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The properties of water can have a strong dependence on the confinement. Here, we consider a water monolayer nanoconfined between hydrophobic parallel walls under conditions that prevent its crystallization. We investigate, by simulations…

Soft Condensed Matter · Physics 2014-03-24 Valentino Bianco , Giancarlo Franzese

Results for the kinetics of vapor-liquid phase transition have been presented from the molecular dynamics simulations of a single component two-dimensional Lennard-Jones fluid. The phase diagram for the model, primary prerequisite for this…

Soft Condensed Matter · Physics 2017-03-08 Jiarul Midya , Subir K. Das

We describe two distinct approaches to obtaining cloud point densities and coexistence properties of polydisperse fluid mixtures by Monte Carlo simulation within the grand canonical ensemble. The first method determines the chemical…

Statistical Mechanics · Physics 2009-11-11 Matteo Buzzacchi , Peter Sollich , Nigel B. Wilding , Marcus Mueller

The study of liquid-liquid phase transition has attracted considerable attention. One interesting example of such phenomenon is phosphorus for which the existence a first-order phase transition between a low density insulating molecular…

Soft Condensed Matter · Physics 2021-08-25 Manyi Yang , Tarak Karmakar , Michele Parrinello

We have investigated the phase behaviour of a symmetrical binary fluid mixture for the situation where the chemical potentials $\mu_1$ and $\mu_2$ of the two species differ. Attention is focused on the set of interparticle interaction…

Statistical Mechanics · Physics 2015-06-25 Juergen Koefinger , Nigel B. Wilding , Gerhard Kahl

The binodal of a boson square-well fluid is determined as a function of the particle mass through the newly devised quantum Gibbs ensemble Monte Carlo algorithm [R. Fantoni and S. Moroni, {\sl to be published}]. In the infinite mass limit…

Statistical Mechanics · Physics 2014-08-26 Riccardo Fantoni

We examine two aspects of Stockmayer fluids which consists of point dipoles that additionally interact via an attractive Lennard-Jones potential. We perform Monte Carlo simulations to examine the effect of an applied field on the liquid-gas…

mtrl-th · Physics 2016-09-07 Mark J. Stevens , Gary S. Grest

Using state-of-the-art rare-event sampling simulations, we precisely characterize the nucleation of liquid droplets from a supersaturated Lennard-Jones gas and uncover a key physical feature: critical clusters nucleate with a density that…

Chemical Physics · Physics 2026-01-07 Yijian Wu , Thomas Philippe , Aymane Graini , Julien Lam

A semi-grand-canonical Monte Carlo algorithm is employed in conjunction with the bond fluctuation model to investigate the critical properties of an asymmetric binary (AB) polymer mixture. By applying the equal peak-weight criterion to the…

Condensed Matter · Physics 2009-10-22 M. Mueller , N. B. Wilding

The blinking-checkers model [F. Caupin and M. A. Anisimov, Phys. Rev. Lett, 127,185701 (2021)] is a minimal lattice model which has demonstrated that, in the meanfield approximation, it can reproduce the phenomenon of fluid polyamorphism.…

Statistical Mechanics · Physics 2024-06-18 Sergey V. Buldyrev , Thomas J. Longo , Frederic Caupin , Mikhail A. Anisimov

Liquid-gas equilibrium is considered using the global isomorphism with the Ising-like (lattice gas) model. Such an approach assumes the existence of the order parameter in terms of which the symmetry of binodal is restored not only in the…

Soft Condensed Matter · Physics 2025-06-26 L. A. Bulavin , V. L. Kulinskii , A. M. Katts , A. M. Maslechko

Integral equation theory calculations within the mean spherical approximation (MSA) and grand canonical Monte Carlo (MC) simulations are employed to study the phase behaviour of a symmetrical binary fluid mixture in the presence of a field…

Statistical Mechanics · Physics 2009-11-11 Juergen Koefinger , Gerhard Kahl , Nigel B. Wilding

A previously developed fundamental measure fucntional [J. Chem. Phys. vol.107, 6379 (1997)] is used to study the phase behavior of a system of parallel hard cubes. The single-component fluid exhibits a continuous transition to a solid with…

Soft Condensed Matter · Physics 2009-10-31 Y. Martinez-Raton , J. A. Cuesta

Results from the state-of-the-art molecular dynamics simulations are presented for both equilibrium and nonequilibrium dynamics following vapor-liquid transition in a single component Lennard-Jones system. We have fixed the overall density…

Statistical Mechanics · Physics 2018-03-09 Sutapa Roy , Subir K. Das

We report a Monte Carlo simulation study of the properties of highly asymmetric binary hard sphere mixtures. This system is treated within an effective fluid approximation in which the large particles interact through a depletion potential…

Statistical Mechanics · Physics 2009-11-11 Julio Largo , Nigel B. Wilding

Within the coexistence region between liquid and vapor the equilibrium pressure of a simulated fluid exhibits characteristic jumps and plateaus when plotted as a function of density at constant temperature. These features exclusively…

Statistical Mechanics · Physics 2015-09-09 S. Prestipino , C. Caccamo , D. Costa , G. Malescio , G. Munaò

The critical behavior of the Widom-Rowlinson mixture [J. Chem. Phys. 52, 1670 (1970)] is studied in d=3 dimensions by means of grand canonical Monte Carlo simulations. The finite size scaling approach of Kim, Fisher, and Luijten [Phys. Rev.…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink

The phase behavior of a cross-linked polymer blend made of two incompatible species, $A$ and $B$, of different chemical nature is analyzed. Besides a homogeneous phase, this system also exhibits two microphases and a phase of total…

Condensed Matter · Physics 2007-05-23 Edilson Vargas , Marcia C. Barbosa

We present a single-particle Lennard-Jones (L-J) model for CO2 and N2. Simplified L-J models for other small polyatomic molecules can be obtained following the methodology described herein. The phase-coexistence diagrams of single-component…

Computational Physics · Physics 2015-06-11 Jun Li , Victor M. Calo

Linearly-sloped or `ramp' potentials belong to a class of core-softened models which possess a liquid-liquid critical point (LLCP) in addition to the usual liquid-gas critical point. Furthermore they exhibit thermodynamic anomalies in the…

Statistical Mechanics · Physics 2009-11-11 Helen M. Gibson , Nigel B. Wilding