English

Electron correlations and superconductivity in La$_3$Ni$_2$O$_7$ under pressure tuning

Superconductivity 2024-08-01 v2 Strongly Correlated Electrons

Abstract

Motivated by the recent discovery of superconductivity in La3_3Ni2_2O7_7 under pressure, we discuss the basic ingredients of a model that captures its microscopic physics under pressure tuning. We anchor our description in terms of the spectroscopic evidence of strong correlations in this system. In a bilayer Hubbard model including the Ni 3d3d x2y2x^2-y^2 and z2z^2 orbitals, we show the ground state of the model crosses over from a low-spin S=1/2S=1/2 state to a high-spin S=3/2S=3/2 state. In the high-spin state, the two x2y2x^2-y^2 and the bonding z2z^2 orbitals are all close to half-filling, which promotes a strong orbital selectivity in a broad crossover regime of the phase diagram pertinent to the system. Based on these results, we construct an effective multiorbital tt-JJ model to describe the superconductivity of the system, and find the leading pairing channel to be an intraorbital spin singlet with a competition between the extended ss-wave and dx2y2d_{x^2-y^2} symmetries. Our results highlight the role of strong multiorbital correlation effects in driving the superconductivity of La3_3Ni2_2O7_7.

Keywords

Cite

@article{arxiv.2307.16697,
  title  = {Electron correlations and superconductivity in La$_3$Ni$_2$O$_7$ under pressure tuning},
  author = {Zhiguang Liao and Lei Chen and Guijing Duan and Yiming Wang and Changle Liu and Rong Yu and Qimiao Si},
  journal= {arXiv preprint arXiv:2307.16697},
  year   = {2024}
}

Comments

5.5+4 pages, 4+3 figures, 2 tables, updated version with supplemental material