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We used tip-enhanced Raman spectroscopy to study the diameter-dependent Raman modes in a contacted carbon nanotube rope. We show that with the near-field tip enhancement a large number of nanotubes within a rope can be identified, even if…

Mesoscale and Nanoscale Physics · Physics 2012-08-30 Karin Goß , Niculina Peica , Christian Thomsen , Janina Maultzsch , Claus M. Schneider , Carola Meyer

The capabilities of the mechanical resonator-based nanosensors in detecting ultra-small mass or force shifts have driven a continuing exploration of the palette of nanomaterials for such application purpose. Based on large-scale molecular…

Materials Science · Physics 2015-06-25 Haifei Zhan , Guiyong Zhang , Baocheng Zhang , John M. Bell , Yuantong Gu

The vibrational structure of chromium germanium telluride (Cr$_2$Ge$_2$Te$_6$, CGT) is investigated and a strong spin-phonon coupling is revealed. The measured high-resolution Raman scattering (RS) spectra are composed of the 10…

We study large-amplitude oscillations of carbon nanotubes with chiralities $(m,0)$ and $(m,m)$ and predict the existence of localized nonlinear modes in the form of {\em discrete breathers}. In nanotubes with the index $(m,0)$ {\em three…

Pattern Formation and Solitons · Physics 2007-06-01 Alexander V. Savin , Yuri S. Kivshar

We have used a femtosecond pump-probe impulsive Raman technique to explore the polarization dependence of coherent optical phonons in highly-purified and aligned semiconducting single-wall carbon nanotubes (SWCNTs). Coherent phonon spectra…

Mesoscale and Nanoscale Physics · Physics 2013-06-11 Yuki Honda , Elizabeth Maret , Atsushi Hirano , Takeshi Tanaka , Kotaro Makino , Muneaki Hase

We have performed the LiTaWO$_6$ vibrational studies for both Raman and infrared actives modes. Although we do not have crystalline samples, the study was conducted qualitatively, firstly comparing the sample with similar compounds in the…

Materials Science · Physics 2019-02-15 D. Valim , AG Souza Filho , J M Filho , OL Alves , MAC de Santis , E N Silva

Carbon nanotubes (CNTs) are nonlinear high-Q resonators with strong coupling to single-electron tunneling. We begin by describing several methods to detect the flexural motion of a CNT resonator. Next, we illustrate how single-electron…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 Harold B. Meerwaldt , Gary A. Steele , Herre S. J. van der Zant

We report a detailed study of the vibrational properties of BN single-walled nanotubes and of the BN monolayer. Our results have been obtained from a well-established Tight-Binding model complemented with an electrostatic model to account…

Materials Science · Physics 2009-11-07 Daniel Sanchez-Portal , Eduardo Hernandez

We study 23 to 30 nm long suspended single-wall carbon nanotube quantum dots and observe both their stretching and bending vibrational modes. We use low-temperature DC electron transport to excite and measure the tubes' bending mode by…

Mesoscale and Nanoscale Physics · Physics 2012-09-21 J. O. Island , V. Tayari , A. C. McRae , A. R. Champagne

Carbon-based tubular materials have sparked a great interest for future electronics and optoelectronics device applications. In this work, we computationally studied the mechanical properties of nanotubes generated from popgraphene…

Materials Science · Physics 2020-10-08 W. H. S. Brandão , A. L. Aguiar , L. A. Ribeiro , D. S. Galvão , J. M. De Sousa

The eigenmodes and the vibrational density of states of the ground state configuration of graphene clusters are calculated using atomistic simulations. The modified Brenner potential is used to describe the carbon-carbon interaction and…

Materials Science · Physics 2013-01-29 Sandeep Kumar Singh , F. M. Peeters

The Raman spectrum and particularly the Raman scattering intensities of monoclinic $\beta\text{-Ga}_2\text{O}_3$ are investigated by experiment and theory. The low symmetry of $\beta\text{-Ga}_2\text{O}_3$ results in a complex dependence of…

Materials Science · Physics 2017-02-07 Christian Kranert , Chris Sturm , Rüdiger Schmidt-Grund , Marius Grundmann

Second-order Raman scattering has been extensively studied in carbon-based nanomaterials, \emph{e.g.} nanotube and graphene, because it activates normally forbidden Raman modes that are sensitive to crystal disorder, such as defects,…

We examine the vibrational stability of three candidate structures for the B24N24 cage and report their infra-red (IR) and Raman spectra. The candidate structures considered are a round cage with octahedral O symmetry, a cage with S_4…

Atomic and Molecular Clusters · Physics 2016-09-08 Rajendra R. Zope , Tunna Baruah , Mark R. Pederson , Brett I. Dunlap

Vibrational-excitation cross sections of ground electronic state of carbon dioxide molecule by electron-impact through the CO2-(2\Pi) shape resonance is considered in the separation of the normal modes approximation. Resonance curves and…

Chemical Physics · Physics 2016-11-01 V. Laporta , J. Tennyson , R. Celiberto

We have observed large-amplitude coherent phonon oscillations of radial breathing modes (RBMs) in single-walled carbon nanotubes excited through the lowest-energy (E11) interband transitions. In contrast to the previously-studied coherent…

Mesoscale and Nanoscale Physics · Physics 2010-08-11 Y. -S. Lim , J. -G. Ahn , J. -H. Kim , K. -J. Yee , T. Joo , S. -H. Baik , E. H. Haroz , L. G. Booshehri , J. Kono

The vibrational properties of three sodosilicate glasses have been investigated in the framework of Density Functional Theory. The pure vibrational density of states has been calculated for all systems and the different vibrational modes…

Materials Science · Physics 2019-02-21 Dimitrios Kilymis , Simona Ispas , Bernard Hehlen , Sylvain Peuget , Jean-Marc Delaye

In order to investigate the origin of the phase transition observed in NaV$_2$O$_5$, as well as its electronic structure, we have measured Raman intensities as a function of the laser wavelength above and below the phase transition…

Strongly Correlated Electrons · Physics 2015-06-25 M. J. Konstantinovic , Z. V. Popovic , T. Ruf , M. Cardona , A. N. Vasil'ev , M. Isobe , Y. Ueda

Carbon nanorings are hoop-shaped, {\pi}-conjugated macrocycles which form the fundamental annular segments of single-walled carbon nanotubes (SWNTs). In a very recent report, the structures of chiral carbon nanorings (which may serve as…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Bryan M. Wong , Jonathan W. Lee

Phonon modes found in low frequency Raman scattering from $CdS_{1-x}Se_x$ nanocrystals embedded in borosilicate glass arising from confined acoustic phonons are investigated. In addition to the breathing modes and quadrupolar modes, two…

Materials Science · Physics 2008-03-10 Sanjeev K. Gupta , Satyaprakash Sahoo , Prafulla K. Jha , A. K. Arora , Y. M. Azhniuk