Related papers: Spin tunnelling in Molecular Magnets
This article presents a review on the theoretical and the experimental developments on macroscopic quantum tunneling and phase transition of the escape rate in spin systems. We present the basic ideas with simplified calculations so that it…
We study low temperature resonant spin tunneling in molecular magnets induced by a field sweep with account of dipole-dipole interactions. Numerical simulations uncovered formation of self-organized patterns of the magnetization and of the…
We report spin-pair tunneling observed in Mn$_3$ single-molecule magnet, which is a crystal with 2D network of identical exchange coupling. We observed a series of extra quantum tunnelings by the ac susceptibility measurements, and…
Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…
We report observation of coherent quantum oscilations in spin-10 Fe8 molecular clusters. The powder of magnetically oriented Fe8 crystallites was placed inside a resonator, in a dc magnetic field perpendicular to the magnetization axis. The…
We study the magnetic relaxation of a system of localized spins interacting through weak dipole interactions, at a temperature large with respect to the ordering temperature but low with respect to the crystal field level splitting. The…
A new mechanism is proposed for the magnetization reversal of molecular nanomagnets such as \Fe8. In this process the spin tunnels from the lowest state near one easy direction to the first excited state near the opposite easy direction,…
The manipulation of single magnetic molecules may enable new strategies for high-density information storage and quantum-state control. However, progress in these areas depends on developing techniques for addressing individual molecules…
The synthesis, crystal structure and magnetic characterization of a high spin cluster comprising eight iron ions, are presented in this contribution. The cluster has formula [(tacn)6Fe8O2(OH)12Br4.3(ClO4)3.7]6H2O, (Fe8PCL) where tacn is the…
We study the points of degeneracy (diabolical points) in magnetic molecules such as Mn_{12}-acetate that have an easy axis of four-fold symmetry. This is done for general magnetic field that need not be oriented along a high-symmetry…
We solve Schr\"odinger equation describing a tunneling macrospin coupled to a torsional oscillator. Energy spectrum is studied for various quantum regimes. Magnetic susceptibility and noise spectrum are computed. We show that entanglement…
We show that the dynamic magnetic susceptibility and the superparamagnetic blocking temperature of an Fe8 single molecule magnet oscillate as a function of the magnetic field Hx applied along its hard magnetic axis. These oscillations are…
We study tunneling of the magnetic moment in a particle that has full rotational freedom. Exact energy levels are obtained and the ground-state magnetic moment is computed for a symmetric rotor. The effect of the mechanical freedom on spin…
We study the macroscopic quantum tunneling of magnetization of the F=1 spinor condensate interacting through dipole-dipole interaction with an external magnetic field applied along the longitudinal or transverse direction. We show that the…
The quantum tunneling of the magnetization vector between excited levels are studied theoretically in single-domain ferromagnetic nanoparticles with biaxial crystal symmetry placed in an external magnetic field at an arbitarily directed…
High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…
Single molecule magnets straddle the classical and quantum mechanical worlds, displaying many fascinating phenomena. They may have important technological applications in information storage and quantum computation. We review the physical…
We analyze the interference between tunneling paths that occurs for a spin system with special Hamiltonian both for dipole and quadrupole excitation. Using an instanton approach, we find that as the strength of the second-order transverse…
A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…
In this study, we have studied the quantum tunneling of a single spin-orbit-coupled atom held in a periodically modulated optical lattice with an impurity. At the pseudocollapse points of quasienergy bands, where the dynamical localization…