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We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…

Paraxial light skyrmions are topological configurations that map a spatial domain of the field onto the full Poincar\'e sphere of polarization states. While optical skyrmions have been explored in continuous-wave regimes, their realization…

Optics · Physics 2025-10-17 David Marco , Luis Plaja , Carlos Hernández-García

Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber,…

Quantum Physics · Physics 2025-04-21 Philipp Stammer , Javier Rivera-Dean , Maciej Lewenstein

With the generation of high order harmonics (HHG) on the plasma surface it is possible to turn the laser pulse into a train of attosecond or even zeptosecond pulses in the back radiation. These attosecond pulses may have amplitude several…

Plasma Physics · Physics 2015-12-17 Mykyta Cherednychek , Alexander Pukhov

The detection of electron motion and electronic wavepacket dynamics is one of the core goals of attosecond science. Recently, choosing the nitric oxide (NO) molecule as an example, we have introduced and demonstrated a new experimental…

Atomic and Molecular Clusters · Physics 2015-04-17 Song Bin Zhang , Denitsa Baykusheva , Peter M. Kraus , Hans Jakob Wörner , Nina Rohringer

High harmonic generation (HHG) in gaseous media provides a robust method for producing coherent extreme-ultraviolet (EUV) radiation and attosecond pulses. However, the spectral and temporal properties of these pulses -- such as bandwidth…

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…

Atomic Physics · Physics 2008-08-14 Anh-Thu Le , Toru Morishita , C. D. Lin

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

Recent advancements in the generation of mid-infrared and terahertz laser pulses have enabled us to observe strong-field driven non-perturbative high-harmonic generation (HHG) from semiconductors, dielectrics, and semimetals. HHG has added…

Optics · Physics 2022-03-22 M. S. Mrudul

In recent publications, it has been shown that high-order harmonic generation can be manipulated by employing a time-delayed attosecond pulse train superposed to a strong, near-infrared laser field. It is an open question, however, which is…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , P. Salieres

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

Recent developments in high-power ultrafast optical technology and emerging theoretical frameworks in strong-field quantum electrodynamics (SF-QED) are unveiling nuanced differentiations between the semi-classical and full quantum…

In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…

We study the linear- and nonlinear-optical lineshapes of metal nanoparticles (theory) and metallic photonic crystal slabs (experiment and theory). For metal nanoparticle ensembles, we show analytically and numerically that femtosecond…

Materials Science · Physics 2007-05-23 M. W. Klein , T. Tritschler , M. Wegener , S. Linden

High Harmonic Generation (HHG) creates coherent high frequency radiation via the process of strong field ionization followed by recombination. Recently, a complementary approach based on Frustrated Tunnel Ionization (FTI) was demonstrated…

Atomic Physics · Physics 2022-04-15 L. Ortmann , C. Hofmann , I. A. Ivanov , A. S. Landsman