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We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this…

Quantum Physics · Physics 2019-07-10 Roberto de J. León-Montiel , Jiří Svozilík , Juan P. Torres , Alfred B. U'Ren

This paper presents the optimization of a dual-chirped optical parametric amplification (DC-OPA) scheme for producing an ultrafast intense infrared (IR) pulse. By employing a total energy of 0.77 J Ti:sapphire pump laser and type-I BBO…

Doubly charged molecular cations often carry signatures of electronic correlation and electron-nuclear entanglement present in the parent cation. Here, we produce ethylene dications using a combination of an extreme ultraviolet pump and…

We consider the ionization of neon induced by a femtosecond laser pulse composed of overlapping, linearly polarized bichromatic extreme ultraviolet and infrared fields. In particular, we study the effects of the infrared light on a…

Atomic Physics · Physics 2017-01-25 Nicolas Douguet , Alexei N. Grum-Grzhimailo , Klaus Bartschat

Arbitrary Detuning ASynchronous OPtical Sampling (ADA-SOPS) is an emerging technique for extending standard pump--probe experiments performed with two femtosecond lasers to multitimescale experiments, which are of great interest for the…

Optics · Physics 2026-04-17 Laura Antonucci , A. Bonvalet , X. Solinas , M. Joffre

On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum…

We demonstrate an efficient fiber-coupled source of nondegenerate polarization entangled photons at 795 and 1609 nm using bidirectionally pumped parametric down-conversion in bulk periodically poled lithium niobate. The single-mode source…

Quantum Physics · Physics 2016-08-16 Friedrich König , Elliott J. Mason , Franco N. C. Wong , Marius A. Albota

Integrated green light sources are essential for telecommunications and quantum applications, while the performance of current on-chip green light generation is still limited in power and tunability. In this work, we demonstrate green light…

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

We present a Ho:YLF Chirped-Pulse Amplification (CPA) laser for pumping a longwave infrared Optical Parametric Chirped Pulse Amplifier (OPCPA) at a 1 kHz repetition rate. By utilizing a Ti:Sapphire laser as a frontend, 5-{\mu}J seed pulses…

Ultrafast electron dynamics drive phenomena such as photochemical reactions, catalysis, and light harvesting. To capture such dynamics in real-time, femtosecond to attosecond light sources are extensively used. However, an exact match…

Microresonator-based degenerate optical parametric oscillation (DOPO) has recently been explored as a compelling platform for all-optical computing and quantum information applications, such as truly random number generation and the…

We demonstrate a new regime for mid-infrared optical parametric chirped pulse amplification (OPCPA) based on achromatic quasi-phase-matching. Our mid-infrared OPCPA system is based on collinear aperiodically poled lithium niobate (APPLN)…

A cascade of two-level superconducting artificial atoms -- a source and a probe -- strongly coupled to a semi-infinite waveguide is a promising tool for observing nontrivial phenomena in quantum nonlinear optics. The probe atom can scatter…

Spontaneous Raman emission in atomic gases provides an attractive source of photon pairs with a controllable delay. We show how this technique can be implemented in solid state systems by appropriately shaping the inhomogeneous broadening.…

Quantized nano-objects offer a myriad of exciting possibilities for manipulating electrons and light that impact photonics, nanoelectronics, and quantum information. In this context, ultrashort laser pulses combined with nanotips and field…

Multi-photon microscopy has played a significant role in biological imaging since it allows to observe living tissues with improved penetration depth and excellent sectioning effect. Multi-photon microscopy relies on multi-photon…

While time-resolved pump-probe differential reflectivity and transmitivity measurements are routinely used to monitor the population relaxation dynamics on the subpicosecond time scale, it is also known that the signal in the negative delay…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Richarj Mondal , Basabendra Roy , Bipul Pal , Bhavtosh Bansal

We present an entirely fiber based laser source for non-linear imaging with a novel approach for multi-color excitation. The high power output of an actively modulated and amplified picosecond fiber laser at 1064 nm is shifted to longer…