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Doping problems in GaN and in AlGaN alloys are addressed on the basis of state-of-the-art first-principles calculations. For n-type doping we find that nitrogen vacancies are too high in energy to be incorporated during growth, but silicon…

Condensed Matter · Physics 2009-10-31 Chris G. van de Walle , Catherine Stampfl , Joerg Neugebauer

Controllable doping in AlN and its alloys is essential for deep-ultraviolet light sources. Ionization energies for donors in AlN ($\mathrm{Si_{Al}}$, $\mathrm{S_N}$, $\mathrm{Se_N}$) are high. We report first-principles calculations…

Materials Science · Physics 2026-03-05 Haochen Wang , Chris G. Van de Walle

Hyperdoping, overcoming the solubility limit of dopants in a crystalline semiconductor, is a fertile method for the enhancement of the electrical, structural and optical devices' performances and for the exploration of exotic phases such as…

Achieving efficient n-type doping in AlN, a representative ultrawide bandgap (UWBG) semiconductor, remains a longstanding challenge that limits its application in high-power electronics and deep-ultraviolet optoelectronics. Conventional…

Materials Science · Physics 2025-12-04 Yujie Liu , Sieun Chae , Emmanouil Kioupakis

Transitioning to solid-state ultraviolet (UV) lighting is critical for reducing global energy utilization to meet net-zero targets. AlGaN-based far-UVC LEDs offer a mercury-free, energy-efficient alternative to conventional mercury lamps,…

Materials Science · Physics 2026-03-18 Ling Zhang , Miao Zhou , Alex M. Ganose

(Al$_x$Ga$_{1{\rm -}x})_2$O$_3$ alloys are frequently used in heterostructures with monoclinic Ga$_2$O$_3$, resulting in a large conduction-band offset, which leads to charge carrier confinement, a property that is desirable for device…

Materials Science · Physics 2026-05-13 Sierra Seacat , Hartwin Peelaers

N-type doping in Si by shallow impurities, such as P, As and Sb, exhibits an intrinsic limit due to the Fermi-level pinning via defect complexes at high doping concentrations. Here we demonstrate that doping Si with the chalcogen Te by…

In this letter, carrier transport in graded Al$\mathrm{_x}$Ga$\mathrm{_{1-x}}$N with a polarization-induced n-type doping as low as ~ 10$\mathrm{^{17}}$ cm$\mathrm{^{-3}}$ is reported. The graded Al$\mathrm{_x}$Ga$\mathrm{_{1-x}}$N is grown…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Mingda Zhu , Meng Qi , Kazuki Nomoto , Zongyang Hu , Bo Song , Ming Pan , Xiang Gao , Debdeep Jena , Huili Grace Xing

Polarization induced degenerate $n$-type doping with electron concentrations up to $\sim$10$^{20}$\,cm$^{-3}$ is achieved in graded Al$_{x}$Ga$_{1-x}$N layers ($x$: 0\%$\rightarrow$37\%) grown on unintentionally doped and on $n$-doped…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 R. Adhikari , Tian Li , G. Capuzzo , A. Bonanni

Cubic boron nitride (cBN) is an ultra-wide bandgap, super-hard material with potential for extreme-temperature and -pressure applications. A proof-of-principle p-n junction using cBN was demonstrated almost three decades ago. However, to…

Materials Science · Physics 2022-02-04 Tamanna Joshi , Pankaj Kumar , Bipul Poudyal , Sean Paul Russell , Priyanka Manchanda , Pratibha Dev

We use hybrid density functional calculations to assess n-type doping in monoclinic (Al$_x$Ga$_{1-x}$)$_2$O$_3$ alloys. We focus on Si, the most promising donor dopant, and study the structural properties, formation energies and…

While Si is an effective insertion type anode for Li-ion batteries, crystalline Si has been shown to be unsuitable for Na and Mg storage due, in particular, to insufficient binding strength. It has recently been reported that Si nanowires…

Materials Science · Physics 2016-02-05 Fleur Legrain , Sergei Manzhos

Semiconductor materials that can be doped both n-type and p-type are desirable for diode-based applications and transistor technology. Copper nitride (Cu3N) is a metastable semiconductor with a solar-relevant bandgap that has been reported…

We report the effect of germanium as n-type dopant on the electrical and optical properties of AlxGa1-xN layers grown by plasma assisted molecular-beam epitaxy. The Al content has been varied from x = 0 to 0.66, confirmed by Rutherford…

Materials Science · Physics 2019-02-12 R. Blasco , A. Ajay , E. Robin , C. Bougerol , K. Lorentz , L. C. Alves , I. Mouton , L. Amichi , A. Grenier , E. Monroy

We present ab initio density-functional calculations for acceptors, donors, and native defects in aluminum nitride, showing that acceptors are deeper (Be ~ 0.25 eV, Mg_ 0.45 eV) and less soluble than in GaN; at further variance with GaN,…

Materials Science · Physics 2009-10-31 Antonella Fara , Fabio Bernardini , Vincenzo Fiorentini

We investigate the self-compensation mechanism in phosphorus-doped CdTe. The formation energies, charge transition levels, and defects states of several P-related point defects susceptible to cause self-compensation are addressed by…

Materials Science · Physics 2017-10-20 Mauricio A. Flores , Walter Orellana , Eduardo Menéndez-Proupin

Aluminum nitride is a promising ultra-wide band gap semiconductor for optoelectronics and power electronics. However, its practical applications have been limited by challenges with doping and achieving high electrical conductivity. Recent…

Materials Science · Physics 2025-06-12 Amanda Wang , Nick Pant , Woncheol Lee , Jie-Cheng Chen , Feliciano Giustino , Emmanouil Kioupakis

Diamond, a wide band-gap semiconductor, can be engineered to exhibit superconductivity when doped heavily with boron. The phenomena has been demonstrated in samples grown by chemical vapour deposition where the boron concentration exceeds…

A nonequilibrium Green's function technique combined with density functional theory is used to study the spin-dependent electronic band structure and transport properties of zigzag silicene nanoribbons (ZSiNRs) doped with aluminum (Al) or…

Materials Science · Physics 2014-09-01 J. Chen , X. F. Wang , P. Vasilopoulos , A. B. Chen , J. C. Wu

Acceptor-type defects in highly n-type InN are probed using positron annihilation spectroscopy. Results are compared to Hall effect measurements and calculated electron mobilities. Based on this, self-compensation in n-type InN is studied…

Materials Science · Physics 2012-07-09 C. Rauch , F. Tuomisto , P. D. C. King , T. D. Veal , H. Lu , W. J. Schaff
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