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A novel algorithm is presented that yields precise estimates of coexisting liquid and gas densities, $\rho^{\pm}(T)$, from grand canonical Monte Carlo simulations of model fluids near criticality. The algorithm utilizes data for the…

Statistical Mechanics · Physics 2009-11-10 Young C. Kim , Michael E. Fisher

The prediction of the equation of state and the phase behavior of simple fluids (noble gases, carbon dioxide, benzene, methane, short alkane chains) and their mixtures by Monte Carlo computer simulation and analytic approximations based on…

Statistical Mechanics · Physics 2009-11-13 B. M. Mognetti , P. Virnau , L. Yelash , W. Paul , K. Binder , M. Mueller , L. G. MacDowell

We report the discovery of a multicritical point that extends the liquid-gas paradigm to systems with competing symmetry-breaking orders. Using large-scale Monte Carlo simulations of a frustrated bilayer Ising antiferromagnet with tunable…

Strongly Correlated Electrons · Physics 2025-10-08 Yuchen Fan

We use discontinuous molecular dynamics and grand-canonical transition-matrix Monte Carlo simulations to explore how confinement between parallel hard walls modifies the relationships between packing fraction, self-diffusivity, partial…

Soft Condensed Matter · Physics 2009-11-13 Jeetain Mittal , Vincent K. Shen , Jeffrey R. Errington , Thomas M. Truskett

Continuum models with critical end points are considered whose Hamiltonian ${\mathcal{H}}[\phi,\psi]$ depends on two densities $\phi$ and $\psi$. Field-theoretic methods are used to show the equivalence of the critical behavior on the…

Statistical Mechanics · Physics 2011-04-15 H. W. Diehl , M. Smock

In simulations of a water-like model (ST2) that exhibits a liquid-liquid phase transition, we test for the occurrence of a thermodynamic region in which the liquid can be modelled as a two-component mixture. We assign each molecule to one…

Statistical Mechanics · Physics 2011-03-24 Megan J. Cuthbertson , Peter H. Poole

The equilibrium density distribution and thermodynamic properties of a Lennard-Jones fluid confined to nano-sized spherical cavities at constant chemical potential was determined using Monte Carlo simulations. The results describe both a…

Mesoscale and Nanoscale Physics · Physics 2010-04-27 James F. Lutsko , Julien Laidet , Patrick Grosfils

We perform Monte-Carlo simulations to analyse the structure and microscopic dynamics of a viscous Lennard-Jones liquid coupled to a quenched reference configuration of the same liquid. The coupling between the two replicas is introduced via…

Statistical Mechanics · Physics 2015-10-20 Andrea Ninarello , Ludovic Berthier , Daniele Coslovich

We investigate finite-size effects on diffusion in confined fluids using molecular dynamics simulations and hydrodynamic calculations. Specifically, we consider a Lennard-Jones fluid in slit pores without slip at the interface and show that…

Computational Physics · Physics 2017-03-16 Pauline Simonnin , Benoit Noetinger , Carlos Nieto-Draghi , Virginie Marry , Benjamin Rotenberg

We analyze the interrelation between the coexistence curve of the Lennard-Jones fluid and the Ising model in two and three dimensions within the global isomorphism approach proposed earlier [V. L. Kulinskii, J. Phys. Chem. B \textbf{114}…

Statistical Mechanics · Physics 2013-04-26 Vladimir Kulinskii

Liquids displaying strong virial-potential energy correlations conform to an approximate density scaling of their structural and dynamical observables. This scaling property does not extend to the entire phase diagram, in general. The…

Soft Condensed Matter · Physics 2020-12-23 Thibaud Maimbourg , Jeppe C. Dyre , Lorenzo Costigliola

The application of an external field often renders empirical criteria for identifying liquid-gas phase transitions ambiguous. Here, we demonstrate that the finite-size scaling of the density profile provides a definitive criterion to…

Statistical Mechanics · Physics 2025-10-28 Chong Zha , Yanshuang Chen , Cheng-Ran Du , Peng Tan , Yuliang Jin

We demonstrate that the law of the rectilinear coexistence diameter in two-dimensional (2D) mixtures of non-spherical colloids and non-adsorbing polymers is violated. Upon approach of the critical point, the diameter shows logarithmic…

Statistical Mechanics · Physics 2007-05-23 R. L. C. Vink , H. H. Wensink

We present an experimental and theoretical study of the phase behavior of a binary mixture of colloids with opposite adsorption preferences in a critical solvent. As a result of the attractive and repulsive critical Casimir forces, the…

Soft Condensed Matter · Physics 2011-10-03 O. Zvyagolskaya , A. J. Archer , C. Bechinger

The Bielefeld Parma Collaboration has in recent years put forward a method to probe finite density QCD by the detection of Lee-Yang singularities. The location of the latter is obtained by multi-point Pad\`e approximants, which are in turn…

High Energy Physics - Lattice · Physics 2024-05-21 F. Di Renzo , D. A. Clarke , P. Dimopoulos , J. Goswami , C. Schmidt , S. Singh , K. Zambello

The symmetrical restricted Gibbs ensemble (RGE) is a version of the Gibbs ensemble in which particles are exchanged between two boxes of fixed equal volumes. It has recently come to prominence because -- when combined with specialized…

Statistical Mechanics · Physics 2015-05-14 Douglas J. Ashton , Nigel B. Wilding , Peter Sollich

The second-order phase transitions in the Ising model and liquid-gas systems share a universality class and critical exponents, despite the absence of $Z_2$ symmetry in the liquid-gas Hamiltonian. This discrepancy highlights a central…

Statistical Mechanics · Physics 2025-12-10 Xinyang Li , Yuliang Jin

We present a high accuracy Monte Carlo simulation study of the Isotropic - Nematic phase transition of a lattice dispersion model of biaxial liquid crystals. The NI coexistence curve terminating at the Landau critical point have been…

Soft Condensed Matter · Physics 2019-02-20 Nababrata Ghoshal , Soumyajit Pramanick , Sudeshna DasGupta , Soumen Kumar Roy

We find a thermodynamic description of gas-liquid criticality that is different from van der Waals and mean-field theories. At the critical temperature there is no critical point; a liquid phase coexists with a vapor phase with densities…

Statistical Mechanics · Physics 2012-07-13 Leslie V. Woodcock

We present a novel method to derive liquid-gas coexisting densities, $\rho^{\pm}(T)$, from grand canonical simulations (without knowledge of $\Tc$ or criticality class). The minima of $ Q_{L}\equiv< m^{2} >_{L}^{2}/< m^{4}>_{L}$ in an…

Statistical Mechanics · Physics 2009-11-10 Young C. Kim , Michael E. Fisher , Erik Luijten