Related papers: Giant nonlinear optical chirality in twisted heter…
While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is…
The transition metal monopnictide family of Weyl semimetals recently has been shown to exhibit anomalously strong second-order optical nonlinearity, which is theoretically attributed to a highly asymmetric polarization distribution induced…
Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…
Conventional linear optical activity effects are widely used for studying chiral materials. However, poor contrast and artifacts due to sample anisotropy limit the applicability of these methods. Here we demonstrate that nonlinear…
Theory shows that a slab of a dielectric structurally chiral material (DSCM) exhibits both linear and circular dichroisms because of its anisotropy and structural chirality, for normal as well as oblique incidence. This conclusion was…
The interplay between magnetism and light can create abundant optical phenomena. Here, we demonstrate the emergence of an unconventional magnetization-induced second-harmonic generation (MSHG) stemming from vector spin chirality, denoted as…
Chiral photonics provides powerful routes for controlling the light handedness, yet nonlinear chiral responses are typically associated with intricate three-dimensional systems. Here, we demonstrate that strong nonlinear chirality can…
We investigate the interaction between a monolayer of WS2 and a chiral plasmonic metasurface. WS2 possesses valley excitons that selectively couple with one-handed circularly polarised light. At the same time, the chiral plasmonic…
The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…
Chirality arises from the asymmetry of matters, where two counterparts are the mirror image of each other. The interaction between circular-polarization light and quantum materials is enhanced in chiral space groups due to the structural…
Chirality-driven optical properties in charge density waves are of fundamental and practical importance. Here, we investigate the interaction between circularly polarized light and emergent chiral stacking orders in quasi-one-dimensional…
Atomically thin two-dimensional (2D) materials can be vertically stacked with van der Waals bonds, which enable interlayer coupling. In the particular case of transition metal dichalcogenide (TMD) bilayers, the relative direction between…
Metasurfaces have revolutionized nonlinear and quantum light manipulation in the past decade, enabling the design of materials that can tune polarization, frequency, and direction of light simultaneously. However, tuning of metasurfaces is…
Nonlinear optical frequency conversion, in which optical fields interact with a nonlinear medium to produce new field frequencies, is ubiquitous in modern photonic systems. However, the nonlinear electric susceptibilities that give rise to…
Over the past two decades, metamaterials have led to an increasing number of biosensing and nanophotonic applications due to the possibility of a careful control of light propagating through subwavelength features. Chiral nanostructures…
Chiral nonlinear response has been explored for decades due to its extreme sensitivity to molecular and structural dissymmetry. Conventional approaches often require bulky systems and produce only static nonlinear chirality. Here, we report…
Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…
Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…
Stacked atomically thin transition metal dichalcogenides (TMDs) exhibit fundamentally new physical properties compared to those of the individual layers. The twist angle between the layers plays a crucial role in tuning these properties.…
Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers,…