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We study the crystalline and electronic properties of the $\textrm{Fe}_{1-x}\textrm{Co}_x\textrm{Se}$ system ($x=0$, 0.25, 0.5, 0.75, and 1.0) using X-ray diffraction, X-ray spectroscopy and density functional theory. We show that the…

Superconductivity · Physics 2014-07-22 I. Perez , J. A. McLeod , R. J. Green , R. Escamilla , V. Ortiz , A. Moewes

Erbium ions in crystals show considerable promise for the technologies that will form the backbone of future networked quantum information technology. Despite advances in leveraging erbium's fibre-compatible infrared transition for…

Photoabsorption spectra of N$_2$ and CO were recorded at 900K, using the vacuum-ultraviolet Fourier-transform spectrometer at the DESIRS beamline of synchrotron SOLEIL. These high-temperature and high-resolution measurements allow for…

We demonstrate thermally switchable chiroptical activity in a chiral spin crossover (SCO) material, where circular dichroism is significant in the low spin state but quenched in the high-spin state for both enantiomers. With magnetometry we…

Perovskite manganite thin films, $Pr_{0.55}(Ca_{1-y}Sr_y)_{0.45}MnO_3$, have been studied using x-ray photoemission spectroscopy in order to clarify the consequence of the competition between ferromagnetic metal (FM) and charge-orbital…

Strongly Correlated Electrons · Physics 2009-11-13 K. Takubo , J. -Y. Son , T. Mizokawa , N. Takubo , K. Miyano

Integrated optics are used to achieve astronomical interferometry inside robust and compact materials, improving the instrument's stability and sensitivity. In order to perform differential phase measurements at the H$\alpha$ line (656.3…

High resolution spin- and angle-resolved photoemission spectroscopy (spin-ARPES) was performed on the three-dimensional topological insulator Bi$_2$Se$_3$ using a recently developed high-efficiency spectrometer. The topological surface…

Light absorption of myoglobin triggers diatomic ligand photolysis and spin crossover transition of iron(II) that initiate protein conformational change. The photolysis and spin crossover reactions happen concurrently on a femtosecond…

Chemical Physics · Physics 2018-11-19 K. Falahati , H. Tamura , H. Burghardt , M. Huix-Rotllant

Mid-infrared (mid-IR) photo-detection has been recently growing in importance because of its multiple applications, including vibrational spectroscopy and thermal imaging. We propose and demonstrate a novel pyro-resistive photo-detection…

We investigate the electronic structure of BaIrO3, an interesting compound exhibiting charge density wave transition in its insulating phase and ferromagnetic transition at the same temperature, using full potential linearized augmented…

Strongly Correlated Electrons · Physics 2009-11-11 Kalobaran Maiti

Using time-, spin- and angle-resolved photoemission, we investigate the ultrafast spin dynamics of hot electrons on the surface of the topological insulator Bi$_2$Te$_3$ following optical excitation by fs-infrared pulses. We observe two…

Mesoscale and Nanoscale Physics · Physics 2017-05-22 J. Sánchez-Barriga , M. Battiato , M. Krivenkov , E. Golias , A. Varykhalov , A. Romualdi , L. V. Yashina , J. Minár , O. Kornilov , H. Ebert , K. Held , J. Braun

{\alpha}-RuCl3 is a Kitaev material suggested to be a proximate quantum spin liquid in a certain temperature and magnetic field range. Nonequilibrium measurements of transient dynamics have been proposed to detect fractionalized particles…

Strongly Correlated Electrons · Physics 2024-08-23 Haochen Zhang , Subin Kim , Young-June Kim , Hae-Young Kee , Luyi Yang

To help address the need for predicting radiative heat transfer (RHT) behavior of molten salts, we conducted a comprehensive review of methods and data from infrared optical spectroscopic measurements on molten fluoride salts.…

X-ray absorption spectroscopy (XAS) as well as x-ray magnetic circular dichroism (XMCD) and magnetization of hybrid pyrochlore Eu2-xFexTi2O7 were investigated, where the rare earth Eu (4f) was replaced with transition metal Fe (3d) to…

Band gap engineering in SrTiO${}_{3}$ and related titanate perovskites has long been explored due to the intriguing properties of the materials for photocatalysis and photovoltaic applications. A popular approach in the materials chemistry…

Materials Science · Physics 2016-01-12 Ryan B. Comes , Tiffany C. Kaspar , Steve M. Heald , Mark E. Bowden , Scott A. Chambers

Silicene (a monolayer of silicon atoms) is a quantum spin Hall insulator (QSHI), which undergoes a topological phase transition to a band insulator under external electric field $E_{z}$. We investigate a photo-induced topological phase…

Mesoscale and Nanoscale Physics · Physics 2013-01-15 Motohiko Ezawa

We report on the high resolution photoassociation spectroscopy of a $^{87}$Rb spin-1 Bose-Einstein condensate to the $1_\mathrm{g} (P_{3/2}) v = 152$ excited molecular states. We demonstrate the use of spin dependent photoassociation to…

Atomic Physics · Physics 2009-11-13 C. D. Hamley , E. M. Bookjans , G. Behin-Aein , P. Ahmadi , M. S. Chapman

Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…

We have studied spin excitation spectra in the Shastry-Sutherland model compound SrCu$_2$(BO$_3$)$_2$ in magnetic fields using far-infrared Fourier spectroscopy. The transitions from the ground singlet state to the triplet state at 24…

Other Condensed Matter · Physics 2009-11-10 T. Rõõm , D. Hüvonen , U. Nagel , J. Hwang , T. Timusk

Infrared vibration-rotation lines can be valuable probes of interstellar and circumstellar molecules, especially symmetric molecules, which have no pure rotational transitions. But most such observations have been interpreted with an…

Astrophysics of Galaxies · Physics 2015-06-15 John H. Lacy