Related papers: Spin tunnelling in Molecular Magnets
We present topological interference effects for the tunneling of a single large spin, which are caused by the symmetry of a general class of magnetic anisotropies. The interference originates from spin Berry phases associated with different…
The equal-interval splitting of quantum tunneling observed in simple-Ising-model systems of Ni$_{4}$ (3D) and Mn$_3$ (2D) single-molecule magnets (SMMs) is reported. The splitting is due to the identical exchange coupling in the SMMs, and…
We present detailed calculations of low-energy spin dynamics in the ``ferric wheel'' systems Na:Fe_6 and Cs:Fe_8 in a magnetic field. We compute by exact diagonalisation the low-energy spectra and matrix elements for total-spin and…
We theoretically study the effects of bias-controlled interdot tunneling in vertically coupled quantum dots on the emission properties of spin excitons in various bias-controlled tunneling regimes. As a main result, for strongly coupled…
We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (<20 $\mu$s) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a…
We present an exact analytic study on the topological phase interference effect in resonant quantum tunneling of the magnetization between degenerate excited levels for biaxial ferromagnets in an arbitrarily directed magnetic field. We show…
The ground state tunnel splitting for the biaxial spin model in the magnetic field, H = -D S_{x}^2 + E S_{z}^2 - g \mu_B S_z H_z, has been investigated using an instanton approach. We find a new type of spin instanton and a new quantum…
Scattering of electrons by localized spins is the ultimate process enabling electrical detection and control of the magnetic state of a spin-doped material. At the molecular scale, this scattering is mediated by the electronic orbitals…
We investigate the effect of dynamic nuclear spin fluctuation on quantum tunneling of the magnetization (QTM) in the molecular magnet Fe8 by increasing the nuclei temperature using radio frequency (RF) pulses before the hysteresis loop…
The level splitting formulae much discussed in the study of spin tunneling in macroscopic ferromagnetic particles and previously derived only by complicated pseudoparticle methods for the ground state, are derived from those of eigenvalues…
Berry phase effects in spin systems lead to the suppression of tunneling effects when different tunneling paths interfere destructively. Such effects have been seen in several single-molecule magnets (SMMs) through measurements of…
The effect of spin-disorder scattering on perpendicular transport in a magnetic monolayer is considered within the single-site Coherent Potential Approximation (CPA). The exchange interaction between a conduction electron and localized…
It is shown that in a structure consisting of a superconducting ring-shaped electrode overlapped by a normal metal contact through a thin oxide barrier, measurements of the tunnel current in magnetic field can probe persistent currents in…
We investigate the topological quenching of spin tunneling in Mn_12-acetate molecules with an applied magnetic field along the hard axis. The model Hamiltonian describing this system has a fourth-order term due to the tetragonal anisotropy.…
Magnetic relaxation in molecular magnets under a sweeping field is studied by taking into account local stray fields. It is found that the randomness of local stray field leads to a distribution of the relaxation rate which subsequently…
We present a theoretical study of magnetic field driven spin transitions of electrons in coupled lateral quantum dot molecules. A detailed numerical study of spin phases of artificial molecules composed of two laterally coupled quantum dots…
Below 360 mK, Fe8 magnetic molecular clusters are in the pure quantum relaxation regime. We showed recently that the predicted ``square-root time'' relaxation is obeyed, allowing us to develop a new method for watching the evolution of the…
The theory for the quantum tunneling of nano-magnets is developed within the intermediate spin framework. Periodic magnetic effects are seen to reflect that associated with a change of flux by a single flux quantum $\Phi_{0}$. Essential are…
Spin-polarized tunneling in FMS/M/FMS double tunnel junctions where FMSs are ferromagnetic semiconductor layers and M is a metal spacer is studied theoretically within the single-site coherent potential approximation (CPA). The exchange…
Below 360 mK, Fe magnetic molecular clusters are in the pure quantum relaxation regime and we show that the predicted square-root time relaxation is obeyed, allowing us to develop a new method for watching the evolution of the distribution…