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Related papers: Highly site-specific H2 adsorption on vicinal Si(0…

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We use kinetic Monte Carlo simulations to understand growth- and etching-induced step bunching of 6H-SiC{0001} vicinal surfaces oriented towards [1-100] and [11-20]. By taking account of the different rates of surface diffusion on three…

Materials Science · Physics 2009-09-30 Valery Borovikov , Andrew Zangwill

The hydrogen adsorption sites in MOF5 were determined using neutron powder diffraction along with first-principles calculations. The metal-oxide cluster is primarily responsible for the adsorption while the organic linker plays only a…

Materials Science · Physics 2009-11-11 T. Yildirim , M. R. Hartman

Molecular hydrogen normally has only weak, quadrupole transitions between its rovibrational states, but in a static electric field it acquires a dipole moment and a set of allowed transitions. Here we use published ab initio calculations of…

Astrophysics of Galaxies · Physics 2022-06-09 Mark A. Walker

The absorption sites and the low-lying rotational and vibrational (RV) energy states for H$_2$ adsorbed within a metal-organic framework are calculated via van der Waals density functional theory. The induced dipole due to bond stretching…

Other Condensed Matter · Physics 2015-05-20 Lingzhu Kong , Yves J. Chabal , David C. Langreth

We study the atomic oxygen adsorption on Pb(111) surface by using density-functional theory within the generalized gradient approximation and a supercell approach. The atomic and energetic properties of purely on-surface and subsurface…

Materials Science · Physics 2009-11-13 Bo Sun , Ping Zhang , Zhigang Wang , Suqing Duan , Xian-Geng Zhao , Xuchun Ma , Qi-Kun Xue

Halogenated aromatic molecules assemble on surfaces forming both hydrogen and halogen bonds. Even though these systems have been intensively studied on flat metal surfaces, high-index vicinal surfaces remain challenging, as they may induce…

Materials Science · Physics 2018-01-17 Rengin Peköz , Davide Donadio

The photosensitivity of silicon is inherently very low in the visible electromagnetic spectrum, and it drops rapidly beyond 800 nm in near-infrared wavelengths. Herein, we have experimentally demonstrated a technique utilizing…

Cosine-shaped bands that occur in DFT-based electronic band structures for MgB2 are further analyzed with calculations along reciprocal directions parallel to the high symmetry G-A direction at regular intervals along G-M. Band degeneracies…

Superconductivity · Physics 2026-03-24 Jose A. Alarco , Ian D. R. Mackinnon

CO adsorption on the Pt(111) surface is studied using first-principles methods. As found in a recent study [Feibelman, et al., J. Phys. Chem. B 105, 4018 (2001)], we find the preferred adsorption site within density functional theory to be…

Materials Science · Physics 2009-11-07 Ilya Grinberg , Yashar Yourdshahyan , Andrew M. Rappe

We study optical properties of two dimensional silicene using density functional theory based calculations. Our results on optical response property calculations show that they strongly depend on direction of polarization of light, hence…

Mesoscale and Nanoscale Physics · Physics 2012-05-24 Kamal Chinnathambi , Aparna Chakrabarti , Arup Banerjee , S. K. Deb

The main feature of vicinal surfaces of crystals characterized by the Miller indices (hhm) is rather small width (less than 10 nm) and substantially large length (more than 200 nm) of atomically-flat terraces on sample surface. This makes…

Materials Science · Physics 2024-09-30 A. Yu. Aladyshkin , A. N. Chaika , V. N. Semenov , A. M. Ionov , S. I. Bozhko

We have studied the adsorption of NO, and the coadsorption of N and O, on four physical and hypothetical systems: unstrained and strained Rh(100) surfaces and monolayers of Rh atoms on strained and unstrained MgO(100) surfaces. We find that…

Materials Science · Physics 2008-10-13 Raghani Pushpa , Prasenjit Ghosh , Shobhana Narasimhan , Stefano de Gironcoli

Two kinds of configurations involving steps on surfaces are reviewed. The first one results from an initially planar vicinal surface, i.e. slightly deviating from a high-symmetry (001) or (111) orientation. In some cases, these surfaces…

Statistical Mechanics · Physics 2007-05-23 Anna Chame , Sylvie Rousset , Hans P. Bonzel , Jacques Villain

We present a new ultra-violet spectrum of the QSO 0013-004 with 0.9 \AA resolution obtained with the MMT Blue spectrograph. The \upsilon = 0 - 0, 1 - 0, 2 - 0 and 3 - 0 Lyman bands of H_2 associated with the z = 1.9731 damped Ly alpah…

Astrophysics · Physics 2016-08-30 Jian Ge , Jill Bechtold

Si/Ge heteroepitaxial dots under tensile strain are grown on nanostructured Ge substrates produced by high-temperature flash heating exploiting the spontaneous faceting of the Ge(001) surface close to the onset of surface melting. A very…

Mesoscale and Nanoscale Physics · Physics 2019-04-18 L. Persichetti , M. Fanfoni , B. Bonanni , M. De Seta , L. Di Gaspare , C. Goletti , L. Ottaviano , A. Sgarlata

Recently, the hydrogen adsorption and diffusion on the CeO2 (111) surface have been a vividly discussed topic because of its outstanding catalytic activity and selectivity in hydrogenation reactions. However, for the strongly reduced CeO2…

Materials Science · Physics 2019-05-01 Xiaoke Li , Joachim Paier , Joachim Sauer

We present a computational study into the adsorption properties of CO$_2$ on amorphous and crystalline water surfaces under astrophysically relevant conditions. Water and carbon dioxide are two of the most dominant species in the icy…

Astrophysics of Galaxies · Physics 2017-09-13 L. J. Karssemeijer , G. A. de Wijs , H. M. Cuppen

Using coherent x-ray scattering, we evidenced atomic step roughness at the [111] vicinal surface of a silicon monocrystal of 0.05 degree miscut. Close to the (1/2 1/2 1/2) anti-Bragg position of the reciprocal space which is particularly…

Materials Science · Physics 2009-08-12 F. Livet , G. Beutier , M. de Boissieu , S. Ravy , F. Picca , D. Le Bolloc'h , V. Jacques

Water absorption and dissociation processes on pristine low-index TiO$_2$ interfaces are important but poorly understood outside the well-studied anatase (101) and rutile (110). To understand these, we construct three sets of machine…

Materials Science · Physics 2023-03-15 Zezhu Zeng , Felix Wodaczek , Keyang Liu , Frederick Stein , Jürg Hutter , Ji Chen , Bingqing Cheng

The existence of intrinsic vacancies in cubic (monoclinic) TiO suggests opportunity for hydrogen absorption, which was addressed in recent experiments. In the present work, based on first principle calculations, the preferences are studied…

Materials Science · Physics 2023-08-01 S. Vahid Hosseini , Andrei Postnikov , Mohammad Reza Mohammadizadeh