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The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

We report Raman forbidden layer-breathing modes (LBMs) in layered semiconductor materials (LSMs). The intensity distribution of all observed LBMs depends on layer number, incident light wavelength and refractive index mismatch between LSM…

Raman spectroscopic investigations are carried out on one-dimensional nanostructures of InN,such as nanowires and nanobelts synthesized by chemical vapor deposition. In addition to the optical phonons allowed by symmetry; A1, E1 and…

Materials Science · Physics 2009-11-13 Satyaprakash Sahoo , M. S. Hu , C. W. Hsu , C. T. Wu , K. H. Chen , L. C. Chen , A. K. Arora , S. Dhara

Nonlinear optical processes are used in biological microscopy to surpass the diffraction limit on resolution, image deeper into brain tissues, and identify biomolecules without exogenous labels. These techniques typically require high…

Nanophotonics research has focused recently on the ability of non-linear optical processes to mediate and transform optical signals in a myriad of novel devices, including optical modulators, transducers, color filters, photodetectors,…

We report on efficient surface-enhanced Raman spectroscopy (SERS) supporting substrates, which are based on DNA-assisted lithography (DALI) and a layered configuration of materials. In detail, we used nanoscopic DNA origami bowtie templates…

Materials Science · Physics 2023-04-25 Kabusure M. Kabusure , Petteri Piskunen , Jiaqi Yang , Veikko Linko , Tommi K. Hakala

In the realm of healthcare, label-free sensing is a vital component for various applications. Micro-photonic technology presents a promising avenue to pursue pivotal goals. With the use of this technology, healthcare professionals and…

Optics · Physics 2024-04-24 Giuseppina Simone

We revisit laser intensity noise in the context of stimulated Raman scattering (SRS), which has recently proved to be a key technique to provide label free images of chemical bonds in biological and medical samples. Contrary to most…

Instrumentation and Detectors · Physics 2019-10-29 Xavier Audier , Sandro Heuke , Peter Volz , Ingo Rimke , Hervé Rigneault

Stimulated Raman scattering is a well-known nonlinear process that can be harnessed to produce optical gain in a wide variety of media. This effect has been used to produce the first silicon-based lasers and high-gain amplifiers.…

Optics · Physics 2008-10-13 D. R. Solli , P. Koonath , B. Jalali

We employ a quantum theory of the nonlinear optical response from an actual solid-state material possessing an intrinsic bulk contribution to the third-order nonlinear susceptibility (Kerr-type nonlinearity), which can be arbitrarily…

Mesoscale and Nanoscale Physics · Physics 2012-01-25 Sara Ferretti , Dario Gerace

We theoretically analyze and experimentally demonstrate the possibility of amplifying optical signals in an unrepeatered mode-division multiplexed tranmsmission system, through inter-modal stimulated Raman scattering process between signal…

Hyperfine atomic states are among the most promising candidates for qubit encoding in quantum information processing. In atomic systems, hyperfine transitions are typically driven through a two-photon Raman process by a laser field which is…

QED-model for multichain coupled qubit system, proposed in \cite{Part1}, was confirmed by Raman scattering studies of quasi-1D carbon zigzag-shaped nanotubes (CZSNTs), produced by high energy ion beam modification of natural diamond single…

Quantum Physics · Physics 2011-05-27 Dmitry Yearchuck , Alla Dovlatova

Quadratic optical parametric processes form the foundation for a variety of applications related to classical and quantum frequency conversion, which have attracted significant interest recently in on-chip implementation. These processes…

Optics · Physics 2018-09-19 Rui Luo , Yang He , Hanxiao Liang , Mingxiao Li , Qiang Lin

We explore the possibility of achieving a significant nonlinear phase shift among photons propagating in nanoscale waveguides exploiting interactions among photons that are mediated by vibrational modes and induced through Stimulated…

Quantum Physics · Physics 2017-09-28 Hashem Zoubi , Klemens Hammerer

We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…

Micro-ring resonators (MRRs) "trap" incoming light, and therefore, have been shown to achieve extremely high local intensities of light. Thus, they can be used to facilitate highly non-linear optical signals. By embedding materials that…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 A. Sharma , Y. Li , M. K. Prasad , W. L. Ho , S. T. Chu , I. V. Borzenets

Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…

The interest of micro and tip-enhanced Raman spectroscopy to analyze nanosized and nanostructured materials, chiefly semiconductors, oxides and pristine or functionalized carbon nanotubes, is reviewed at the light of the contributions to…

Materials Science · Physics 2007-06-07 Philippe Colomban , Gwénael Gouadec

A possibility to greatly enhance frequency-conversion efficiency of stimulated Raman scattering is shown by making use of extraordinary properties of three-wave mixing of ordinary and backward waves. Such processes are commonly attributed…