In magnetic fields applied parallel to the anisotropy axis, the relaxation of the magnetization of Mn12 measured for different sweep rates is shown to collapse onto a single scaled curve. The form of the scaling implies that the dominant symmetry-breaking process that gives rise to tunneling is a locally varying second-order anisotropy, forbidden by tetragonal symmetry in the perfect crystal, which gives rise to a broad distribution of tunnel splittings in a real crystal of Mn12-acetate. Different forms applied to even and odd-numbered steps provide a distinction between even step resonances (associated with crystal anisotropy) and odd resonances (which require a transverse component of magnetic field).
@article{arxiv.cond-mat/0106579,
title = {A Distribution of Tunnel Splittings in Mn$_{12}$-Acetate},
author = {K. M. Mertes and Yoko Suzuki and M. P. Sarachik and Y. Paltiel and H. Shtrikman and E. Zeldov and E. Rumberger and D. N. Hendrickson and G. Christou},
journal= {arXiv preprint arXiv:cond-mat/0106579},
year = {2009}
}
Comments
4 pages, 5 figures. New title; text more clearly written