English
Related papers

Related papers: Electronic-vibrational coupling in single-molecule…

200 papers

We theoretically study electronic transport through a layer of quantum dots connecting two metallic leads. By the inclusion of an inductor in series with the junction, we show that steady electronic transport in such a system may be…

Mesoscale and Nanoscale Physics · Physics 2015-03-14 Danko Radic , Anatoly M. Kadigrobov , Leonid Y. Gorelik , Robert I. Shekhter , Mats Jonson

Electron-electron (e-e) collisions can impact transport in a variety of surprising and sometimes counterintuitive ways. Despite strong interest, experiments on the subject proved challenging because of the simultaneous presence of different…

Electronic transport properties for single-molecule junctions have been widely measured by several techniques, including mechanically controllable break junctions, electromigration break junctions or by means of scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2020-07-22 Ferdinand Evers , Richard Korytár , Sumit Tewari , Jan M. van Ruitenbeek

We identify an intriguing feature of the electron-vibrational dynamics of molecular systems via a computational examination of \emph{trans}-polyacetylene oligomers. Here, via the vibronic interactions, the decay of an electron in the…

Quantum Physics · Physics 2013-04-09 Ignacio Franco , Angel Rubio , Paul Brumer

Quantum transport of electrons through a molecule is a series of individual electron tunnelling events separated by stochastic waiting time intervals. We study the emergence of temporal correlations between successive waiting times for the…

Mesoscale and Nanoscale Physics · Physics 2017-09-19 Daniel S. Kosov

Electronic conductance through a single molecule is sensitive towards its structural orientation between two electrodes, owing to the distribution of molecular orbitals and their coupling to the electrode levels, that are governed by…

Mesoscale and Nanoscale Physics · Physics 2023-08-11 Koushik R. Das , Sudipta Dutta

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

It is often intriguing experimentally to take stock of how conformational changes in the device configuration may impact the overall charge transport behavior of single-molecule junctions. Based on the allied approach of density functional…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 Talem Rebeda Roy , Arijit Sen

Inelastic effects in electron transport through nano-sized devices are addressed with a method based on nonequilibrium Green's functions (NEGF) and perturbation theory to infinite order in the electron-vibration coupling. We discuss the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Thomas Frederiksen , Mads Brandbyge , Nicolas Lorente , Antti-Pekka Jauho

Low-temperature transport spectroscopy measurements on a suspended few-hole carbon nanotube quantum dot are presented, showing a gate-dependent harmonic excitation spectrum which, strikingly, occurs in the Coulomb blockade regime. The…

Mesoscale and Nanoscale Physics · Physics 2009-06-02 A. K. Huettel , B. Witkamp , M. Leijnse , M. R. Wegewijs , H. S. J. van der Zant

We investigate the dynamics of entanglement in the excitation transfer through a chain of interacting molecules. In the case of two-molecule coupled to noisy environments we show that entanglement can be further enhanced if the distance…

Quantum Physics · Physics 2015-08-18 Wei Song , Yi-Sheng Huang , Ming Yang , Zhuo-Liang Cao

Molecular vibrations play a key role in magnetic relaxation processes of molecular spin qubits as they couple to spin states, leading to the loss of quantum information. Direct experimental determination of vibronic coupling is crucial to…

The current-induced vibrational dynamics is a key factor determining the stability of molecular nanojunctions. Beyond conventional Joule heating, a different mechanism caused by nonconservative current-induced forces has been predicted for…

Mesoscale and Nanoscale Physics · Physics 2026-02-20 Martin Mäck , Michael Thoss , Samuel L. Rudge

We investigate the electronic origin of the bending stiffness of conducting molecules. It is found that the bending stiffness associated with electronic motion, which we refer to as electro-stiffness, $\kappa_{e}$, is governed by the…

Soft Condensed Matter · Physics 2009-11-11 Young-Ho Eom , Hawoong Jeong , Juyeon Yi , Henri Orland

We study the motion of strongly inelastic particles in a narrow vibrating tube using molecular dynamics simulation. At low frequency of the vibration, we observe qualitative changes of the motion, as the depth of the pile increases. The…

Statistical Mechanics · Physics 2009-10-31 Jysoo Lee

General discrete one-dimensional stochastic models to describe the transport of single molecules along coupled parallel lattices with period $N$ are developed. Theoretical analysis that allows to calculate explicitly the steady-state…

Soft Condensed Matter · Physics 2009-11-11 Evgeny B. Stukalin , Anatoly B. Kolomeisky

We characterize both entanglement and quantum coherence in a molecular system by connecting the linear entropy of electronic-nuclear entanglement with Wigner-Yanase skew information measuring vibronic coherence and local quantum uncertainty…

Quantum Physics · Physics 2018-11-21 Mihaela Vatasescu

We investigate how vibration affects molecular photoemission dynamics, through simulations on two-dimension asymmetric model molecules including the electronic and nuclear motions in a fully correlated way. We show that a slight anisotropy…

Chemical Physics · Physics 2024-02-14 Antoine Desrier , Morgan Berkane , Camille Lévêque , Richard Taïeb , Jérémie Caillat

Single-molecule junctions are found to show anomalous spikes in dI/dV spectra. The position in energy of the spikes are related to local vibration mode energies. A model of vibrationally induced two-level systems reproduces the data very…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. H. A. Thijssen , D. Djukic , A. F. Otte , R. H. Bremmer , J. M. van Ruitenbeek

Viscous flow of interacting electrons in two dimensional materials features a bunch of exotic effects. A model resembling the Navier-Stokes equation for classical fluids accounts for them in the so called hydrodynamic regime. We performed a…

Mesoscale and Nanoscale Physics · Physics 2025-07-01 Jorge Estrada-Álvarez , Francisco Domínguez-Adame , Elena Díaz