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Panel-based, kernel-split quadrature is currently one of the most efficient methods available for accurate evaluation of singular and nearly singular layer potentials in two dimensions. However, it can fail completely for the layer…

Numerical Analysis · Mathematics 2022-01-20 Fredrik Fryklund , Ludvig af Klinteberg , Anna-Karin Tornberg

The accurate prediction of protein-ligand binding affinities is crucial for drug discovery. Alchemical free energy calculations have become a popular tool for this purpose. However, the accuracy and reliability of these methods can vary…

The charged environment within a dense plasma leads to the phenomenon of ionization potential depression (IPD) for ions embedded in the plasma. Accurate predictions of the IPD effect are of crucial importance for modeling atomic processes…

Plasma Physics · Physics 2014-07-10 Sang-Kil Son , Robert Thiele , Zoltan Jurek , Beata Ziaja , Robin Santra

We report density-functional studies of several small molecules ($H_{2}, N_{2}, CO, H_{2}O$, and $CH_{4}$) within the Krieger-Li-Iafrate (KLI) approximation to the exact Kohn-Sham local exchange potential, using a three-dimensional…

Chemical Physics · Physics 2009-10-31 Yong-Hoon Kim , Martin Städele , Richard M. Martin

Quantum--Mechanical methods that are both computationally fast and accurate are not yet available for electronic excitations having charge transfer character. In this work, we present a significant step forward towards this goal for those…

Chemical Physics · Physics 2015-06-12 Michele Pavanello , Troy Van Voorhis , Lucas Visscher , Johannes Neugebauer

Study of scattering process in the nonlocal interaction framework leads to an integro-differential equation. The purpose of the present work is to develop an efficient approach to solve this integro-differential equation with high degree of…

Nuclear Theory · Physics 2018-08-09 N. J. Upadhyay , A. Bhagwat

The self-consistent random phase approximation (RPA) based on a correlated realistic nucleon-nucleon interaction is used to evaluate correlation energies in closed-shell nuclei beyond the Hartree-Fock level. The relevance of contributions…

Nuclear Theory · Physics 2007-05-23 C. Barbieri , N. Paar , R. Roth , P. Papakonstantinou

We describe a method of solving the nuclear Skyrme-Hartree-Fock problem by using a deformed Cartesian harmonic oscillator basis. The complete list of expressions required to calculate local densities, total energy, and self-consistent…

Nuclear Theory · Physics 2009-10-30 J. Dobaczewski , J. Dudek

The $\alpha$-optical potential is one of the key input parameters used to measure the reaction rate of the ($\gamma,\alpha$)-process using the Hauser-Feshbach(HF) statistical model and the principle of detailed balance. $\alpha$-elastic…

Calculating highly accurate thermochemical properties of condensed matter via wave function-based approaches (such as e.g. Hartree-Fock or hybrid functionals) has recently attracted much interest. We here present two strategies providing…

We estimate the prediction sensitivity with respect to Hartree-Fock exchange in approximate density functionals for representative Fe(II) and Fe(III) octahedral complexes. Based on the observation that the range of parameters spanned by the…

Materials Science · Physics 2015-07-16 Efthymios I. Ioannidis , Heather J. Kulik

We examine the performance of our recently developed LFAs-PBE exchange-correlation (XC) potential [C.-R. Pan, P.-T. Fang, and J.-D. Chai, Phys. Rev. A, 2013, 87, 052510] for the high-order harmonic generation (HHG) spectra and related…

Chemical Physics · Physics 2016-06-14 Hsiao-Ling Sun , Wei-Tao Peng , Jeng-Da Chai

An exact method is suggested to treat the nonlinear self-interactions (NLSI) in the relativistic Hartree-Fock (RHF) approach for nuclear systems. We consider here the NLSI constructed from the relativistic scalar nucleon densities and…

Nuclear Theory · Physics 2008-11-26 S. Marcos , L. N. Savushkin , V. N. Fomenko , M. Lopez-Quelle , R. Niembro

We calculate the ground-state expectation value of scalar observables in the matrix formulation of the random phase approximation (RPA). Our expression, derived using the quasiboson approximation, is a straightforward generalization of the…

Nuclear Theory · Physics 2009-11-07 Calvin W. Johnson , Ionel Stetcu

We review self-consistent spectral methods for nuclear matter calculations. The in-medium T-matrix approach is conserving and thermodynamically consistent. It gives both the global and the single-particle properties the system. The T-matrix…

Nuclear Theory · Physics 2009-11-11 P. Bozek

A new scheme to study the properties of finite nuclei is proposed based on the Dirac-Brueckner-Hartree-Fock (DBHF) approach starting from a bare nucleon-nucleon interaction. The relativistic structure of the nucleon self-energies in nuclear…

Slater basis functions have desirable properties that can improve electronic structure simulations, but improved numerical integration methods are needed. This work builds upon the SlaterGPU library for evaluation of Hamiltonian matrix…

Chemical Physics · Physics 2025-10-20 Alexander Stark , Nathan Meier , Jeffrey Hatch , Joshua Kammeraad , Duy-Khoi Dang , Paul Zimmerman

We present a second-nearest-neighbor Modified Embedded Atom Method (2NN--MEAM) potential for Scandium (Sc) and Aluminum-Scandium (Al--Sc) alloys that unifies cohesive, thermodynamic, and solidification behavior within a single transferable…

Materials Science · Physics 2025-12-11 Avik Mahata

Accurate prediction of shallow-donor electron binding energies is critical for device modeling, dopant activation, and donor-based quantum technologies. Traditional beyond-DFT approaches (e.g., hybrid functionals, GW) are prohibitively…

Materials Science · Physics 2025-10-30 Joshua Claes , Bart Partoens , Dirk Lamoen , Marcelo Marques , Lara K. Teles

We present a general scheme for treating the integrable singular terms within exact exchange (EXX) Kohn-Sham or Hartree-Fock (HF) methods for periodic solids. We show that the singularity corrections for treating these divergencies depend…

Materials Science · Physics 2009-11-11 Pierre Carrier , Stefan Rohra , Andreas Goerling
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