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Resonant angle scanned x-ray photoelectron diffraction (RXPD) allows the determination of the atomic and magnetic structure of surfaces and interfaces. For the case of magnetized nickel the resonant L2 excitation with circularly polarized…

Other Condensed Matter · Physics 2015-05-27 M. Morscher , F. Nolting , T. Brugger , T. Greber

A systematic analysis of resonant x-ray Bragg diffraction data for UPd$_3$, with signal enhancement at the U M$_{IV}$ edge, including possible structural phase-transitions leads to a new determination of the space groups of the material in…

Strongly Correlated Electrons · Physics 2014-05-22 Javier Fernandez-Rodriguez , Stephen W. Lovesey , Jesus A. Blanco

Ordered magnetic charge created by Dirac multipoles that are magnetic and polar is examined. It has previously been revealed in the pseudo-gap phase of high-Tc materials by use of the Kerr effect and magnetic neutron Bragg diffraction.…

Strongly Correlated Electrons · Physics 2017-05-24 S. W. Lovesey , D. D. Khalyavin

The higher order multipoles above the electric quadrupole are commonly neglected in metamaterial homogenization. We show that they nevertheless can be significant when second order spatial dispersive effects, such as the magnetic response,…

Based on a localized crystal electric field model for the U^{4+} in the (5f)^2-configuration, we analyze the resonant x-ray scattering spectra around U M_{IV} and M_{V} edges in URu_{2}Si_{2}, taking full Coulomb and spin-orbit interactions…

Strongly Correlated Electrons · Physics 2009-11-10 Tatsuya Nagao , Jun-ichi Igarashi

A theory that fully describes previously observed neutron Bragg spots indicative of magnetic order in the pseudo-gap phase of YBa2Cu3O6 + x is presented. Magnetic diffraction intensities, unveiled by polarization analysis, are explained by…

Strongly Correlated Electrons · Physics 2015-05-01 S. W. Lovesey , D. D. Khalyavin , U. Staub

KV3Sb5 has recently attracted a considerable attention, due to its low temperature superconducting properties, which are heralded by a charge density wave. The apparent presence of a very weak magnetism does not result in long range…

Strongly Correlated Electrons · Physics 2022-08-31 V. Scagnoli , D. D. Khalyavin , S. W. Lovesey

Four crystal classes are optically active yet not chiral (non-enantiomorphic). Corresponding Bragg diffraction patterns calculated for circularly polarized (helical) x-rays tuned to an atomic resonance prove that angular anisotropy in the…

Strongly Correlated Electrons · Physics 2021-12-15 Stephen W. Lovesey

Here we report a resonant x-ray diffraction (RXD) study at the Cu L3 edge on the multi-chiral system CsCuCl3, exhibiting helical magnetic order in a chiral crystal structure. RXD is a powerful technique to disentangle electronic degrees of…

Magnetic axial and polar (Dirac) nickel multipoles contribute to resonant x-ray Bragg amplitudes in a symmetry informed analysis of monoclinic Li2Ni3P4O14 presented for future diffraction experiments. Magnetic long-range order below a…

Strongly Correlated Electrons · Physics 2025-08-08 Stephen W. Lovesey

Resonant soft x-ray Bragg diffraction at the Dy M$_{4,5}$ edges has been used to study Dy multipoles in the combined magnetic and orbitally ordered phase of DyB$_2$C$_2$. The analysis incorporates both the intra-atomic magnetic and…

Strongly Correlated Electrons · Physics 2015-03-19 A. J. Princep , A. M. Mulders , U. Staub , V. Scagnoli , T. Nakamura , A. Kikkawa , S. W. Lovesey , E. Balcar

Resonant x-ray diffraction performed at the $\rm L_{II}$ and $\rm L_{III}$ absorption edges of Ru has been used to investigate the magnetic and orbital ordering in Ca$_2$RuO$_4$ single crystals. A large resonant enhancement due to electric…

Gradient metasurfaces have been extensively applied in recent years for enabling an unprecedented control of light beam over thin optical components. However, these metasurfaces suffer from low efficiency when it comes to bending light with…

Optics · Physics 2020-10-22 Tie-Jun Huang , Li-Zheng Yin , Jin Zhao , Chao-Hai Du , Pu-Kun Liu

Possibility of a novel pseudo-scalar (octupole) order is studied theoretically for orbitally degenerate systems with strong spin-orbit coupling such as Ce$_x$La$_{1-x}$B$_6$. It is discussed that coexistence of an octupole order parameter…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshio Kuramoto , Hiroaki Kusunose

Complete polarization analysis applied to resonant x-ray scattering at the Cr K-edge in K2CrO4 shows that incident linearly polarized x-rays can be converted into circularly polarized x-rays by diffraction at the Cr pre-edge (E = 5994 eV).…

Strongly Correlated Electrons · Physics 2009-11-11 C. Mazzoli , S. B. Wilkins , S. Di Matteo , B. Detlefs , C. Detlefs , V. Scagnoli , L. Paolasini , P. Ghigna

We study the resonant x-ray scattering (RXS) spectra at the Dy $L_{\rm III}$ absorption edge in the quadrupole ordering phase of DyB$_2$C$_2$. Analyzing the buckling of sheets of B and C atoms, we construct an effective model that the…

Strongly Correlated Electrons · Physics 2009-11-10 Jun-ichi Igarashi , Tatsuya Nagao

It is proposed that the observation of orbital ordering in manganite materials should be possible at the L_II and L_III edges of manganese using X-ray resonant scattering. If performed, dipole selection rules would make the measurements…

Condensed Matter · Physics 2009-10-31 C. W. M. Castleton , M. Altarelli

In contrast to magnetic order formed by electrons' dipolar moments, ordering phenomena associated with higher-order multipoles (quadrupoles, octupoles, etc.) are more difficult to characterize because of the limited choice of experimental…

We propose that X-ray absorption and emission magnetic circular dichroism (XAS-MCD and XES-MCD) are promising measurements to directly detect ferroic higher-rank multipoles as candidate order parameters in altermagnets. Using the sum rules…

Strongly Correlated Electrons · Physics 2025-09-19 Masaichiro Mizumaki , Norimasa Sasabe , Takayuki Uozumi , Rikuto Oiwa , Hiroaki Kusunose

Here we show that the low temperature phase of magnetite is associated with an effective, although fractional, ordering of the charge. Evidence and a quantitative evaluation of the atomic charges are achieved by using resonant x-ray…

Strongly Correlated Electrons · Physics 2009-11-11 E. Nazarenko , J. E. Lorenzo , Y. Joly , J. L. Hodeau , D. Mannix , C. Marin