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The Random Phase Approximation (RPA) for total energies has previously been shown to provide a qualitatively correct description of static correlation in molecular systems, where density functional theory (DFT) with local functionals are…

Materials Science · Physics 2017-09-27 Thomas Olsen

Range-separated methods combining a short-range density functional with long-range random phase approximations RPAs with or without exchange response kernel are tested on rare-gas dimers and the S22 benchmark set of weakly interacting…

Chemical Physics · Physics 2014-04-10 Wuming Zhu , Julien Toulouse , Andreas Savin , János G. Angyán

The exact-exchange relativistic density functional theory (Ex-RDFT) of atomic nuclei has been solved in three-dimensional lattice space for the first time. The exchange energy is treated within the framework of the orbital-dependent…

Nuclear Theory · Physics 2024-12-16 Qiang Zhao , Zhengxue Ren , Pengwei Zhao , Kenichi Yoshida

We perform the self-consistent Skyrme Hartree-Fock calculation with the Coulomb exchange functional in the form of generalized gradient approximation (GGA). It is found that the Perdew-Burke-Ernzerhof GGA (PBE-GGA) Coulomb exchange…

Nuclear Theory · Physics 2019-02-15 Tomoya Naito , Xavier Roca-Maza , Gianluca Colò , Haozhao Liang

We derive a robust error estimate for a recently proposed numerical method for $\alpha$-dissipative solutions of the Hunter-Saxton equation, where $\alpha \in [0, 1]$. In particular, if the following two conditions hold: i) there exist a…

Numerical Analysis · Mathematics 2024-10-10 Thomas Christiansen

The exchange contribution to the energy of the hydrogen atom interacting with a proton is calculated from the polarization expansion of the wave function using the conventional surface-integral formula and two formulas involving volume…

Quantum Physics · Physics 2016-11-02 Piotr Gniewek , Bogumił Jeziorski

This paper presents a matrix formulation of the scalar laws of radiative transfer. The method applies to coupled mixed boundary condition problems on general domains. Participating media can range from transparent to absorbing, emitting,…

Computational Physics · Physics 2026-05-27 Nikolaj Maack Bielefeld

A Kubo-Greenwood-like equation for the Gilbert damping parameter $\alpha$ is presented that is based on the linear response formalism. Its implementation using the fully relativistic Korringa-Kohn-Rostoker (KKR) band structure method in…

Materials Science · Physics 2015-05-27 H. Ebert , S. Mankovsky , D. Koedderitzsch , P. J. Kelly

The density matrix expansion is used to derive a local energy density functional for finite range interactions with a realistic meson exchange structure. Exchange contributions are treated in a local momentum approximation. A generalized…

Nuclear Theory · Physics 2008-11-26 F. Hofmann , H. Lenske

Simulations of radiation damage in single molecule imaging using a X-ray free electron laser use atomic rates calculated in the lowest order. We investigate the difference in ion yield predictions using Hartree-Fock and Hartree-Fock-Slater…

Atomic Physics · Physics 2019-05-22 Alexander Kozlov , Harry M. Quiney

We present a comprehensive investigation of electron capture (EC) ratios spanning a broad range of atomic numbers. The study employs a self-consistent computational method that incorporates electron screening, electron correlations, overlap…

Nuclear Theory · Physics 2023-07-26 V. A. Sevestrean , O. Niţescu , S. Ghinescu , S. Stoica

The nucleon-pair approximation (NPA) can be a compact alternative to full configuration-interaction (FCI) diagonalization in nuclear shell-model spaces, but selecting good pairs is a long-standing problem. While seniority-based pairs work…

Nuclear Theory · Physics 2020-08-25 G. J. Fu , Calvin W. Johnson

We derive and employ a local potential to represent the Fock exchange operator in electronic single-particle equations. This local Fock-exchange (LFX) potential is very similar to the exact exchange (EXX) potential in density functional…

Materials Science · Physics 2016-12-21 T. W. Hollins , S. J. Clark , K. Refson , N. I. Gidopoulos

Using the shift-operator technique, a compact formula for the Fourier transform of a product of two Slater-type orbitals located on different atomic centers is derived. The result is valid for arbitrary quantum numbers and was found to be…

Materials Science · Physics 2009-11-13 T. A. Niehaus , R. López , J. F. Rico

We recently introduced an efficient methodology to perform density-corrected Hartree-Fock density functional theory (DC(HF)-DFT) calculations and an extension to it we called "corrected" HF DFT (C(HF)-DFT). In this work, we take a further…

Chemical Physics · Physics 2023-11-10 Daniel Graf , Alex J. W. Thom

Self interaction error remains an impotrant problem in density functional theory. A number of approximations to exact exchange aimed to correct for this error while retainining computational efficiency had been suggested recently. We…

Chemical Physics · Physics 2012-01-31 Valentin V. Karasiev , Eduardo V. Ludeña , Artëm E. Masunov

The Slater-type orbital basis with non-integer principal quantum numbers is a physically and mathematically motivated choice for molecular electronic structure calculations in both non-relativistic and relativistic theory. The…

Quantum Physics · Physics 2022-03-15 A Bagci , Philip E Hoggan , M Adak

We present a new type of the Hamiltonian replica-exchange method, in which not temperatures but the van der Waals radius parameter is exchanged. By decreasing the van der Waals radii that control spatial sizes of atoms, this Hamiltonian…

Statistical Mechanics · Physics 2015-05-14 Satoru G. Itoh , Hisashi Okumura , Yuko Okamoto

We discuss two different approximation schemes for the self-consistent solution of the {\it relativistic} Brueckner-Hartree-Fock equation for finite nuclei. In the first scheme, the Dirac effects are deduced from corresponding nuclear…

Nuclear Theory · Physics 2009-10-22 R. Fritz H. Müther , R. Machleidt

The random phase approximation (RPA) for the electron correlation energy, combined with the exact-exchange energy, represents the state-of-the-art exchange-correlation functional within density-functional theory (DFT). However, the standard…

Other Condensed Matter · Physics 2015-05-20 Xinguo Ren , Patrick Rinke , Alexandre Tkatchenko , Matthias Scheffler