We examined a two-dimensional Heisenberg model with two kinds of exchange energies, Je and Jc. This model describes localized spins at vanadium ions in a layer of CaV4O9, for which a spin gap is found by a recent experiment. Comparing the high temperature expansion of the magnetic susceptibility to experimental data, we determined the exchange energies as Je≃ 610 K and Jc≃ 150 K. By the numerical diagonalization we estimated the spin gap as Δ∼0.2Je≃ 120 K, which consists with the experimental value 107 K. Frustration by finite Jc enhances the spin gap.
@article{arxiv.cond-mat/9510160,
title = {Spin Gap of Two-Dimensional Antiferromagnet Representing CaV$_4$O$_9$},
author = {Kazuhiro Sano and Ken'ichi Takano},
journal= {arXiv preprint arXiv:cond-mat/9510160},
year = {2009}
}
Comments
12 pages of LaTex, 4 figures availavule upon request