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IR spectroscopy has been widely used for chemical identification and quantitative analysis of reactions occurring in a specific time and space domains by measuring an average signal of the entire system1. Achieving IR measurements with…

Using soft x-ray absorption spectroscopy and magnetic circular dichroism at the Co-$L_{2,3}$ edge we reveal that the spin state transition in LaCoO$_{3}$ can be well described by a low-spin ground state and a triply-degenerate high-spin…

In haemoglobin (consisting of four globular myoglobin-like subunits), the change from the low-spin (LS) hexacoordinated haem to the high spin (HS) pentacoordinated domed form upon ligand detachment and the reverse process upon ligand…

Topological insulators are characterized by Dirac cone surface states with electron spins aligned in the surface plane and perpendicular to their momenta. Recent theoretical and experimental work implied that this specific spin texture…

Infrared (IR) spectroscopy is an indispensable tool for many practical applications including material analysis and sensing. Existing IR spectroscopy techniques face challenges related to the inferior performance and the high cost of…

Optics · Physics 2017-03-13 Anna Paterova , Shaun Lung , Dmitry Kalashnikov , Leonid Krivitsky

We demonstrate a new scheme of infrared spectroscopy with visible light sources and detectors. The technique relies on the nonlinear interference of correlated photons, produced via spontaneous parametric down conversion in a nonlinear…

The discovery of enhanced superconductivity (SC) in FeSe films grown on SrTiO3 (FeSe/STO) has revitalized the field of Fe-based superconductors. In the ultrathin limit, the superconducting transition temperature Tc is increased by almost an…

Mid-infrared photothermal microscopy is a new chemical imaging technology in which a visible beam senses the photothermal effect induced by a pulsed infrared laser. This technology provides infrared spectroscopic information at sub-micron…

Optics · Physics 2021-04-08 Yi Zhang , Haonan Zong , Cheng Zong , Yuying Tan , Meng Zhang , Yuewei Zhan , Ji-Xin Cheng

Powerful mid-infrared illumination combined with mechanical detection via force microscopy provides access to nanoscale spectroscopic imaging in Materials and Life Sciences. Photo-induced force microscopy (PiFM) employs pulsed illumination…

Optics · Physics 2025-09-09 Shohely Tasnim Anindo , Daniela Täuber , Christin David

Ferropericlase (Fp), (Mg$_\mathrm{1-x}$Fe$_\mathrm{x}$)O, is the second most abundant phase in the Earths lower mantle. At relevant pressure-temperature conditions, iron in Fp undergoes a high spin (HS), S=2, to low spin (LS), S=0, state…

Geophysics · Physics 2020-10-28 Michel L. Marcondes , Fawei Zheng , Renata M. Wentzcovitch

Erbium-doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically-sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for…

By direct measurements of the complex optical conductivity $\sigma(\nu)$ of FeSi we have discovered a broad absorption peak centered at frequency $\nu_{0}(4.2 K) \approx 32 cm^{-1}$ that develops at temperatures below 20 K. This feature is…

Strongly Correlated Electrons · Physics 2015-03-19 V. V. Glushkov , B. P. Gorshunov , E. S. Zhukova , S. V. Demishev , A. A. Pronin , N. E. Sluchanko , S. Kaiser , M. Dressel

We calculate the angular dependence of the x-ray linear and circular dichroism at the $L_{2,3}$ edges of $\alpha$-Fe(II) Phthalocyanine (FePc) thin films using a ligand field model with full configuration interaction. We find the best…

Strongly Correlated Electrons · Physics 2015-06-24 Javier Fernandez-Rodriguez , Brian Toby , Michel van Veenendaal

We studied the novel multiferroic material Sr$_2$FeSi$_2$O$_7$, and found 3 absorption modes above the magnetic ordering transition temperature using time-domain terahertz spectroscopy. These absorption modes can be explained as the optical…

Strongly Correlated Electrons · Physics 2016-12-21 Thuc T. Mai , C. Svoboda , M. T. Warren , T. -H. Jang , J. Brangham , Y. H. Jeong , S-W. Cheong , R. Valdés Aguilar

An impedance spectroscopy (IS) is a versatile tool to study the effect of grains (bulk), grain boundaries and electrode-electrolyte interface on dielectric and electrical properties of electro-ceramics. This study only focuses the high…

Materials Science · Physics 2014-07-30 Hitesh Borkar , M Tomar , Vinay Gupta , Ashok Kumar

Infrared optical investigations of $\alpha$-(BEDT-TTF)$_2$I$_3$ have been performed in the spectral range from 80 to 8000~cm$^{-1}$ down to temperatures as low as 10~K by applying hydrostatic pressure. In the metallic state, $T > 135$~K, we…

Strongly Correlated Electrons · Physics 2016-05-10 R. Beyer , A. Dengl , T. Peterseim , S. Wackerow , T. Ivek , A. V. Pronin , D. Schweitzer , M. Dressel

Structural phase separation in A$_x$Fe$_{2-y}$Se$_2$ system has been studied by different experimental techniques, however, it should be important to know how the electronic uniformity is influenced, on which length scale the electronic…

Millimeter-sized single crystals of LaFeAsO were grown from NaAs flux and the in-plane optical properties were studied over a wide frequency range. A sizable electronic correlation effect was indicated from the analysis of the free-carrier…

Superconductivity · Physics 2015-05-14 Z. G. Chen , R. H. Yuan , T. Dong , N. L. Wang

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

Achieving spin squeezing within solid-state devices is a long standing research goal, due to the promise of their particularities, for instance their long coherence times, the possibility of low-temperature experiments or integration of…