Related papers: Mesoscopic Spin Tunneling in Molecular Crystals
We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…
Precise magnetic hysteresis measurements of small single crystals of Mn$_{12}$ acetate of spin 10 have been conducted down to 0.4 K using a high sensitivity Hall magnetometer. At higher temperature (>1.6K) step-like changes in magnetization…
The ground states of artificial molecules made of two vertically coupled quantum rings are studied within the spin density functional theory for systems containing up to 13 electrons. Quantum tunneling effects on the electronic structure of…
The laws of quantum mechanics are often tested against the behaviour of the lightest element in the periodic table, hydrogen. One of the most striking properties of molecular hydrogen is the coupling between molecular rotational properties…
The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…
In magnetic fields applied parallel to the anisotropy axis, the relaxation of the magnetization of Mn$_{12}$ measured for different sweep rates is shown to collapse onto a single scaled curve. The form of the scaling implies that the…
We investigate the topological quenching of spin tunneling in Mn_12-acetate molecules with an applied magnetic field along the hard axis. The model Hamiltonian describing this system has a fourth-order term due to the tetragonal anisotropy.…
We present a new theoretical approach to describe the quantum behavior of a macroscopic system interacting with an external irradiation field, close to the resonant condition. Here we consider the extremely underdamped regime for a system…
Molecular spin clusters are mesoscopic systems whose structural and physical features can be tailored at the synthetic level. Besides, their quantum behavior is directly accessible in laboratory and their magnetic properties can be…
A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…
The macroscopic quantum tunneling between two coupled Bose-Einstein condensates (BEC) (radio-frequency coupled two-component BECs or two BECs confined in a double-well potential) is mapped onto the tunneling of an uniaxial spin with an…
The stranglehold of low temperatures on fascinating quantum phenomena in one-dimensional quantum magnets has been challenged recently by the discovery of anomalous spin transport at high temperatures. Whereas both regimes have been…
In spin-crossover materials, the volume of a molecule changes depending on whether it is in the high-spin (HS) or low-spin (LS) state. This change causes distortion of the lattice. Elastic interactions among these distortions play an…
We investigate the role of topology and distortions in the quantum dynamics of magnetic molecules, using a cyclic spin system as reference. We consider three variants of antiferromagnetic molecular ring, i.e. Cr$_8$, Cr$_7$Zn and Cr$_7$Ni,…
Quantum tunneling often allows pathways to relaxation past energy barriers which are otherwise hard to overcome classically at low temperatures. However, this is not always the case. In this paper we provide simple exactly solvable examples…
The Mn cluster complexes Mn12(RCOO)16(H2O)4O12 with R=CH3 and 2ClPh (hereafter referred to as Mn12 acetate and Mn12 2-Cl benzoate, respectively) exhibit macroscopic magnetic quantum tunneling. Dynamical magnetic measurements indicate for…
We predict wide-band suppression of tunneling of spin-orbit-coupled atoms (or noninteracting Bose-Einstein condensate) in a double-well potential with periodically varying depths of the potential wells. The suppression of tunneling is…
We present muon spin lattice relaxation measurements in the V15 spin 1/2 molecular nano-magnet. We find that the relaxation rate in low magnetic fields (<5 kG) is temperature independent below ~10 K, implying that the molecular spin is…
We study the tunneling current through a mesoscopic two-terminal ring with spin-orbit coupling, which is threaded by a magnetic flux. The electron-electron interaction in the ring is described in terms of a Tomonaga-Luttinger model which…
Dielectric measurements at very low temperature indicate that in a glass with the eutectic composition BaO-Al$_2$O$_3$-SiO$_2$ a phase transition occurs at 5.84 mK. Below that temperature small magnetic fields of the order of 10 $\mu$T…