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We develop a general theory of electron--hole recombination in organic light emitting diodes that leads to formation of emissive singlet excitons and nonemissive triplet excitons. We briefly review other existing theories and show how our…

Materials Science · Physics 2009-11-07 K. Tandon , S. Ramasesha , S. Mazumdar

We extend our theory of electron--hole recombination in organic light emitting diodes to investigate the possibility that high energy singlet and triplet excited states with large electron--hole separations are generated in such processes,…

Strongly Correlated Electrons · Physics 2007-05-23 Mousumi Das , S. Mazumdar , S. Ramasesha

We have measured the ratio, r = $\sigma_S/\sigma_T$ of the formation cross section, $\sigma$ of singlet ($\sigma_S$) and triplet ($\sigma_T$) excitons from oppositely charged polarons in a large variety of $\pi$-conjugated oligomer and…

Soft Condensed Matter · Physics 2009-11-07 M. Wohlgenannt , X. M. Jiang , Z. V. Vardeny , R. A. J. Janssen

Electron-hole (e-h) capture in luminescent conjugated polymers (LCPs) is modeled by the dissipative dynamics of a multilevel electronic system coupled to a phonon bath. Electroinjected e-h pairs are simulated by a mixed quantum state, which…

Materials Science · Physics 2007-05-23 S. Karabunarliev , Eric R. Bittner

The scattering and recombination processes between two triplet excitons in conjugated polymers are investigated by using a nonadiabatic evolution method, based on an extended Su-Schrieffer-Heeger model including interchain interactions. Due…

Chemical Physics · Physics 2010-10-05 Y. Meng , B. Di , X. J. Liu , Y. D. Wang , Z. An

This paper presents a possible explanation for the enhanced singlet exciton yield in light emitting polymers. We propose a theory of electron-hole recombination via inter-molecular inter-conversion from inter-molecular weakly bound polaron…

Chemical Physics · Physics 2009-11-10 William Barford

We investigate the physical mechanisms for spin-dependent recombination of a strongly bound pair of triplet excitons generated by singlet fission and forming a spin quintet (total spin of two) bi-exciton. For triplet excitons the…

Mesoscale and Nanoscale Physics · Physics 2024-02-16 Yan Sun , L. R. Weiss , V. Derkach , J. E. Anthony , M. Monteverde , A. D. Chepelianskii

The effect of exchange interactions within spin pairs on spin-dependent transport and recombination rates through localized states in semiconductors during coherent electron spin resonant excitation is studied theoretically. It is shown…

Materials Science · Physics 2008-01-09 A. Gliesche , C. Michel , V. Rajevac , K. Lips , S. D. Baranovskii , F. Gebhard , C. Boehme

A spin-charge recombination route to superconductivity, proposed earlier (1992)], is examined using the Schwinger boson representation of the t-J model. The representation is known to work well at half-filling. It was shown in the earlier…

Condensed Matter · Physics 2007-05-23 Sanjoy K. Sarker

We report on small-cluster exact-diagonalization calculations which prove the formation of electron-hole pairs (excitons) as prerequisite for spontaneous interlayer phase coherence in bilayer systems described by the extended…

Strongly Correlated Electrons · Physics 2013-07-25 T. Kaneko , S. Ejima , H. Fehske , Y. Ohta

We estimate the triplet-singlet relaxation rate due to spin-orbit coupling assisted by phonon emission in weakly-confined quantum dots. Our results for two and four electrons show that the different triplet-singlet relaxation trends…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Juan I. Climente , Andrea Bertoni , Guido Goldoni , Massimo Rontani , Elisa Molinari

We consider the charged exciton complexes of an ideal two-dimensional electron-hole system in the limit of strong magnetic fields. A series of charged multiple-exciton states is identified and variational and finite-size exact…

Condensed Matter · Physics 2009-10-28 J. J. Palacios , D. Yoshioka , A. H. MacDonald

The region surrounding the excitonic insulator phase is a three-component plasma composed of electrons, holes, and excitons. Due to the extended nature of the excitons, their presence influences the surrounding electrons and holes. We…

Strongly Correlated Electrons · Physics 2015-06-22 B Zenker , D Ihle , F X Bronold , H Fehske

We introduce density imbalanced electron-hole bilayers at a commensurate 2 : 1 density ratio as a platform for realizing novel phases involving electrons, excitons and trions. Three length scales are identified which characterize the…

Strongly Correlated Electrons · Physics 2024-05-28 David D. Dai , Liang Fu

Muon spin relaxation ($\mu$SR) and nuclear magnetic resonance (NMR) experiments revealed that the spin singlet state with an excitation gap of $\sim$200 K is realized from $S = 1/2$ Nb$_4$ tetrahedral clusters in a cluster Mott insulator…

Materials Science · Physics 2009-06-30 T. Waki , Y. Kajinami , Y. Tabata , M. Yoshida , M. Takigawa , I. Watanabe , H. Nakamura

We have studied the nature and dynamics of spin-dependent charge carrier recombination in Tris(8-hydroxyquinolinato) aluminum (Alq$_3$) films in light emitting diodes at room temperature using continuous wave and pulsed electrically…

Mesoscale and Nanoscale Physics · Physics 2020-09-09 H. Popli , X. Liu , T. H. Tennahewa , M. Y. Teferi , E. Lafalce , H. Malissa , Z. V. Vardeny , C. Boehme

In photovoltaic diodes recombination of photogenerated electrons and holes is a major loss process. Biological light harvesting complexes (LHCs) prevent recombination via the use of cascade structures, which lead to spatial separation of…

We use temporally resolved intensity cross-correlation measurements to identify the biexciton-exciton radiative cascades in a negatively charged QD. The polarization sensitive correlation measurements show unambiguously that the excited two…

Mesoscale and Nanoscale Physics · Physics 2014-02-11 Y. Benny , R. Presman , Y. Kodriano , E. Poem , D. Gershoni , T. A. Truong , P. M. Petroff

We study the theory of itinerant-hole photoluminescence of two-dimensional electron systems in the regime of the magnetically induced Wigner crystal. We show that the exciton recombination transition develops structure related to the…

Condensed Matter · Physics 2009-10-28 N. R. Cooper

Carrier and spin recombination are investigated in p-type GaAs of acceptor concentration NA = 1.5 x 10^(17) cm^(-3) using time-resolved photoluminescence spectroscopy at 15 K. At low pho- tocarrier concentration, acceptors are mostly…

Materials Science · Physics 2017-04-05 F. Cadiz , D. Lagarde , P. Renucci , D. Paget , T. Amand , H. Carrère , A. C. H. Rowe , S. Arscott
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