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We study the origin of spin-gap in recently discovered material CaV$_4$O$_9$. We analyze the spin-$1/2$ Heisenberg model on the $1/5$ depleted square lattice with nearest neighbor (nn) and next nearest neighbor (nnn) interactions, in terms…

Condensed Matter · Physics 2009-10-28 O. A. Starykh , M. E. Zhitomirsky , D. I. Khomskii , R. R. P. Singh , K. Ueda

We examined a two-dimensional Heisenberg model with two kinds of exchange energies, $J_e$ and $J_c$. This model describes localized spins at vanadium ions in a layer of CaV$_4$O$_9$, for which a spin gap is found by a recent experiment.…

Condensed Matter · Physics 2009-10-28 Kazuhiro Sano , Ken'ichi Takano

I report results of a density matrix renormalization group (DMRG) study of a model for the two dimensional spin-gapped system CaV$_4$O$_9$. This study represents the first time that DMRG has been used to study a two dimensional system on…

Condensed Matter · Physics 2009-10-28 Steven R. White

A theoretical model is presented to explain the spin gap observed for CaV$_4$O$_9$. The underlying lattice of the 1/5-depleted square lattice favors a formation of plaquette resonating valence bond state. Inclusion of the frustrating second…

Condensed Matter · Physics 2009-10-28 Kazuo Ueda , Hiroshi Kontani , Manfred Sigrist , Patrick A. Lee

Second neighbor dominated exchange coupling in CaV4O9 has been obtained from ab initio density functional (DF) calculations. A DF-based self-consistent atomic deformation model reveals that the nearest neighbor coupling is small due to…

Materials Science · Physics 2009-10-31 C. Stephen Hellberg , W. E. Pickett , L. L. Boyer , Harold T. Stokes , Michael J. Mehl

We investigate the connection between doping-induced in-gap states and underlying spin excitations in Mott insulators by employing cluster perturbation theory on one-dimensional (1D) and quasi-1D Kitaev-Hubbard models. By manipulating…

Strongly Correlated Electrons · Physics 2026-05-13 Si-Qi Hou , Shun-Li Yu , Zhao-Yang Dong , Jian-Xin Li

We study the stability of the 4-site plaquette order in a model recently introduced by Katoh and Imada to explain the spin gap in CaV4O9. We show that all relevant types of order can be described within the framework of Schwinger boson mean…

Condensed Matter · Physics 2008-02-03 Marc Albrecht , Frederic Mila

We study the spin gap of the S=1/2 Heisenberg model on the distorted diamond chain, which is recently proposed to represent magnetic properties of Cu_3 Cl_6 (H_2 O)_2 2H_8 C_4 SO_2. This model is composed of stacked trimers and has three…

Strongly Correlated Electrons · Physics 2009-10-31 Kazuhiro Sano , Ken'ichi Takano

We have carried out a wide range of calculations for the $S=1/2$ Heisenberg model with nearest- and second-neighbor interactions on a two-dimensional lattice which describes the geometry of the vanadium ions in the spin-gap system…

Condensed Matter · Physics 2009-10-28 M. P. Gelfand , Z. Weihong , R. R. P. Singh , J. Oitmaa , C. J. Hamer

We consider the exchange Hamiltonian H_ST = -J Sum_{<rr'>} (2 S_r S_r' - 1/2) (2 T_r T_r' - 1/2) describing two isotropic spin-1/2 Heisenberg antiferromagnets coupled by a quartic term on equivalent bonds. The model is relevant for systems…

Strongly Correlated Electrons · Physics 2009-10-31 L. Guidoni , G. Santoro , S. Sorella , A. Parola , E. Tosatti

Magnetic susceptibility measured for CaV$_4$O$_9$ is analyzed by a method with high temperature expansion. The analysis is consistent with the $g$-value which is close to 2 and is observed by an ESR experiment. Four exchange parameters in a…

Condensed Matter · Physics 2007-05-23 Ken'ichi Takano , K. Sano

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

In order to discuss the spin-gap formation in a multiorbital system, we analyze an e_g-orbital Hubbard model on a geometrically frustrated zigzag chain by using a density-matrix renormalization group method. Due to the appearance of a…

Strongly Correlated Electrons · Physics 2015-06-25 Hiroaki Onishi , Takashi Hotta

We report $^{63}$Cu nuclear magnetic resonance and muon spin rotation measurements on the S=1/2 antiferromagnetic Heisenberg spin chain compound Sr$_{1.9}$Ca$_{0.1}$CuO$_3$. An exponentially decreasing spin-lattice relaxation rate 1/T$_1$…

Strongly Correlated Electrons · Physics 2014-05-21 F. Hammerath , E. M. Brüning , S. Sanna , Y. Utz , N. S. Beesetty , R. Saint-Martin , A. Revcolevschi , C. Hess , B. Büchner , H. -J. Grafe

Effects of possible orbital order in magnetic properties of two-dimensional spin gap system for CaV$_4$O$_9$ are investigated theoretically. After analyzing experimental data, we show that single orbital models assumed in the literature are…

Strongly Correlated Electrons · Physics 2009-10-30 Nobuyuki Katoh , Masatoshi Imada

We investigate the formation of spin gap in one-dimensional models characterized by the groups with hidden dynamical symmetries. A family of two-parametric models of isotropic and anisotropic Spin-Rotator Chains characterized by SU(2)x…

Strongly Correlated Electrons · Physics 2009-11-10 M. N. Kiselev , D. N. Aristov , K. Kikoin

Using resonant inelastic x-ray scattering, we observe in the bilayer iridate Sr3Ir2O7, a spin-orbit coupling driven magnetic insulator with a small charge gap, a magnon gap of ~92 meV for both acoustic and optical branches. This…

Strongly Correlated Electrons · Physics 2012-12-11 Jungho Kim , A. H. Said , D. Casa , M. H. Upton , T. Gog , M. Daghofer , G. Jackeli , J. van den Brink , G. Khaliullin , B. J. Kim

Using exact diagonalizations of finite clusters with up to 32 sites, we study the $J_1-J_2$ model on the 1/5 depleted square lattice. Spin-spin correlation functions are consistent with plaquette order in the spin gap phase which exists for…

Condensed Matter · Physics 2009-10-28 Marc Albrecht , Frederic Mila , Didier Poilblanc

The Heisenberg-Kitaev (HK) model on the triangular lattice is conceptually interesting for its interplay of geometric and exchange frustration. HK models are also thought to capture the essential physics of the spin-orbital entanglement in…

Strongly Correlated Electrons · Physics 2015-04-29 Michael Becker , Maria Hermanns , Bela Bauer , Markus Garst , Simon Trebst

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

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