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Motivated by the report of superconductivity in bilayer La$_3$Ni$_2$O$_7$ at high pressure, we examine the interacting electrons in this system. First-principles many-body theory is utilized to study the normal-state electronic properties.…

Strongly Correlated Electrons · Physics 2023-12-04 Frank Lechermann , Jannik Gondolf , Steffen Bötzel , Ilya M. Eremin

We study the nature of orbital correlations present in the bilayer nickelate within a minimal two-orbital tight-binding model to gain insights into their possible role in stabilizing the less-known weakly-insulating state. The latter has…

Strongly Correlated Electrons · Physics 2025-03-11 Garima Goyal , Aastha Jain , Dheeraj Kumar Singh

Developing a low-energy model is essential for understanding unconventional superconductivity in bilayer nickelate La$_3$Ni$_2$O$_7$. Here, we analyze distinct low-energy scenarios of the normal state by downfolding the ab-initio determined…

Strongly Correlated Electrons · Physics 2025-05-19 Frank Lechermann , Steffen Bötzel , Ilya M. Eremin

Motivated by the high temperature superconductivity observed in the bilayer nickelate La$_3$Ni$_2$O$_7$ and the spectroscopic evidences of strong electron correlations in this compound, we address the role of its multiorbital electron…

Superconductivity · Physics 2024-12-31 Zhiguang Liao , Yiming Wang , Lei Chen , Guijing Duan , Rong Yu , Qimiao Si

Motivated by the discovery of high-temperature superconductivity in bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure, we investigate the ground-state phase diagram and correlation effects using determinant quantum Monte Carlo simulations…

Strongly Correlated Electrons · Physics 2025-02-07 Jian-Jian Yang , Dao-Xin Yao , Han-Qing Wu

Recently discovered high-$T_c$ superconductivity in thin-film bilayer nickelates La$_3$Ni$_2$O$_7$ under ambient pressure has attracted great interest. Non-Fermi-liquid transport behaviors, such as $T$-linear resistivity and a positive Hall…

Strongly Correlated Electrons · Physics 2026-05-13 Seiichiro Onari , Daisuke Inoue , Rina Tazai , Youichi Yamakawa , Hiroshi Kontani

Motivated by the recently reported high-temperature superconductivity in the bilayer La$_3$Ni$_2$O$_7$ (LNO) under pressure, here we comprehensively study this system using {\it ab initio} techniques. The Ni $3d$ orbitals have a large…

Superconductivity · Physics 2023-11-29 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

The interplay of spin-orbit-coupling and strong electronic correlations is studied for the single-layer and the bilayer compound of the strontium ruthenate Ruddlesden-Popper series by a combination of first-principles band-structure theory…

Strongly Correlated Electrons · Physics 2012-08-08 Malte Behrmann , Christoph Piefke , Frank Lechermann

Motivated by the recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ under pressure, we discuss the basic ingredients of a model that captures its microscopic physics under pressure tuning. We anchor our description in terms of the…

Superconductivity · Physics 2024-08-01 Zhiguang Liao , Lei Chen , Guijing Duan , Yiming Wang , Changle Liu , Rong Yu , Qimiao Si

Recently, signatures of superconductivity with critical temperature from 20 to 30 K have been reported in pressured trilayer nickelate La$_4$Ni$_3$O$_{10}$ through a pressure-induced structure transition. Here we explore the evolution of…

Strongly Correlated Electrons · Physics 2024-06-18 Peng-Fei Tian , Hao-Tian Ma , Xing Ming , Xiao-Jun Zheng , Huan Li

It has been recently shown that under pressure trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ (LNO) becomes superconducting below a critical temperature $\sim$20 K, in addition to the infinite-layer and bilayer systems. Motivated…

Strongly Correlated Electrons · Physics 2024-06-12 I. V. Leonov

We explore the optical properties of La3Ni2O7 bilayer nickelates by using density functional theory including a Coulomb repulsion term. Convincing agreement with recent experimental ambient-pressure spectra is achieved for U=3eV, which…

Recently, superconductivity with a $T_c$ up to 78 K has been reported in bulk samples of the bilayer nickelate La$_3$Ni$_2$O$_7$ at pressures above 14 GPa. Important theoretical tasks are the formulation of relevant low-energy models and…

Strongly Correlated Electrons · Physics 2023-11-17 Viktor Christiansson , Francesco Petocchi , Philipp Werner

We propose a theory for bilayer nickelate materials, where a large tetragonal field - intrinsic or induced by epitaxial strain - lifts the orbital degeneracy and localizes the $3z^2-r^2$ orbital states. These states host local spins $S=1/2$…

Strongly Correlated Electrons · Physics 2026-01-22 Giniyat Khaliullin , Jiří Chaloupka

High-pressure superconductivity in the bilayer nickelate La$_3$Ni$_2$O$_7$, with a transition temperature approaching 80 K, has stimulated intense debate regarding its microscopic origin. Although an $s_{\pm}$ gap symmetry has been widely…

Superconductivity · Physics 2026-03-17 Hiroshi Watanabe , Hirofumi Sakakibara , Kazuhiko Kuroki

The recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ raises key questions about its mechanism and the nature of pairing symmetry. This system is believed to be described by a bilayer two-orbital Hubbard model. The considerations…

Superconductivity · Physics 2025-02-14 Guijing Duan , Zhiguang Liao , Lei Chen , Yiming Wang , Rong Yu , Qimiao Si

Superconductivity in nickelates apparently takes place in two different Ni oxidation regimes, namely either for infinite-layer-type compounds close to Ni$^{+}$, or for Ruddlesden-Popper materials close to Ni$^{2+}$. The reduced…

Strongly Correlated Electrons · Physics 2025-12-12 Frank Lechermann , Steffen Bötzel , Ilya M. Eremin

Superconductivity has been demonstrated in the family of multi-layered nickelates La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$. Key questions remain open regarding the low-energy electronic states that support superconductivity in these…

Recent angle-resolved photoemission measurements on La$_3$Ni$_2$O$_7$ have challenged the density-functional-theory-based picture of three Fermi surfaces by revealing that the $d_{z^2}$-derived $\gamma$ band can reside below the Fermi…

Strongly Correlated Electrons · Physics 2026-05-12 Yong-Yue Zong , Shun-Li Yu , Jian-Xin Li

Recently, the bulk nickelate La$_3$Ni$_2$O$_7$ is reported to show signature of high-temperature superconductivity under high pressure above $14$GPa [H. Sun et al., Nature 621, 493 (2023)]. We analyze the pairing mechanism and pairing…

Superconductivity · Physics 2023-10-19 Qing-Geng Yang , Da Wang , Qiang-Hua Wang
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