Related papers: Giant nonlinear optical chirality in twisted heter…
Circular dichroism is widely used for characterizing organic and biological materials, but measurements at a single molecule level are challenging because differences in absorption for opposite helicities are small. Here we show that…
Chiral crystals exhibit enantiomer-dependent transport phenomena that generate pure spin or orbital currents, while the handedness sensitivity of spin and orbital Hall conductivities (SHC/OHC) remains insufficiently understood. Using…
Layered van der Waals (vdW) materials have emerged as a promising platform for nanophotonics due to large refractive indexes and giant optical anisotropy. Unlike conventional dielectrics and semiconductors, the absence of covalent bonds…
We show that the nonlinear optical response reflects sensitively the electronic structure of transition-metal surfaces and interfaces. $d$ and $s$ electrons may contribute rather differently to the second harmonic generation (SHG) signal.…
The observation of chirality is ubiquitous in nature. Contrary to intuition, the population of opposite chiralities is surprisingly asymmetric at fundamental levels. Examples range from parity violation in the subatomic weak force to the…
Paucity of naturally occurring noncentrosymmetric materials is stimulating growing interest in engineered two-dimensional systems for nonlinear optical applications. Here, we show that breaking inversion symmetry in centrosymmetric bilayer…
Resonant dielectric planar structures can interact selectively with light of particular helicity thus providing an attractive platform for chiral flat optics. The absence of mirror-symmetry planes defines geometric chirality, and it remains…
Chirality is a pervasive property of matter that underpins many important phenomena across physics, chemistry and biology. Given its broad significance, the development of protocols for rational control of chirality in solid state systems…
Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular…
Shift current and second harmonic generation (SHG) are nonlinear optical responses that are often used for photovoltaic effect and the detection of subtle symmetry breaking patterns in materials. It has been recently shown that topological…
We present an analytical theory of second harmonic generation (SHG) in hybrid structures combining a nonlinear 2D crystal with a dielectric metasurface waveguide. The theory describes the excitation spectrum and enhancement of SHG at both…
The interface between two different semiconductors is crucial in determining the electronic properties at the heterojunction, therefore novel techniques that can probe these regions are of particular interest. Recently it has been shown…
Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is…
Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular…
Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single…
A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2…
Chirality, a fundamental concept from biological molecules to advanced materials, is prevalent in nature. Yet, its intricate behavior in specific topological systems remains poorly understood. Here, we investigate the emergence of hidden…
Non-trivial electronic states are attracting intense attention in low-dimensional physics. Though chirality has been identified in charge states with a scalar order parameter, its intertwining with charge density waves (CDW), film thickness…
Nonlinear chiral photonics explores nonlinear response of chiral structures, and it offers a pathway to novel optical functionalities not accessible through linear or achiral systems. Here we present the first application of nanostructured…
Chiroptical signals, optical responses sensitive to molecular handedness, are rapidly suppressed by multiple scattering, fundamentally limiting their use in turbid media. Here we show that coupling molecular chirality to the topological…