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Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…

Excitation of the isomeric nuclear state 229m Th in the process of thorium atom irradiation by two-color femtosecond pulse of Ti: Sa laser at the fundamental wavelength and second harmonic is analyzed. It is shown that the rate of isomeric…

Optics · Physics 2019-01-23 A. V. Andreev , A. B. Savelyev , S. Yu. Stremoukhov , O. A. Shoutova

$^{229}$Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of $^{229}$Th has so far hindered…

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…

The nucleus of 229Thorium presents a unique isomer state of very low energy and long lifetime, current estimates are around 7.8 eV and seconds to hours respectively. This nuclear transitions therefore is a promising candidate for a novel…

Atomic Physics · Physics 2013-04-18 G. A. Kazakov , M. Schreitl , G. Winkler , J. H. Sterba , G. Steinhauser , T. Schumm

Motivated by recent experimental breakthroughs toward a realization of a solid-state Thorium-229 nuclear clock, we review the technology, basic physics motivation, and limitations of the present generation of atomic clocks. We then discuss…

Atomic Physics · Physics 2025-11-18 Steven M. Girvin , Leo Radzihovsky

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

The recent demonstration of laser excitation of the $\approx 8$ eV isomeric state of Thorium-229 is a significant step towards a nuclear clock. The low excitation energy likely results from a cancellation between electromagnetic and strong…

High Energy Physics - Phenomenology · Physics 2025-09-16 Andrea Caputo , Doron Gazit , Hans-Werner Hammer , Joachim Kopp , Gil Paz , Gilad Perez , Konstantin Springmann

In-source resonance ionization spectroscopy was used to identify an efficient and selective three step excitation/ionization scheme of thorium, suitable for titanium:sapphire (Ti:sa) lasers. The measurements were carried out in preparation…

We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou

We review the ideas and concepts for a clock that is based on a radiative transition in the nucleus rather than in the electron shell. This type of clock offers advantages like an insensitivity against field-induced systematic frequency…

Nuclear Experiment · Physics 2015-06-18 Ekkehard Peik , Maxim Okhapkin

The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…

Quantum Physics · Physics 2025-08-15 Jingbo Wang , Haixing Miao , Shiqian Ding , Dong E. Liu

Given the drastic progress achieved during recent years in our knowledge on the decay and nuclear properties of the thorium isomer 229mTh, the focus of research on this potential nuclear clock transition will turn in the near future from…

Nuclear Experiment · Physics 2021-09-08 P. G. Thirolf , B. Seiferle , L. v. d. Wense , I. Amersdorffer , D. Moritz , J. Weitenberg

Continuous-wave output at 229 nm for the application of laser cooling of Cd atoms was generated by the 4th harmonic using two successive second harmonic generation stages. Employing a single-frequency optically pumped semiconductor laser as…

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…

Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of the…

Laser excitation of thorium-229 nuclei in doped wide bandgap crystals has been demonstrated recently, opening the possibility of developing ultrastable solid-state clocks and sensitive searches for new physics. We develop a quantitative…

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

The $^{229}$Th nucleus has a unique transition at only 8 eV which could be used for a novel nuclear clock. We investigate theoretically the prospects of driving this transition with vortex light beams carrying orbital angular momentum.…

Atomic Physics · Physics 2024-04-22 Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy

The most probable candidate for the role of a nuclear optical standard is the 8.338-eV isomer of the 229mTh isotope of the thorium nucleus. Ways of using the resonance properties of the electron shell as an optical resonator to create…

Nuclear Theory · Physics 2023-07-19 F. F. Karpeshin , L. F. Vitushkin