English

Correlated electronic structure of La$_3$Ni$_2$O$_7$ under pressure

Strongly Correlated Electrons 2023-11-17 v2

Abstract

Recently, superconductivity with a TcT_c up to 78 K has been reported in bulk samples of the bilayer nickelate La3_3Ni2_2O7_7 at pressures above 14 GPa. Important theoretical tasks are the formulation of relevant low-energy models and the clarification of the normal state properties. Here, we study the correlated electronic structure of the high-pressure phase in a four-orbital low-energy subspace using different many-body approaches: GWGW, dynamical mean field theory (DMFT), extended DMFT (EDMFT) and GWGW+EDMFT, with realistic frequency-dependent interaction parameters. The nonlocal correlation and screening effects captured by GWGW+EDMFT result in an instability towards the formation of charge stripes, with the 3dz23d_{z^2} as the main active orbital. We also comment on the potential relevance of the rare-earth self-doping pocket, since hole doping suppresses the ordering tendency.

Keywords

Cite

@article{arxiv.2306.07931,
  title  = {Correlated electronic structure of La$_3$Ni$_2$O$_7$ under pressure},
  author = {Viktor Christiansson and Francesco Petocchi and Philipp Werner},
  journal= {arXiv preprint arXiv:2306.07931},
  year   = {2023}
}

Comments

Published version