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The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are…

Atomic Physics · Physics 2017-02-22 S. Schippers , A. L. D. Kilcoyne , R. A. Phaneuf , A. Müller

Two dimensional (2D) semiconductors present unique opportunities to intertwine optical and magnetic functionalities and to tune these performances through defects and dopants. Here, we integrate exciton pumping into a quantum sensing…

Three-body recombination of identical, spin-polarized fermionic atoms in the ultracold limit is investigated. The mechanisms for recombination are described in terms of the ``scattering volume'' $V_p$ in the framework of the adiabatic…

Atomic Physics · Physics 2009-11-07 H. Suno , B. D. Esry , Chris H. Greene

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

We describe a pseudo-3D photoionization code, NEBU_3D and its associated visualization tool, VIS_NEB3D, which are able to easily and rapidly treat a wide variety of nebular geometries, by combining models obtained with a 1D photoionization…

Astrophysics · Physics 2009-11-13 C. Morisset , G. Stasinska , M. Pena

A key insight of Einstein's theory of the photoelectric effect is that a minimum energy is required for photoexcited electrons to escape from a material. For the past century it has been assumed that photoexcited electrons of lower energies…

We formulate a three-dimensional semi-classical model to treat three-electron escape dynamics in a strongly-driven linear triatomic molecule, HeH$_{2}^{+}$. Our model includes the Coulomb singularities. Hence, to avoid unphysical…

Atomic Physics · Physics 2021-04-21 M. B. Peters , V. P. Majety , A. Emmanouilidou

Studies of ion-molecule reactions at low temperatures are difficult because stray electric fields in the reaction volume affect the kinetic energy of charged reaction partners. We describe a new experimental approach to study ion-molecule…

An additional channel opens for photoionization of atom $A$ by an electromagnetic field if it traverses a gas of atoms $B$ resonantly coupled to this field. We show that this channel, in which $A$ is ionized via resonant photoexcitation of…

Atomic Physics · Physics 2018-09-19 A. B. Voitkiv , C. Müller , S. F. Zhang , X. Ma

We propose differential holography as a method to overcome the long-standing forward-scattering problem in photoelectron holography and related techniques for the three-dimensional imaging of atoms. Atomic images reconstructed from…

In this work, we extend the x-ray constrained wavefunction fitting approach, a key method in quantum crystallography for charge density reconstruction, to incorporate experimental observables beyond x-ray diffraction. Unlike traditional…

Quantum Physics · Physics 2024-10-31 Stasis Chuchurka , Milaim Kas , Andrei Benediktovitch , Nina Rohringer

A first principles approach, based on the real space multiple scattering Green's function method, is presented for spin- and angle-resolved resonant photoemission from magnetic surfaces. It is applied to the Fe(010) valence band…

Strongly Correlated Electrons · Physics 2015-06-17 Fabiana Da Pieve , Peter Krueger

Ensembles of negatively charged boron vacancy (V$_{\text{B}}^-$) centers in hexagonal boron nitride (hBN) have emerged as a two-dimensional spin qubit system interfaced with optics to advance nanoscale quantum sensing. However, a…

Materials Science · Physics 2026-05-07 Zsolt Benedek , Ádám Ganyecz , Oscar Bulancea-Lindvall , Gergely Barcza , Viktor Ivády

The low-energy electron-impact dissociation of molecular hydrogen has been a source of disagreement between various calculations and measurements for decades. Excitation of the ground state of H$_2$ into the dissociative $b ^3\Sigma_u^+$…

Plasma Physics · Physics 2021-02-24 Liam H. Scarlett , Dmitry V. Fursa , Jack Knol , Mark C. Zammit , Igor Bray

Using the new version of the photoionization code Titan designed for plane-parallel photoionized thick hot media, which is unprecedented from the point of view of line transfer, we have undertaken a study of the influence of different…

Astrophysics · Physics 2009-11-10 Séverine Coupé , Olivier Godet , A. -M. Dumont , Suzy Collin

The narrowing of electron and ion wave packets in the process of photoionization is investigated, with the electron-ion recoil fully taken into account. Packet localization of this type is directly related to entanglement in the joint…

Quantum Physics · Physics 2009-11-10 M. V. Fedorov , M. A. Efremov , A. E. Kazakov , K. W. Chan , C. K. Law , J. H. Eberly

The combination of density-functional theory with other approaches to the many-electron problem through the separation of the electron-electron interaction into a short-range and a long-range contribution (range separation) is a successful…

Other Condensed Matter · Physics 2015-05-13 Paola Gori-Giorgi , Andreas Savin

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

Atomic and Molecular Clusters · Physics 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

Absorption of infrared and visible radiation from stellar emission spectra by the negatively charged hydrogen ions H$^{-}$ is considered. The explicit formula for the photodetachment cross-section of the negatively charged hydrogen ion(s)…

Solar and Stellar Astrophysics · Physics 2015-06-01 Alexei M. Frolov