English

Superconductivity in nickelate and cuprate superconductors with strong bilayer coupling

Superconductivity 2024-07-30 v2

Abstract

The discovery of superconductivity at 80 K under high pressure in La3_3Ni2_2O7_7 presents the groundbreaking confirmation that high-TcT_c superconductivity is a property of strongly correlated materials beyond cuprates. We use density functional theory (DFT) calculations of the band structure of La3_3Ni2_2O7_7 under pressure to verify that the low-energy bands are composed almost exclusively of Ni 3dx2y2d_{x^2-y^2} and O 2pp orbitals. We deduce that the Ni 3dz2d_{z^2} orbitals are essentially decoupled by the geometry of the high-pressure structure and by the effect of the Ni Hund coupling being strongly suppressed, which results from the enhanced interlayer antiferromagnetic interaction between dz2d_{z^2} orbitals and the strong intralayer hybridization of the dx2y2d_{x^2-y^2} orbitals with O 2pp. By introducing a tight-binding model for the Fermi surfaces and low-energy dispersions, we arrive at a bilayer tt-tt_\perp-JJ model with strong interlayer hopping, which we show is a framework unifying La3_3Ni2_2O7_7 with cuprate materials possessing similar band structures, particularly the compounds La2_2CaCu2_2O6_6, Pb2_2Sr2_2YCu3_3O8_8, and EuSr2_2Cu2_2NbO8_8. We use a renormalized mean-field theory to show that these systems should have (dd+isis)-wave superconductivity, with a dominant dd-wave component and the high TcT_c driven by the near-optimally doped β\beta band, while the α\alpha band adds an ss-wave component that should lead to clear experimental signatures.

Keywords

Cite

@article{arxiv.2312.17064,
  title  = {Superconductivity in nickelate and cuprate superconductors with strong bilayer coupling},
  author = {Zhen Fan and Jian-Feng Zhang and Bo Zhan and Dingshun Lv and Xing-Yu Jiang and Bruce Normand and Tao Xiang},
  journal= {arXiv preprint arXiv:2312.17064},
  year   = {2024}
}

Comments

11 pages, 4 figures