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Related papers: Photofragmentation of the H_3 molecule, including …

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Cross-sections for dissociative recombination and electron-impact vibrational excitation of the BF$^+_2$ molecular ion are computed using a theoretical approach that combines the normal modes approximation for the vibrational states of the…

Plasma Physics · Physics 2024-05-03 V. Kokoouline , M. Ayouz , J. Zs. Mezei , K. Hassouni , I. F. Schneider

New high-resolution dissociative recombination rate coefficients of rotationally cool and hot H3+ in the vibrational ground state have been measured with a 22-pole trap setup and a Penning ion source, respectively, at the ion storage ring…

We propose a novel mechanism of electron localization and molecular symmetry breaking in dissociative photoionization of the H$_2$ molecule. The Coulomb field of the ejected electron can induce transition of the remaining H$_2^+$ ion from…

Atomic Physics · Physics 2014-03-12 Vladislav V. Serov , A. S. Kheifets

The theoretical approach developed here treats uniformly the direct and indirect mechanisms of dissociative recombination (DR) in a diatomic ion. The present theory is based on electron scattering calculations performed at several…

We have theoretically studied the effect of dissociative autoionization on the photoelectron energy spectrum in (1+2)-photon above threshold ionization(ATI) of H2 molecules. We have considered excitation from the ground state…

Atomic and Molecular Clusters · Physics 2009-10-31 Krishna Rai Dastidar , Ratan Kumar Das

We propose a novel method to describe realistically ionization processes with absorbing boundary conditions in basis expansion within the formalism of the so-called Non-Adiabatic Quantum Molecular Dynamics. This theory couples…

Quantum Physics · Physics 2015-06-26 Mathias Uhlmann , Thomas Kunert , Ruediger Schmidt

We present a new extension of the UKRmol electron-molecule scattering code suite, which allows one to compute ab initio photoionization and photorecombination amplitudes for complex molecules, resolved both on the molecular alignment…

Chemical Physics · Physics 2014-02-18 Alex G Harvey , Danilo S Brambila , Felipe Morales , Olga Smirnova

We present a robust, ab initio method for addressing atom-light interactions and apply it to photoionization of argon. We use a close-coupling ansatz constructed on a multi-configurational Hartree-Fock description of localized states and…

Atomic Physics · Physics 2015-06-12 T. Carette , J. M. Dahlström , L. Argenti , E. Lindroth

X-ray photoelectron spectra provide a wealth of information on the electronic structure. The extraction of molecular details requires adequate theoretical methods, which in case of transition metal complexes has to account for effects due…

It is demonstrated that recent experiments on ionization of 3p and 3s electrons in Ni film and solid body cannot be described in the frames of Hartree-Fock or the random phase approximation with exchange. The deviation is so big that from…

Atomic Physics · Physics 2015-06-15 Miron Ya. Amusia , Larissa V. Chernysheva , Victor G. Yarzhemsky

Inelastic low-energy (0--1 eV) collisions of electrons with HeH$^+$ cations are treated theoretically, with a focus on the rovibrational excitation and dissociative recombination (DR) channels. In an application of {\it ab initio}…

Chemical Physics · Physics 2017-10-30 Roman Čurík , Chris H. Greene

The article presents calculated dissociative recombination (DR) rate coefficients for H+3 . The previous theoretical work on H+3 was performed using the adiabatic hyperspherical approximation to calculate the target ion vibrational states…

Atomic Physics · Physics 2007-08-22 Samantha Fonseca dos Santos , Viatcheslav Kokoouline , Chris H. Greene

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

Atomic Physics · Physics 2015-02-25 Lun Yue , Lars Bojer Madsen

Partial photoionization cross sections from the ^1S ground and the ^3P metastable states of the Be isoelectronic series to different final states including a number of satellite (ionization plus excitation) channels are studied using the…

Atomic Physics · Physics 2012-05-25 W. -C. Chu , H. -L. Zhou , A. Hibbert , S. T. Manson

We develop and implement a Gaussian approach to calculate partial cross-sections and asymmetry parameters for molecular photoionization. Optimal sets of complex Gaussian-type orbitals (cGTOs) are first obtained by non-linear optimization,…

Chemical Physics · Physics 2021-11-17 Abdallah Ammar , Lorenzo Ugo Ancarani , Arnaud Leclerc

The collision-energy resolved rate coefficient for dissociative recombination of HD+ ions in the vibrational ground state is measured using the photocathode electron target at the heavy-ion storage ring TSR. Rydberg resonances associated…

Theoretical investigation of the dissociative recombination (DR) of NeH+ with low-energy electrons in the regime where the process occurs without direct potential energy curve crossings is presented. The calculations are performed using…

Atomic and Molecular Clusters · Physics 2025-09-09 Riyad Hassaine , Janos Zsolt Mezei , Dahbia Talbi , Jonathan Tennyson , Ioan F. Schneider

The absolute cross sections for the production of X2+ and X3+ ions following absorption of monochromatized SOLEIL synchrotron radiation by the HX+ hydride molecular ions (X = S,Cl) are presented as a function of photon energy in the region…

Dissociative recombination of N$_2$H$^+$ is explored in a two-step theoretical study. In a first step, a diatomic (1D) rough model with frozen NN bond and frozen angles is adopted, in the framework of the multichannel quantum defect theory…

Instrumentation and Methods for Astrophysics · Physics 2023-08-16 J. Zs Mezei , M. A. Ayouz , A. Orbán , A. Abdoulanziz , D. Talbi , D. O. Kashinski , E. Bron , V. Kokoouline , I. F. Schneider

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

Quantum Physics · Physics 2013-05-29 Szczepan Chelkowski , André D. Bandrauk