 parts-per-billion (ppb) uncertainty is limited primarily by the residual first-order Doppler shift.

Keywords

Cite

@article{arxiv.2002.09333,
  title  = {Sub-ppb measurement of a fundamental band rovibrational transition in HD},
  author = {Arthur Fast and Samuel A. Meek},
  journal= {arXiv preprint arXiv:2002.09333},
  year   = {2020}
}

Comments

5 pages, 4 figures