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Pump-probe experiments combining pulses from a X-ray FEL and an optical femtosecond laser are very attractive for sub-picosecond time-resolved studies. Since the synchronization between the two independent light sources to an accuracy of…

Accelerator Physics · Physics 2009-11-10 J. Feldhaus , M. Koerfer , T. Moeller , J. Pflueger , E. L. Saldin , E. A. Schneidmiller , S. Schreiber , M. V. Yurkov

We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled…

Quantum Physics · Physics 2016-11-23 Abu Thomas , Mackenzie Van Camp , Olga Minaeva , David Simon , Alexander V. Sergienko

We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…

Chemical Physics · Physics 2017-05-03 Denis Jelovina , Johannes Feist , Fernando Martín , Alicia Palacios

Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…

A chirped-pulse interleaving method is reported for generation of dual optical frequency combs based on electro-optic phase modulators (EOM) in a free-running all-fiber based system. Methods are discussed to easily modify the linear chirp…

We present a joint experimental and theoretical study on strong-field photo-ionization of sodium atoms using chirped femtosecond laser pulses. By tuning the chirp parameter, selectivity among the population in the highly excited states 5p,…

Atomic Physics · Physics 2015-05-28 M Krug , T Bayer , M Wollenhaupt , C Sarpe-Tudoran , T Baumert , S S Ivanov , N V Vitanov

We present the experimental demonstration of a method for generating two spectrally and temporally separated pulses by an externally seeded, single-pass free-electron laser operating in the extreme-ultraviolet spectral range. Our results,…

Four-wave mixing processes are ubiquitous in ultrafast optics and the determination of the coefficients of the $\chi^{(3)}$ tensor is thus essential. We introduce a novel time-resolved ultrafast spectroscopic method to characterize the…

Two color laser pulses are used to form an air plasma and generate broadband infrared radiation suitable as a seed for backward Raman amplification of CO2 laser pulses. Broadband radiation in the atmospheric window from 8-14 microns is…

We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…

Optics · Physics 2018-06-22 Xavier Audier , Naveen Balla , Herve Rigneault

We present an experimental implementation of a chirped mid-infrared (mid-IR) high-power laser source with variable center frequency between 4 THz to 30 THz and continuously tunable frequency sweep of up to 20 % within one pulse, with a…

In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…

Chemical Physics · Physics 2019-11-28 Giovanni Batignani , Carino Ferrante , Giuseppe Fumero , Tullio Scopigno

Lithium niobate on insulator (LNOI) has a great potential for photonic integrated circuits, providing substantial versatility in design of various integrated components. To properly use these components in the implementation of different…

Quantum Physics · Physics 2021-10-22 L. Ebers , A. Ferreri , M. Hammer , M. Albert , C. Meier , J. Förstner , P. R. Sharapova

The blooming of attosecond science (1 as = $10^{-18}$ s) has raised the need to exquisitely control the delay between two ultrashort light pulses, one of them being intense and in the visible spectral range, while the second is weak and in…

Advanced photonic materials showing two-photon absorption (2PA) have been widely explored to develop three-dimensional imaging, micro and nanofabrication, all-optical switching, lithography on a nanoscale and many other enabling…

We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…

Atomic Physics · Physics 2009-10-20 Andrey Gandman , Leonid Rybak , Michal Bronstein , Naser Shakour , Zohar Amitay

Photon pairs produced by the pulse-pumped nonlinear parametric processes have been a workhorse of quantum information science. Engineering the spectral property of the photon pairs is crucial in practical applications. In this article, we…

Quantum Physics · Physics 2022-01-05 Liang Cui , Jinjin Wang , Jiamin Li , Mingyi Ma , Z. Y. Ou , Xiaoying Li

Photonics offers unique capabilities for quantum information processing (QIP) such as room-temperature operation, the scalability of nanophotonics, and access to ultrabroad bandwidths and consequently ultrafast operation. Ultrashort-pulse…

We report on the design and numerical simulation of a tunable, near-infrared (NIR) femtosecond noncollinear optical parametric amplifier (OPA) seeded by a nonlinear fiber amplifier operating in the parabolic and gain-managed regime. With…

Optics · Physics 2023-05-08 Brittany Lu , Keith Wernsing , Sergio Carbajo

We introduce a new scheme for generating short-wavelength coherent broadband radiation with well-controlled spectral characteristics. It is based on shaping long-wavelength femtosecond pulse to coherently control atomic resonance-mediated…

Atomic Physics · Physics 2009-10-20 Leonid Rybak , Lev Chuntonov , Andrey Gandman , Naser Shakour , Zohar Amitay
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