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We derive an expression for the static dielectric constant of the colloidal susp ensions based on the electrokinetic equations. The analysis assumes that the ions have the same diffusivity, and that the double layer is much thinner than the…

Soft Condensed Matter · Physics 2009-11-07 C. -Y. D. Lu

Protein-stabilised emulsions can be seen as mixtures of unadsorbed proteins and of protein-stabilised droplets. To identify the contributions of these two components to the overall viscosity of sodium caseinate o/w emulsions, the…

Soft Condensed Matter · Physics 2019-01-30 Marion Roullet , Paul S. Clegg , William J. Frith

Phase transitions in polar binary mixtures can be drastically altered even by a small amount of salt. This is because the preferential solvation strongly depends on the ambient composition. Together with a summary of our research in this…

Soft Condensed Matter · Physics 2015-05-20 Akira Onuki , Takeaki Araki , Ryuichi Okamoto

We devise a new technique to prove two-dimensional crystallization results in the square lattice for finite particle systems. We apply this strategy to energy minimizers of configurational energies featuring two-body short-ranged particle…

Mesoscale and Nanoscale Physics · Physics 2023-08-22 Leonard Kreutz , Manuel Friedrich

In this paper, we formulate a field-theoretical model of dilute salt solutions of electrically neutral spherical colloid particles. Each colloid particle consists of a 'central' charge that is situated at the center and compensating…

Soft Condensed Matter · Physics 2020-01-08 Yu. A. Budkov

We report on a SANS investigation into the potential for these structural reorganization of complexes composed of lysozyme and small PSS chains of opposite charge if the physicochemical conditions of the solutions are changed after their…

Soft Condensed Matter · Physics 2010-07-26 Fabrice Cousin , Jérémie Gummel , Daniel Clemens , Isabelle Grillo , François Boué

The experimentally observed swelling and collapse response of weakly charged polymers to the addition of specific salts displays quite convoluted behavior that is not easy to categorize. Here we use a minimalistic implicit solvent /…

Chemical Physics · Physics 2018-08-13 Richard Chudoba , Jan Heyda , Joachim Dzubiella

Metal nanoparticles are receiving increased scientific attention owing to their unique physical and chemical properties that make them suitable for a wide range of applications in diverse fields, such as electrochemistry, biochemistry, and…

Chemical Physics · Physics 2020-10-09 Bendix Petersen , Rafael Roa , Joachim Dzubiella , Matej Kanduc

Colloidal model systems allow studying crystallization kinetics under fairly ideal conditions with rather well characterized pair interactions and minimized external influences. In complementary approaches therefore experiment, analytic…

Soft Condensed Matter · Physics 2015-06-19 Thomas Palberg

We generalize the concept of charge regulation of ionic solutions, and apply it to complex fluids with mobile macro-ions having internal non-electrostatic degrees of freedom. The suggested framework provides a convenient tool for…

Soft Condensed Matter · Physics 2018-01-17 Tomer Markovich , David Andelman , Rudi Podgornik

Protein crystal production is a major bottleneck for the structural characterisation of proteins. To advance beyond large-scale screening, rational strategies for protein crystallization are crucial. Understanding how chemical anisotropy…

Biomolecules · Quantitative Biology 2022-05-03 Amir R. Khan , Susan James , Michelle K. Quinn , Irem Altan , Patrick Charbonneau , Jennifer J. McManus

Despite being used for decades as stabilizers, amino acids (AAs) remain mysterious components of many medical and biological formulations. Hypotheses on their role vary ranging from hydrotropic to protein-specific effects (stabilization…

A statistical theory is presented of the magnesium ion interacting with lysozyme under conditions where the latter is positively charged. Temporarily assuming magnesium is not noncovalently bound to the protein, I solve the nonlinear…

Soft Condensed Matter · Physics 2021-08-10 Theo Odijk

Intracellular positive ions neutralise negative charges on the phosphates of a DNA strand conferring greater strength on the hydrogen bonds that connect complementary strands into a double helix and so confer enhanced stability. Beyond a…

Soft Condensed Matter · Physics 2016-04-25 Arghya Maity , Amar Singh , Navin Singh

A reduced model, which can fold both helix and sheet structures, is proposed to study the problem of protein folding. The goal of this model is to find an unbiased effective potential that has included the effects of water and at the same…

Soft Condensed Matter · Physics 2007-05-23 Nan-yow Chen

We investigate numerically and on the scaling level the adsorption of a charged colloid on an oppositely charged flexible membrane. We show that the long ranged character of the electrostatic interaction leads to a wrapping reentrance of…

Biological Physics · Physics 2009-11-10 Christian C. Fleck , Roland R. Netz

Nucleic acids are negatively charged macromolecules and their structure properties are strongly coupled to metal ions in solutions. In this paper, the salt effects on the flexibility of single stranded (ss) nucleic acid chain ranging from…

Biological Physics · Physics 2015-03-13 Feng-Hua Wang , Yuan-Yan Wu , Zhi-Jie Tan

Shortly after the determination of the first protein x-ray crystal structures, researchers analyzed their cores and reported packing fractions $\phi \approx 0.75$, a value that is similar to close packing equal-sized spheres. A limitation…

Biomolecules · Quantitative Biology 2016-04-06 Jennifer C. Gaines , W. Wendell Smith , Lynne Regan , Corey S. O'Hern

In order to inquire the microscopic origin of observed multiple time scales in solvation dynamics we carry out several computer experiments. We perform atomistic molecular dynamics simulations on three protein-water systems namely,…

Soft Condensed Matter · Physics 2017-10-18 Sayantan Mondal , Saumyak Mukherjee , Biman Bagchi

Using a new semi empirical method for calculating molecular polarizabilities and the Clausius Mossotti relation, we calculated the static dielectric constants of dry proteins for all structures in the protein data bank (PDB). The mean…

Biological Physics · Physics 2020-05-14 Muhamed Amin , Jochen Küpper