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We theoretically analyze the cooling dynamics of an atom which is tightly trapped inside a high-finesse optical resonator. Cooling is achieved by suitably tailored scattering processes, in which the atomic dipole transition either scatters…

Quantum Physics · Physics 2012-11-08 Marc Bienert , Giovanna Morigi

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two…

Quantum Physics · Physics 2013-12-24 Daniel M. Reich , Christiane P. Koch

Building a refrigerator based on the conversion of heat into optical energy is an ongoing engineering challenge. Under well-defined conditions, spontaneous anti-Stokes fluorescence of a dopant material in a host matrix is capable of…

Optics · Physics 2009-11-13 Peter Muys

We demonstrate the mixing of rotational states in the ground electronic state using microwave radiation to enhance optical cycling in the molecule yttrium (II) monoxide (YO). This mixing technique is used in conjunction with a frequency…

We provide a theoretical analysis for a recently demonstrated cooling method. Two-level particles undergo successive adiabatic transfers upon interaction with counter-propagating laser beams that are repeatedly swept over the transition…

We demonstrate the possibility of three-dimensional cooling of neutral atoms by illuminating them with two counterpropagating laser beams of mutually orthogonal linear polarization, where one of the lasers is a speckle field, i.e. a highly…

Atomic Physics · Physics 2009-10-31 Peter Horak , Jean-Yves Courtois , Gilbert Grynberg

We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…

Atomic Physics · Physics 2014-08-22 F. Robicheaux

Laser cooling typically requires one or more repump lasers to clear dark states and enable recycling transitions. Here, we have achieved cooling of Be+ ions using a single laser beam, facilitated by one-dimensional heating through…

Atomic Physics · Physics 2024-06-21 Yue Xiao , Yongxu Peng , Linfeng Chen , Chunhui Li , Zongao Song , Xin Wang , Tao Wang , Yurun Xie , Bin Zhao , Tiangang Yang

We discuss techniques to engineer effective long-range interactions between polar molecules using external static electric and microwave fields. We consider a setup where molecules are trapped in a two-dimensional pancake geometry by a…

Quantum Physics · Physics 2009-11-13 A. Micheli , G. Pupillo , H. P. Büchler , P. Zoller

The motion of charged particles can be interfaced with electric circuitry via the current induced in nearby pick-up electrodes. Here we show how the rotational and translational dynamics of levitated objects with arbitrary charge…

Quantum Physics · Physics 2021-10-11 Lukas Martinetz , Klaus Hornberger , Benjamin A. Stickler

We propose a laser cooling concept for the translational motion of molecules which does not require repeated spontaneous emission by each molecule. The cooling works by repetition of three main steps: velocity selection of a narrow momentum…

Quantum Physics · Physics 2007-05-23 C. H. Raymond Ooi , Kar Peter Marzlin , Juergen Audretsch

Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…

We theoretically study the thermal relaxation of many-body systems under the action of oscillating external fields. When the magnitude or the orientation of a field is modulated around values where the pairwise heat-exchange conductances…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Riccardo Messina , Annika Ott , Christoph Kathmann , Svend-Age Biehs , Philippe Ben-Abdallah

Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules.…

We present a mechanism for cooling atoms by a laser beam reflected from a single mirror. The cooling relies on the dipole force and thus in principle applies to arbitrary refractive particles including atoms, molecules, or dielectric…

Quantum Physics · Physics 2009-08-05 André Xuereb , Peter Horak , Tim Freegarde

We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…

Several laser techniques have been suggested and demonstrated recently for preparing polarizable molecules in rapidly spinning states with a disc-like angular distribution. We consider motion of these spinning discs in inhomogeneous fields,…

Chemical Physics · Physics 2015-05-20 Johannes Floss , Erez Gershnabel , Ilya Sh. Averbukh

We determine trapping conditions for ultracold polar molecules, where pairs of internal states experience identical trapping potentials. Such conditions could ensure that detrimental effects of inevitable inhomogeneities across an ultracold…

Atomic Physics · Physics 2015-06-12 Alexander Petrov , Constantinos Makrides , Svetlana Kotochigova

Precision searches for time-reversal symmetry violating interactions in polar molecules are extremely sensitive probes of high energy physics beyond the Standard Model. To extend the reach of these probes into the PeV regime, long coherence…

Atomic Physics · Physics 2017-10-03 Ivan Kozyryev , Nicholas R. Hutzler