Related papers: Raman suppression in nanophotonics enabled by mult…
In optical communications, the Raman effect is exploited for its lasing properties in distributed Raman amplification (DRA) and leads to spectral distortions through inter-channel stimulated Raman scattering (ISRS). In single-mode fibers,…
Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In…
Characterizing a monolayer of biological molecules has been a major challenge. We demonstrate nanophotonic wave-guide enhanced Raman spectroscopy (NWERS) of monolayers in the near-infrared region, enabling real-time measurements of the…
Stimulated Raman scattering (SRS) is a powerful method for label-free imaging and spectroscopy of materials. Recent experiments have shown that quantum-enhanced Raman scattering can surpass the shot noise limit and improve the sensitivity…
Here we show how surface-enhanced Raman spectroscopy (SERS) features can be fine-tuned in optically active substrates made of layered materials. To demonstrate this, we used DNA-assisted lithography (DALI) to create substrates with silver…
Stimulated Raman scattering (SRS) microscopy has emerged as a powerful technique for probing the spatiotemporal dynamics of molecular bonds with exceptional sensitivity, resolution, and speed. However, classically, its performance remains…
Emerging gallium nitride (GaN) vertical power devices require high-quality GaN crystals with reduced crystal defects, especially threading dislocations (TDs), to harness the high critical electric field and electron mobility of the…
We propose a single-atom, cavity quantum electrodynamics system, compatible with recently demonstrated, fiber-integrated micro- and nano-cavity setups, for the on-demand production of optical number-state, $0N$-state, and…
Raman spectroscopy is a label-free, chemically specific optical technique which provides detailed information about the chemical composition and structure of the excited analyte. Because of this, there is growing research interest in…
We propose an all-optical scheme to control the photon statistics using hybrid quantum plasmonic system. With the aid of dressed states assisted quantum interference effects, it is shown that the photon correlations of a signal field can be…
We show that spontaneous Raman scattering of incident radiation can be observed in cavity-QED systems without external enhancement or coupling to any vibrational degree of freedom. Raman scattering processes can be evidenced as resonances…
Solid state quantum emitters have shown strong potential for applications in quantum information, but spectral inhomogeneity of these emitters poses a significant challenge. We address this issue in a cavity-quantum dot system by…
Solid-state quantum emitters coupled to integrated photonic nanostructures are quintessential for exploring fundamental phenomena in cavity quantum electrodynamics and widely employed in photonic quantum technologies such as non-classical…
The coupling evolutions of stimulated Raman scattering (SRS) and Raman rescattering (re-SRS) are studied under the parameter conditions of relevance to the gas-filled hohlraum experiments at the National Ignition Facility by a nonenveloped…
The Raman scattering of light by molecular vibrations offers a powerful technique to 'fingerprint' molecules via their internal bonds and symmetries. Since Raman scattering is weak, methods to enhance, direct and harness it are highly…
Raman scattering, an inelastic scattering mechanism, provides information about molecular excitation energies and can be used to identify chemical compounds. Albeit being a powerful analysis tool, especially for label-free biomedical…
Surface-enhanced Raman scattering (SERS) is a critical tool for chemical sensing and spectroscopy, and a key question is how to optimally design nanostructures for maximizing SERS. We present fundamental limits on spatially-averaged SERS…
Silicon nitride microresonators have become an ubiquitous platform for cutting-edge photonics applications. Improvement in silicon nitride fabrication techniques, providing ultra-high quality-factor values up to $10^7$, has opened up new…
Low-frequency Raman scattering experiments have been performed on thin films consisting of nickel-silver composite nanoparticles embedded in alumina matrix. It is observed that the Raman scattering by the quadrupolar modes, strongly…
It is known that the more tractable Markovian models of coupling suited for weak interactions may overestimate the Rabi frequency notably when applied to the strong-coupling regime. Here, a more significant consequence of the non-Markovian…