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The frequency ratio of the 1S0(F=1/2)-3P0(F=1/2) clock transition in 171Yb and the 1S0(F=9/2)-3P0(F=9/2) clock transition in 87Sr is measured by an optical-optical direct frequency link between two optical lattice clocks. We determined the…

The hyperfine structure of atoms and ions is widely used in fundamental and applied research. Accurate knowledge of hyperfine splitting values is essential for quantum metrology applications as well as for improving the performance of…

Atomic Physics · Physics 2024-07-01 Denis Mishin , Dmitry Tregubov , Nikolay Kolachevsky , Artem Golovizin

We report tests of local position invariance based on measurements of the ratio of the ground state hyperfine frequencies of 133Cs and 87Rb in laser-cooled atomic fountain clocks. Measurements extending over 14 years set a stringent limit…

We report precision measurement of the unperturbed ${^{3}}D_1$ microwave transition frequencies in $^{176}\mathrm{Lu}^+$ to a fractional uncertainty of $4\times10^{-14}$. We find the $|F,m_F\rangle=|8,0\rangle$ to $|7,0\rangle$ hyperfine…

Atomic Physics · Physics 2025-10-09 M. D. K. Lee , Qi Zhao , Qin Qichen , Zhao Zhang , N. Jayjong , K. J. Arnold , M. D. Barrett

Using 201Hg+ contained within a linear quadrupole rf ion trap that is part of an atomic clock, we report the first high-resolution spectroscopy on the hyperfine structure of 201Hg+. We measure the absolute ground state hyperfine interval to…

Atomic Physics · Physics 2015-05-13 E. A. Burt , S. Taghavi-Larigani , R. L. Tjoelker

We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the…

State-resolved laser spectroscopy at the 10$^{-12}$ precision level recently reported in $arXiv$:2406.18719 determined the fractional change in nuclear quadrupole moment between the ground and isomeric state of $^{229}\rm{Th}$, $\Delta…

We have measured the frequency of the $6s^2S_{1/2} - 5d^2D_{3/2}$ electric-quadrupole transition of $^{171}$Yb$^+$ with a relative uncertainty of $1\times 10^{-14}$, $\nu_{Yb}$ = 688 358 979 309 312 Hz $\pm$ 6 Hz. A femtosecond frequency…

Peik and Tamm [Europhys. Lett. 61, 181 (2003)] proposed a nuclear clock based on the isomeric transition between the ground state and the first excited state of thorium-229. This transition was recognized as a potentially sensitive probe of…

Atomic Physics · Physics 2021-01-19 Pavel Fadeev , Julian C. Berengut , Victor V. Flambaum

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…

We demonstrate that several metastable excited states in Hf$~$II, Hf$~$IV and W$~$VI ions may be good clock states since they are sufficiently long-living and are not sensitive to the perturbations. Cooling E1 transitions are available.…

Atomic Physics · Physics 2022-09-20 Saleh O. Allehabi , V. A. Dzuba , V. V. Flambaum

We report new experimental hyperfine structure (HFS) constants of neutral and singly ionized scandium (Sc I and Sc II). We observed spectra of Sc-Ar and Sc-Ne hollow cathode discharges in the region 200-2500 nm (50,000-4000 cm$^{-1}$) using…

Atomic Physics · Physics 2022-09-26 Hala , G. Nave

We present a compact atomic clock interrogating ultracold 87Rb magnetically trapped on an atom chip. Very long coherence times sustained by spin self-rephasing allow us to interrogate the atomic transition with 85% contrast at 5 s Ramsey…

Atomic Physics · Physics 2015-07-14 Ramon Szmuk , Vincent Dugrain , Wilfried Maineult , Jakob Reichel , Peter Rosenbusch

High precision spectroscopy of the $^1S_0$-to-${^1}D_2$ clock transition of $^{176}$Lu is reported. Measurements are performed with Hertz level precision with the accuracy of the hyperfine-averaged frequency limited by the calibration of an…

Atomic Physics · Physics 2019-03-06 R. Kaewuam , T. R. Tan , K. J. Arnold , M. D. Barrett

The absolute frequency of the In$^{+}$ $5s^{2 1}S_{0}$ - $5s5p^{3}P_{0}$ clock transition at 237 nm was measured with an accuracy of 1.8 parts in $10^{13}$. Using a phase-coherent frequency chain, we compared the $^{1}S_{0}$ - $^{3}P_{0}$…

Atomic quadrupole moments and hyperfine constants of the metastable $^2 D_{3/2, 5/2}$ states of Ca$^+$, Sr$^+$, Ba$^+$, Yb$^+$, and Hg$^+$ are calculated by the multiconfiguration Dirac-Hartree-Fock and relativistic…

Atomic Physics · Physics 2009-11-11 W. M. Itano

We report the measurement of hyperfine splitting in the $7d$ $^{2}D_{3/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy in a Cs vapor cell. We determine the hyperfine coupling constants $A = 7.3509(9)$ MHz…

Atomic Physics · Physics 2022-10-05 Bubai Rahaman , Sourav Dutta

We report the measurement of the hyperfine splitting in the $7D_{5/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy enabled by precise frequency scans using an acousto-optic modulator. All the six hyperfine…

Atomic Physics · Physics 2022-09-28 Bubai Rahaman , Sourav Dutta

We report a comprehensive evaluation of all known sources of systematic uncertainty for two independent $^{176}$Lu$^+$ single-ion optical references, finding total systematic uncertainty of $1.1\times10^{-19}$ and $1.4\times10^{-19}$ for…

Atomic Physics · Physics 2025-12-09 K. J. Arnold , M. D. K. Lee , Zhao Qi , Qichen Qin , Zhang Zhao , N. Jayjong , M. D. Barrett

With 87-Sr atoms confined in a one dimensional optical lattice, the frequency of the optical clock transition 5s^2 ^1S_0 - 5s5p ^3P_0 has been determined to be 429 228 004 229 872.9(5) Hz. The transition frequency was measured with the help…