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The existence of bound charge transfer (CT) excitons at the interface of monolayer lateral heterojunctions has been debated in literature, but contrary to the case of interlayer excitons in vertical heterostructure their observation still…

Excitons in two-dimensional semiconductors provide a novel platform for fundamental studies of many-body interactions. In particular, dipolar interactions between spatially indirect excitons may give rise to strongly correlated phases of…

Mesoscale and Nanoscale Physics · Physics 2022-09-14 Rafał Ołdziejewski , Alessio Chiocchetta , Johannes Knörzer , Richard Schmidt

Exciton and polaron pair dissociation is a key functional aspect of photovoltaic devices. To improve upon the current state of interfacial transport models, we augment the existing classical models of dielectric interfaces by incorporating…

Materials Science · Physics 2017-05-08 Michael J. Waters , Daniel Hashemi , John Kieffer

The separation of photogenerated polaron pairs in organic bulk heterojunction solar cells is the intermediate but crucial step between exciton dissociation and charge transport to the electrodes. In state-of-the-art devices, above 80% of…

Materials Science · Physics 2009-07-16 C. Deibel , T. Strobel , V. Dyakonov

Superfluid has been realized in Helium-4, Helium-3 and ultra-cold atoms. It has been widely used in making high-precision devices and also in cooling various systems. There have been extensive experimental search for possible exciton…

Materials Science · Physics 2009-07-10 Jinwu Ye , T. Shi , Longhua Jiang , C. P. Sun

This paper presents a possible explanation for the enhanced singlet exciton yield in light emitting polymers. We propose a theory of electron-hole recombination via inter-molecular inter-conversion from inter-molecular weakly bound polaron…

Chemical Physics · Physics 2009-11-10 William Barford

Excitons in organic crystalline semiconductors play a crucial role in the operation of optoelectronic devices such as organic solar cells, light-emitting diodes, and photodetectors. The excitonic properties of materials are dramatically…

Materials Science · Physics 2023-10-25 M. V. Klymenko , L. Z. Tan , S. P. Russo , J. H. Cole

We consider a simple model for the geminate electron-hole separation process in organic photovoltaic cells, in order to illustrate the influence of dimensionality of conducting channels on the efficiency of the process. The Miller-Abrahams…

Computational Physics · Physics 2014-03-27 Paraskevas Giazitzidis , Panos Argyrakis , Juan Bisquert , Vyacheslav S. Vikhrenko

We study the dynamic equilibrium between trions and excitons in monolayers of transition metal dichalcogenides in the presence of resident charge carriers and continuous photogeneration of excitons. We show that heating of the system via…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 A. M. Shentsev

Semiconductor heterojunctions have gained significant attention for efficient optoelectronic devices owing to their unique interfaces and synergistic effects. Interaction between charge carriers with the heterojunction plays a crucial role…

We present a study of the elastic exciton--electron ($X-e^-$) and exciton--hole ($X-h$) scattering processes in semiconductor quantum wells, including fermion exchange effects. The balance between the exciton and the free carrier…

Other Condensed Matter · Physics 2008-09-24 H. Ouerdane , R. Varache , M. E. Portnoi , I. Galbraith

Strong many-body interactions in two-dimensional (2D) semiconductors give rise to efficient exciton-exciton annihilation (EEA). This process is expected to result in the generation of unbound high energy carriers. Here, we report an…

The electron-hole pair created via photon absorption in organic photoconversion systems must overcome the Coulomb attraction to achieve long-range charge separation. We show that this process is facilitated through the formation of excited,…

Charge-transfer excitons possessing long radiative lifetime and net permanent dipole moment are highly appealing for quantum dot (QD) based energy harvesting and photodetecting devices, in which the efficiency of charge separation after…

Mesoscale and Nanoscale Physics · Physics 2022-07-13 Yamei Zhou , Christos S. Garoufalis , Zaiping Zeng , Sotirios Baskoutas , Yu Jia , Zuliang Du

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

Radiative recombination of excitons dressed by the interactions with free charge carriers often occurs under simultaneous excitation of either electrons or holes to unbound states. This phenomenon, known as the electron recoil effect,…

The interplay of migration, recombination, and dissociation of excitons in disordered media is studied theoretically in the low temperature regime. An exact expression for the photoluminescence spectrum is obtained. The theory is applied to…

Condensed Matter · Physics 2009-10-28 M. C. J. M. Vissenberg , M. J. M. de Jong

We calculate the photoluminescence spectrum and lifetime of a biexciton in a semiconductor using Fermi's golden rule. Our biexciton wavefunction is obtained using a Quantum Monte Carlo calculation. We consider a recombination process where…

Strongly Correlated Electrons · Physics 2013-01-15 M. Bauer , J. Keeling , M. M. Parish , P. Lopez Rios , P. B. Littlewood

Long-range and fast transport of coherent excitons is important for development of high-speed excitonic circuits and quantum computing applications. However, most of these coherent excitons have only been observed in some low-dimensional…

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang