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The ruthenium halide $\alpha$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $\alpha$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for…

Despite the presence of the exact solution and well-established recipe for its realization, the quest for the Kitaev spin liquid in real materials remains exceptionally challenging. Among many magnets, $\alpha$-RuCl$_3$ emerges as a prime…

Strongly Correlated Electrons · Physics 2024-12-30 Lingzhi Zhang , Yukitoshi Motome

The present studies show that long-range magnetic order takes place in RuBr$_3$ at $\approx$ 34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites.…

Strongly Correlated Electrons · Physics 2024-02-27 T. Weinhold , C. Wang , F. Seewald , V. Grinenko , Y. Imai , F. Sato , K. Ohgushi , H. -H. Klauss , R. Sarkar

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

The recent synthesis of ruthenium trihalides Ru$X_3$ ($X$ = Cl, Br, I) has enlarged the set of material candidates for Kitaev spin liquid. The realization of Kitaev model necessitates the formation of $J=1/2$ pseudospins in the octahedral…

Strongly Correlated Electrons · Physics 2024-05-31 H. Gretarsson , H. Fujihara , F. Sato , H. Gotou , Y. Imai , K. Ohgushi , B. Keimer , H. Suzuki

Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

$\alpha$-RuCl$_3$ has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a…

Strongly Correlated Electrons · Physics 2025-07-15 Jiefu Cen , Hae-Young Kee

Van der Waals materials hosting Kitaev interactions are promising platforms for exploring exotic quantum phenomena. Here, we report inelastic neutron scattering investigations of the van der Waals antiferromagnet VBr3, which forms a…

Strongly Correlated Electrons · Physics 2026-03-03 Zeyu Kao , Yimeng Gu , Yiqing Gu , Hao Zhang , Shiyi Zheng , Naoki Murai , Seiko Ohira-Kawamura , Jun Zhao

We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…

Strongly Correlated Electrons · Physics 2024-03-08 Subin Kim , Ezekiel Horsley , Christie Nelson , Jacob Ruff , Young-June Kim

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

Strongly Correlated Electrons · Physics 2022-01-13 Heung-Sik Kim

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

Strongly Correlated Electrons · Physics 2017-12-12 P. Lampen-Kelley , A. Banerjee , A. A. Aczel , H. B. Cao , M. B. Stone , C. A. Bridges , J. -Q. Yan , S. E. Nagler , D. Mandrus

Recent experiments reveal that the honeycomb ruthenium trichloride {\alpha}-RuCl3 is a prime candidate of the Kitaev quantum spin liquid (QSL). However, there is no theoretical model which can properly describe its experimental dynamical…

Strongly Correlated Electrons · Physics 2017-08-16 Y. S. Hou , H. J. Xiang , X. G. Gong

Motivated by recent reports of metallic behavior in the recently synthesized RuI$_3$, in contrast to the Mott-insulating nature of the actively discussed $\alpha$-RuCl$_3$, as well as RuBr$_3$, we present a detailed comparative analysis of…

Strongly Correlated Electrons · Physics 2022-08-17 David A. S. Kaib , Kira Riedl , Aleksandar Razpopov , Ying Li , Steffen Backes , Igor I. Mazin , Roser Valenti

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

Twisted heterostructures of van der Waals materials have received much attention for their many remarkable properties. Here, we present a comprehensive theory of the long-range ordered magnetic phases of twisted bilayer $\alpha$-RuCl$_3$…

Materials Science · Physics 2023-10-20 Muhammad Akram , Jesse Kapeghian , Jyotirish Das , Roser Valenti , Antia S. Botana , Onur Erten

The mechanical properties of magnetic materials are instrumental for the development of the magnetoelastic theory and the optimization of strain-modulated magnetic devices. In particular, two-dimensional (2D) magnets hold promise to enlarge…

We study on transport and magnetic properties of hydrated and lithium-intercalated $\alpha$-RuCl$_3$, Li$_x$RuCl$_3 \cdot y$H$_2$O, for investigating the effect on mobile-carrier doping into candidate materials for a realization of a Kitaev…

Strongly Correlated Electrons · Physics 2019-06-26 Yoshinori Imai , Katsuya Konno , Yoshinao Hasegawa , Takuya Aoyama , Kenya Ohgushi

Cr$_{\frac{1}{4}}$NbSe$_2$ is a triangular lattice magnet in which magnetic Cr$^{3+}$ ions are intercalated to form triangular lattices between NbSe$_2$ van der Waals layers stacked along the c axis. By unpolarized and polarized neutron…

The van der Waals material CrSBr stands out as a promising two-dimensional magnet. Especially, its high magnetic ordering temperature and versatile magneto-transport properties make CrSBr an important candidate for new devices in the…

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