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We present a density-functional study of a binary phase-separating mixture of soft core particles immersed in a random matrix of quenched soft core particles of larger size. This is a model for a binary polymer mixture immersed in a…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , M. Schmidt , R. Evans

We obtain a fundamental measure density functional for mixtures of parallel hard cylinders. To this purpose we first generalize to multicomponent mixtures the fundamental measure functional proposed by Tarazona and Rosenfeld for a…

Soft Condensed Matter · Physics 2009-11-13 Yuri Martinez-Raton , Jose A. Capitan , Jose A. Cuesta

We represent the free energy functional by a diagrammatic series with tensorial coefficients indexed by powers of length scale. For hard cores, we obtain Percus' exact functional in one dimension and the Kierlik-Rosinberg form of…

Soft Condensed Matter · Physics 2015-05-27 Gavin Leithall , Matthias Schmidt

The rational function approximation method, density functional theory, and NVT Monte Carlo simulation are used to obtain the density profiles of multicomponent hard-sphere mixtures near a planar hard wall. Binary mixtures with a size ratio…

Statistical Mechanics · Physics 2007-06-06 Alexandr Malijevsky , Santos B. Yuste , Andres Santos , Mariano Lopez de Haro

By using the Rosenfeld density functional we determine the number density profiles of both components of binary hard-sphere fluids close to a planar hard wall as well as the corresponding excess coverage and surface tension. The comparison…

Soft Condensed Matter · Physics 2009-10-31 R. Roth , S. Dietrich

We derive, from the dimensional cross-over criterion, a fundamental-measure density functional for parallel hard curved rectangles moving on a cylindrical surface. We derive it from the density functional of circular arcs of length $\sigma$…

Soft Condensed Matter · Physics 2015-06-16 Yuri Martinez-Raton , Enrique Velasco

In this article we obtain a fundamental measure functional for the model of aligned hard hexagons in the plane. Our aim is not just to provide a functional for a new, admittedly academic, model, but to investigate the structure of…

Soft Condensed Matter · Physics 2007-11-26 Jose A. Capitan , Jose A. Cuesta

In a recent paper [Phys. Rev. E \textbf{76}, 031202 (2007)], Schmidt has proposed a Fundamental Measure Density Functional Theory for one-dimensional nonadditive hard-rod fluid mixtures and has compared its predictions for the bulk…

Soft Condensed Matter · Physics 2007-12-19 Andres Santos

We examine the reversible adsorption of spherical solutes on a random site surface in which the adsorption sites are uniformly and randomly distributed on a substrate. Each site can be occupied by one solute provided that the nearest…

Soft Condensed Matter · Physics 2008-05-23 J. Talbot , G. Tarjus , P. Viot

We derive from first principles (without resorting to the replica trick) a density functional theory for fluids in quenched disordered matrices (QA-DFT). We show that the disorder-averaged free energy of the fluid is a functional of the…

Soft Condensed Matter · Physics 2007-07-18 Luis Lafuente , Jose A. Cuesta

Random sequential adsorption algorithm is a popular tool for modelling structure of monolayers built in irreversible adsorption experiments. However, this algorithm becomes very inefficient when the density of molecules in a layer rises.…

Computational Physics · Physics 2019-11-25 Michał Cieśla

We provide novel random surface density functional theory (RSDFT) formulation in the case of geometric heterogeneous surface of solid media which is essential for description of thermodynamic properties of confined fluids. The major…

Statistical Mechanics · Physics 2017-11-22 Timur Aslyamov , Aleksey Khlyupin

We propose a new type of effective densities via the potential distribution theorem. These densities are for the sake of enabling the mapping of the free energy of a uniform fluid onto that of a nonuniform fluid. The potential distribution…

Soft Condensed Matter · Physics 2012-02-21 L. L. Lee , G. Pellicane

We examine the reversible adsorption of hard spheres on a random site surface in which the adsorption sites are uniformly and randomly distributed on a plane. Each site can be occupied by one solute provided that the nearest occupied site…

Statistical Mechanics · Physics 2015-06-25 C. Oleyar , J. Talbot

We analyze the structure of the Fundamental Measure Theory for the free energy density functional of hard sphere mixtures. A comparative study of the different versions of the theory, and other density functional approaches, is done in…

Soft Condensed Matter · Physics 2009-11-07 Jose A. Cuesta , Yuri Martinez-Raton , Pedro Tarazona

The structural properties of single component fluids of hard hyperspheres in odd space dimensionalities $d$ are studied with an analytical approximation method that generalizes the Rational Function Approximation earlier introduced in the…

Statistical Mechanics · Physics 2011-11-10 Rene D. Rohrmann , Andres Santos

The equilibrium properties of a Janus fluid confined to a one-dimensional channel are exactly derived. The fluid is made of particles with two faces (active and passive), so that the pair interaction is that of hard spheres, except if the…

Statistical Mechanics · Physics 2020-07-01 M. A. G. Maestre , A. Santos

An approach to obtain the structural properties of additive binary hard-sphere mixtures is presented. Such an approach, which is a nontrivial generalization of the one recently used for monocomponent hard-sphere fluids [S. Pieprzyk, A. C.…

Soft Condensed Matter · Physics 2020-01-20 S. Pieprzyk , A. C. Brańka , S. B. Yuste , A. Santos , M. López de Haro

Fluids made of two-dimensional hard particles with polygonal shapes may stabilize symmetries which do not result directly from the particle shape. This is due to the formation of clusters in the fluid. Entropy alone can drive these effects,…

Soft Condensed Matter · Physics 2024-02-05 Yuri Martinez-Raton , Enrique Velasco

A geometry-based density functional theory is presented for mixtures of hard spheres, hard needles and hard platelets; both the needles and the platelets are taken to be of vanishing thickness. Geometrical weight functions that are…

Soft Condensed Matter · Physics 2009-11-11 Ansgar Esztermann , Hendrik Reich , Matthias Schmidt
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