Related papers: Mesoscopic Spin Tunneling in Molecular Crystals
A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…
A microscopic model is constructed which is able to describe multiple magnetic flux transitions as observed in recent ultra-low temperature tunnel experiments on an aluminum superconducting ring with normal metal - insulator -…
We present low temperature magnetometry measurements on a new Mn3 single-molecule magnet (SMM) in which the quantum tunneling of magnetization (QTM) displays clear evidence for quantum mechanical selection rules. A QTM resonance appearing…
Relaxation phenomena in glasses can be related to jump processes between different minima of the potential energy in the configuration space. These transitions play a key role in the low temperature regime, giving rise to tunneling systems…
We explore the characteristics of equilibrium tunneling of electrons from a 3D electrode into a high mobility 2D electron system. For most 2D Landau level filling factors, we find that tunneling can be characterized by a single,…
The symmetry of magnetic quantum tunneling (MQT) in the single molecule magnet Mn12-acetate has been determined by sensitive low-temperature magnetic measurements in the pure quantum tunneling regime and high frequency EPR spectroscopy in…
We study the macroscopic quantum tunneling of magnetization of the F=1 spinor condensate interacting through dipole-dipole interaction with an external magnetic field applied along the longitudinal or transverse direction. We show that the…
We studied the physical behavior of PdO nanoparticles at low temperatures, which presents an unusual behavior clearly related to macroscopic quantum tunneling. The samples show a tetragonal single phase with P42/mmc space group. Most…
Multi-spins tunneling cross-relaxations in an ensemble of weakly-coupled Ho$^{3+}$ ions, mediated by weak anisotropic dipolar interactions, can be evidenced by ac-susceptibility measurements in a high temperature regime. Based on a…
Recently, Bellessa et al in a Physical Review Letter entitled "Phonon-Assisted Tunneling in High-Spin Molecules: Experimental Evidence", reported observation of a peak in the imaginary part of the ac-susceptibility of Mn-12 molecular…
The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…
Staircase hysteresis loops of the magnetization of a LiY_0.998Ho_0.002F_4 single crystal are observed at subkelvin temperatures and low field sweep rates. This behavior results from quantum dynamics at avoided level crossings of the energy…
In this paper we report magnetic relaxation data for antiferromagnetic alpha-Fe2O3 particles of 5 nm mean diameter in the temperature range 0.1 K to 25 K. The average spin value of these particles S=124 and the uniaxial anisotropy constant…
A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An…
We explore the quantum dynamics of nuclear spin relaxation in cold collisions of $^1\Sigma^+$ molecules with structureless atoms in an external magnetic field. To this end, we develop a rigorous coupled-channel methodology, which accounts…
In the usual quantum tunneling, a low-energy quantum particle penetrates across a physical barrier of higher potential energy, by traversing a classically forbidden region, and finally escapes into another region. In an analogous scenario,…
Modeling blocking temperature in molecular magnets has been a long standing problem in the field of molecular magnetism. We investigate this problem using a kinetic Monte Carlo (kMC) approach on an assembly of 100,000 short molecular…
We calculate the tunneling splittings in a Mn$_{12}$ magnetic molecule taking into account its internal many-spin structure. We discuss the precision and reliability of these calculations and show that restricting the basis (limiting the…
Below 360 mK, Fe8 magnetic molecular clusters are in the pure quantum relaxation regime. We showed recently that the predicted ``square-root time'' relaxation is obeyed, allowing us to develop a new method for watching the evolution of the…
We study spin tunnelling in molecular magnets as an instance of a mesoscopic phenomenon, with special emphasis on the molecule Fe8. We show that the tunnel splitting between various pairs of Zeeman levels in this molecule oscillates as a…